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Performance of simulated flexible integrated gasification polygeneration facilities. Part A: A technical-energetic assessment


  • Meerman, J.C.
  • Ramírez, A.
  • Turkenburg, W.C.
  • Faaij, A.P.C.


This article investigates technical possibilities and performances of flexible integrated gasification polygeneration (IG-PG) facilities equipped with CO2 capture for the near future. These facilities can produce electricity during peak hours, while switching to the production of chemicals during off-peak hours. Several simulations were performed to investigate the influence of substituting feedstock and production on IG-PG facility output, load and efficiency. These simulations were done using a detailed AspenPlus simulation model of a Shell entrained flow gasifier combined with conversion facilities. In this model carbon-rich feedstocks (oil residues, coal and biomass) were converted to a variety of products (H2, electricity, FT-liquids, methanol and urea) using state-of-the-art technology. The size of the gasifier was limited to the equivalent of 2000Â MWth Il #6 coal input. Overall efficiency of the simulated non-flexible configurations to convert pure coal or pure wood pellets to electricity (40%HHV vs 38%HHV), FT-liquids (60%HHV vs 55%HHV), methanol (53%HHV vs 49%HHV) or urea (51%HHV vs 47%HHV) are in good agreement with the literature. Using torrefied wood pellets instead of pure wood pellets reduces the penalty drop in efficiency compared to coal. Moreover, torrefied wood pellets have superior energetic density, handling and feeding compared to wood pellets. In this analysis, the H2:CO ratio of the sweet syngas was fixed to match FT-liquids criterion. As a result, overall CO2 capture rates are low, around 56-65%, depending on the feedstock used. Still, especially with FT-liquids and methanol production, CO2 emissions at the facility are significantly reduced; less than 20% of the carbon feedstock entering the facility is emitted with the flue gas. Applying biomass and CO2 capture shows great opportunities to produce CO2-neutral electricity or chemicals. When the biomass fraction exceeds 40% on an energy basis, production is CO2-neutral, independent of what is produced. Biomass can be co-fed up till 50% on an energy basis. Higher fractions cause significant fouling on cooling equipment. A small part-load penalty is observed during the substitution of coal by biomass. When changing from pure coal to pure wood pellets, the power case suffers a 2.5% efficiency drop, while all three chemical cases have an efficiency drop of less than 1%. At the same time total output is reduced to 67-69%, mainly because of the lower energy density of biomass. By over-dimensioning the gasifier and gas cleanup and optimisation section this drop can be eliminated. The syngas can be tailored to the desired composition regardless of the used feedstock. Therefore, the chemical conversion sections only have to cope with a reduction in syngas flow and not with a change in syngas composition. Altering production between chemicals and electricity is possible, although the load of the conversion sections should remain between 40% and 100% to prevent operational problems. This gives a high degree of flexibility. Complete substitution between chemical and power production while using the same feedstock is possible for the methanol and urea cases. The FT-liquids case is restricted to 60-100% load of the chemical conversion section to prevent that the gas turbine load is reduced below 40%. The economic aspects of flexible IG-PG facilities are addressed in part B.

Suggested Citation

  • Meerman, J.C. & Ramírez, A. & Turkenburg, W.C. & Faaij, A.P.C., 2011. "Performance of simulated flexible integrated gasification polygeneration facilities. Part A: A technical-energetic assessment," Renewable and Sustainable Energy Reviews, Elsevier, vol. 15(6), pages 2563-2587, August.
  • Handle: RePEc:eee:rensus:v:15:y:2011:i:6:p:2563-2587

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    Cited by:

    1. Wolfersdorf, Christian & Boblenz, Kristin & Pardemann, Robert & Meyer, Bernd, 2015. "Syngas-based annex concepts for chemical energy storage and improving flexibility of pulverized coal combustion power plants," Applied Energy, Elsevier, vol. 156(C), pages 618-627.
    2. Thallam Thattai, A. & Oldenbroek, V. & Schoenmakers, L. & Woudstra, T. & Aravind, P.V., 2016. "Experimental model validation and thermodynamic assessment on high percentage (up to 70%) biomass co-gasification at the 253MWe integrated gasification combined cycle power plant in Buggenum, The Neth," Applied Energy, Elsevier, vol. 168(C), pages 381-393.
    3. Buttler, Alexander & Kunze, Christian & Spliethoff, Hartmut, 2013. "IGCC–EPI: Decentralized concept of a highly load-flexible IGCC power plant for excess power integration," Applied Energy, Elsevier, vol. 104(C), pages 869-879.
    4. Jana, Kuntal & De, Sudipta, 2015. "Polygeneration using agricultural waste: Thermodynamic and economic feasibility study," Renewable Energy, Elsevier, vol. 74(C), pages 648-660.
    5. Chen, Shiyi & Xiang, Wenguo & Wang, Dong & Xue, Zhipeng, 2012. "Incorporating IGCC and CaO sorption-enhanced process for power generation with CO2 capture," Applied Energy, Elsevier, vol. 95(C), pages 285-294.
    6. repec:eee:appene:v:198:y:2017:i:c:p:180-191 is not listed on IDEAS
    7. Schakel, Wouter & Meerman, Hans & Talaei, Alireza & Ramírez, Andrea & Faaij, André, 2014. "Comparative life cycle assessment of biomass co-firing plants with carbon capture and storage," Applied Energy, Elsevier, vol. 131(C), pages 441-467.
    8. Meerman, J.C. & Ramírez, A. & Turkenburg, W.C. & Faaij, A.P.C., 2012. "Performance of simulated flexible integrated gasification polygeneration facilities, Part B: Economic evaluation," Renewable and Sustainable Energy Reviews, Elsevier, vol. 16(8), pages 6083-6102.
    9. Kaniyal, Ashok A. & van Eyk, Philip J. & Nathan, Graham J., 2016. "Storage capacity assessment of liquid fuels production by solar gasification in a packed bed reactor using a dynamic process model," Applied Energy, Elsevier, vol. 173(C), pages 578-588.
    10. Brouwer, Anne Sjoerd & van den Broek, Machteld & Seebregts, Ad & Faaij, André, 2015. "Operational flexibility and economics of power plants in future low-carbon power systems," Applied Energy, Elsevier, vol. 156(C), pages 107-128.
    11. Farhat, Karim & Reichelstein, Stefan, 2016. "Economic value of flexible hydrogen-based polygeneration energy systems," Applied Energy, Elsevier, vol. 164(C), pages 857-870.
    12. repec:eee:appene:v:202:y:2017:i:c:p:88-111 is not listed on IDEAS
    13. Kohl, Thomas & Laukkanen, Timo & Järvinen, Mika & Fogelholm, Carl-Johan, 2013. "Energetic and environmental performance of three biomass upgrading processes integrated with a CHP plant," Applied Energy, Elsevier, vol. 107(C), pages 124-134.


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