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Synergistic effect of the co-pyrolysis of cardboard and polyethylene: A kinetic and thermodynamic study

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  • Wen, Yuming
  • Zaini, Ilman Nuran
  • Wang, Shule
  • Mu, Wangzhong
  • Jönsson, Pär Göran
  • Yang, Weihong

Abstract

Pyrolysis of municipal solid waste (MSW) represents one of the most promising solutions to recycle materials and recover energy. Two of the main components of MSW are waste cardboard and plastic. In this study, the pyrolysis of cardboard and polyethylene (PE) and the co-pyrolysis of their mixtures were conducted to investigate the synergistic effect by using thermogravimetric analysis. The whole reaction process was divided into four pseudoreactions, namely, hemicellulose, lignin, cellulose, and PE, by using the Frazer-Suzuki deconvolution method. It was found that the co-pyrolysis of cardboard and PE could promote the decomposition degrees of cardboard from 70.28% to 75.31%, when the PE fraction increased from 0 to 75%. However, the presence of cardboard can hinder the heat adsorption of PE, which shifts the peak of the PE reaction to a higher temperature. This results in higher Ea and ΔH‡ values for PE pyrolysis with an increasing fraction of cardboard. On the other hand, the Ea and ΔH‡ values of cellulose pyrolysis have their lowest values when the mixing rate is around 50%. This research deepens the understanding of the synergistic effect of co-pyrolysis of cardboard and PE, which supports the potential application of pyrolysis of MSW.

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  • Wen, Yuming & Zaini, Ilman Nuran & Wang, Shule & Mu, Wangzhong & Jönsson, Pär Göran & Yang, Weihong, 2021. "Synergistic effect of the co-pyrolysis of cardboard and polyethylene: A kinetic and thermodynamic study," Energy, Elsevier, vol. 229(C).
    • Handle: RePEc:eee:energy:v:229:y:2021:i:c:s0360544221009415
    DOI: 10.1016/j.energy.2021.120693
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    1. Pan, Ruming & Martins, Marcio Ferreira & Debenest, Gérald, 2022. "Optimization of oil production through ex-situ catalytic pyrolysis of waste polyethylene with activated carbon," Energy, Elsevier, vol. 248(C).
    2. Stančin, H. & Mikulčić, H. & Manić, N. & Stojiljiković, D. & Vujanović, M. & Wang, X. & Duić, N., 2021. "Thermogravimetric and kinetic analysis of biomass and polyurethane foam mixtures Co-Pyrolysis," Energy, Elsevier, vol. 237(C).
    3. Mariyam, Sabah & Shahbaz, Muhammad & Al-Ansari, Tareq & Mackey, Hamish. R & McKay, Gordon, 2022. "A critical review on co-gasification and co-pyrolysis for gas production," Renewable and Sustainable Energy Reviews, Elsevier, vol. 161(C).
    4. Zhang, Wenqi & Zhou, Renjie & Gao, Shuaifei & Wang, Yinfeng & Zhu, Lin & Gao, Ying & Zhu, Yuezhao, 2022. "Investigation on cogasification and melting behavior of ash-rich biomass solid waste and Ca-rich petrochemical sludge pyrolysis residue in CO2 atmosphere," Energy, Elsevier, vol. 239(PB).

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