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Recycling of lithium iron phosphate batteries: Status, technologies, challenges, and prospects

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  • Wang, Mengmeng
  • Liu, Kang
  • Dutta, Shanta
  • Alessi, Daniel S.
  • Rinklebe, Jörg
  • Ok, Yong Sik
  • Tsang, Daniel C.W.

Abstract

The limited fossil fuel supply toward carbon neutrality has driven tremendous efforts to replace fuel vehicles by electric ones. The recycling of retired power batteries, a core energy supply component of electric vehicles (EVs), is necessary for developing a sustainable EV industry. Here, we comprehensively review the current status and technical challenges of recycling lithium iron phosphate (LFP) batteries. The review focuses on: 1) environmental risks of LFP batteries, 2) cascade utilization, 3) separation of cathode material and aluminium foil, 4) lithium (Li) extraction technologies, and 5) regeneration and transformation of cathode materials. Detailed analyses are elaborated with case examples and technical challenges. Our critical analysis demonstrates that compared with retired lithium nickel cobalt manganese oxide (NCM) batteries, LFP batteries do not contain the high-value elements such as Co and Ni, so the economic drive for LFP recycling is compromised although future market prospects are substantial. It is of great practical significance to develop low-carbon and cost-effective Li extraction technologies and regeneration processes for cathode materials to ensure a sustainable and stable development of the LFP battery and EV industry.

Suggested Citation

  • Wang, Mengmeng & Liu, Kang & Dutta, Shanta & Alessi, Daniel S. & Rinklebe, Jörg & Ok, Yong Sik & Tsang, Daniel C.W., 2022. "Recycling of lithium iron phosphate batteries: Status, technologies, challenges, and prospects," Renewable and Sustainable Energy Reviews, Elsevier, vol. 163(C).
    • Handle: RePEc:eee:rensus:v:163:y:2022:i:c:s1364032122004191
    DOI: 10.1016/j.rser.2022.112515
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    1. Ingeborgrud, Lina & Ryghaug, Marianne, 2019. "The role of practical, cognitive and symbolic factors in the successful implementation of battery electric vehicles in Norway," Transportation Research Part A: Policy and Practice, Elsevier, vol. 130(C), pages 507-516.
    2. Gavin Harper & Roberto Sommerville & Emma Kendrick & Laura Driscoll & Peter Slater & Rustam Stolkin & Allan Walton & Paul Christensen & Oliver Heidrich & Simon Lambert & Andrew Abbott & Karl Ryder & L, 2019. "Recycling lithium-ion batteries from electric vehicles," Nature, Nature, vol. 575(7781), pages 75-86, November.
    3. Liu, Wenqiu & Liu, He & Liu, Wei & Cui, Zhaojie, 2021. "Life cycle assessment of power batteries used in electric bicycles in China," Renewable and Sustainable Energy Reviews, Elsevier, vol. 139(C).
    4. Wang, Qian & Jiang, Bin & Li, Bo & Yan, Yuying, 2016. "A critical review of thermal management models and solutions of lithium-ion batteries for the development of pure electric vehicles," Renewable and Sustainable Energy Reviews, Elsevier, vol. 64(C), pages 106-128.
    5. Martinez-Laserna, E. & Gandiaga, I. & Sarasketa-Zabala, E. & Badeda, J. & Stroe, D.-I. & Swierczynski, M. & Goikoetxea, A., 2018. "Battery second life: Hype, hope or reality? A critical review of the state of the art," Renewable and Sustainable Energy Reviews, Elsevier, vol. 93(C), pages 701-718.
    6. Schulz, Felix & Rode, Johannes, 2022. "Public charging infrastructure and electric vehicles in Norway," Energy Policy, Elsevier, vol. 160(C).
    7. Gulley, Andrew L. & McCullough, Erin A. & Shedd, Kim B., 2019. "China's domestic and foreign influence in the global cobalt supply chain," Resources Policy, Elsevier, vol. 62(C), pages 317-323.
    8. Zeng, Xianlai & Li, Jinhui & Liu, Lili, 2015. "Solving spent lithium-ion battery problems in China: Opportunities and challenges," Renewable and Sustainable Energy Reviews, Elsevier, vol. 52(C), pages 1759-1767.
    9. Richard Schmuch & Ralf Wagner & Gerhard Hörpel & Tobias Placke & Martin Winter, 2018. "Performance and cost of materials for lithium-based rechargeable automotive batteries," Nature Energy, Nature, vol. 3(4), pages 267-278, April.
    10. Joeri Rogelj & Michel den Elzen & Niklas Höhne & Taryn Fransen & Hanna Fekete & Harald Winkler & Roberto Schaeffer & Fu Sha & Keywan Riahi & Malte Meinshausen, 2016. "Paris Agreement climate proposals need a boost to keep warming well below 2 °C," Nature, Nature, vol. 534(7609), pages 631-639, June.
    11. Shareef, Hussain & Islam, Md. Mainul & Mohamed, Azah, 2016. "A review of the stage-of-the-art charging technologies, placement methodologies, and impacts of electric vehicles," Renewable and Sustainable Energy Reviews, Elsevier, vol. 64(C), pages 403-420.
    12. Chai, Wai Siong & Bao, Yulei & Jin, Pengfei & Tang, Guang & Zhou, Lei, 2021. "A review on ammonia, ammonia-hydrogen and ammonia-methane fuels," Renewable and Sustainable Energy Reviews, Elsevier, vol. 147(C).
    13. Yu, Haijun & Dai, Hongliang & Tian, Guangdong & Wu, Benben & Xie, Yinghao & Zhu, Ying & Zhang, Tongzhu & Fathollahi-Fard, Amir Mohammad & He, Qi & Tang, Hong, 2021. "Key technology and application analysis of quick coding for recovery of retired energy vehicle battery," Renewable and Sustainable Energy Reviews, Elsevier, vol. 135(C).
    14. Ordoñez, J. & Gago, E.J. & Girard, A., 2016. "Processes and technologies for the recycling and recovery of spent lithium-ion batteries," Renewable and Sustainable Energy Reviews, Elsevier, vol. 60(C), pages 195-205.
    15. Wang, Jiajia & Yue, Xiyan & Wang, Peifen & Yu, Tao & Du, Xiao & Hao, Xiaogang & Abudula, Abuliti & Guan, Guoqing, 2022. "Electrochemical technologies for lithium recovery from liquid resources: A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 154(C).
    16. Rebecca E. Ciez & J. F. Whitacre, 2019. "Examining different recycling processes for lithium-ion batteries," Nature Sustainability, Nature, vol. 2(2), pages 148-156, February.
    17. Lai, Xin & Huang, Yunfeng & Deng, Cong & Gu, Huanghui & Han, Xuebing & Zheng, Yuejiu & Ouyang, Minggao, 2021. "Sorting, regrouping, and echelon utilization of the large-scale retired lithium batteries: A critical review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 146(C).
    18. Wang, Wei & Wu, Yufeng, 2017. "An overview of recycling and treatment of spent LiFePO4 batteries in China," Resources, Conservation & Recycling, Elsevier, vol. 127(C), pages 233-243.
    19. Joeri Rogelj & Oliver Geden & Annette Cowie & Andy Reisinger, 2021. "Net-zero emissions targets are vague: three ways to fix," Nature, Nature, vol. 591(7850), pages 365-368, March.
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