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Gas separation of flue gas by tetra-n-butylammonium bromide hydrates under moderate pressure conditions

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  • Hashimoto, Hidenori
  • Yamaguchi, Tsutomu
  • Kinoshita, Takahiro
  • Muromachi, Sanehiro

Abstract

Ionic clathrate hydrates are composed of water and ionic guest substance, which can selectively capture gas under moderate conditions. We performed gas separation experiments with tetra-n-butylammonium bromide (TBAB) widely-used for an ionic guest substance. The experiments in a closed system showed good CO2 gas selectivity of the TBAB hydrates even under the mild conditions: 1 MPa and 282 K. We also performed the gas separation with tetrahydrofuran (THF) which is a guest substance forming the structure II clathrate hydrate. Comparison with THF clearly revealed the better CO2 selectivity of TBAB than that of the structure II clathrate hydrate. We further compared our data with the literature, and found that the condition of low pressure and dense TBAB concentration provided superior CO2 selectivity. Gas separation with continuous gas flow was demonstrated. The hydrate formation behavior was similar to the cases without gas flow. The results showed that controlling the crystal growth temperature is important to capture gases by the TBAB hydrates.

Suggested Citation

  • Hashimoto, Hidenori & Yamaguchi, Tsutomu & Kinoshita, Takahiro & Muromachi, Sanehiro, 2017. "Gas separation of flue gas by tetra-n-butylammonium bromide hydrates under moderate pressure conditions," Energy, Elsevier, vol. 129(C), pages 292-298.
    • Handle: RePEc:eee:energy:v:129:y:2017:i:c:p:292-298
    DOI: 10.1016/j.energy.2017.04.074
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    Cited by:

    1. Wu, Yongji & He, Yurong & Tang, Tianqi & Zhai, Ming, 2023. "Molecular dynamic simulations of methane hydrate formation between solid surfaces: Implications for methane storage," Energy, Elsevier, vol. 262(PB).
    2. Wang, Yan & Zhong, Dong-Liang & Englezos, Peter & Yan, Jin & Ge, Bin-Bin, 2020. "Kinetic study of semiclathrate hydrates formed with CO2 in the presence of tetra-n-butyl ammonium bromide and tetra-n-butyl phosphonium bromide," Energy, Elsevier, vol. 212(C).
    3. Muromachi, Sanehiro, 2021. "CO2 capture properties of semiclathrate hydrates formed with tetra-n-butylammonium and tetra-n-butylphosphonium salts from H2 + CO2 mixed gas," Energy, Elsevier, vol. 223(C).
    4. Yang, Mingjun & Zhou, Hang & Wang, Pengfei & Song, Yongchen, 2018. "Effects of additives on continuous hydrate-based flue gas separation," Applied Energy, Elsevier, vol. 221(C), pages 374-385.
    5. Wang, Yiwei & Deng, Ye & Guo, Xuqiang & Sun, Qiang & Liu, Aixian & Zhang, Guangqing & Yue, Gang & Yang, Lanying, 2018. "Experimental and modeling investigation on separation of methane from coal seam gas (CSG) using hydrate formation," Energy, Elsevier, vol. 150(C), pages 377-395.
    6. Zhang, Qiang & Zheng, Junjie & Zhang, Baoyong & Linga, Praveen, 2023. "Kinetic evaluation of hydrate-based coalbed methane recovery process promoted by structure II thermodynamic promoters and amino acids," Energy, Elsevier, vol. 274(C).
    7. Sa, Jeong-Hoon & Sum, Amadeu K., 2019. "Promoting gas hydrate formation with ice-nucleating additives for hydrate-based applications," Applied Energy, Elsevier, vol. 251(C), pages 1-1.
    8. Wang, Yan & Zhong, Dong-Liang & Li, Zheng & Li, Jian-Bo, 2020. "Application of tetra-n-butyl ammonium bromide semi-clathrate hydrate for CO2 capture from unconventional natural gases," Energy, Elsevier, vol. 197(C).
    9. Satoshi Takeya & Sanehiro Muromachi & Tatsuo Maekawa & Yoshitaka Yamamoto & Hiroko Mimachi & Takahiro Kinoshita & Tetsuro Murayama & Hiroki Umeda & Dong-Hyuk Ahn & Yasunaga Iwasaki & Hidenori Hashimot, 2017. "Design of Ecological CO 2 Enrichment System for Greenhouse Production using TBAB + CO 2 Semi-Clathrate Hydrate," Energies, MDPI, vol. 10(7), pages 1-12, July.

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