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Mitigation effects on thermal runaway propagation of structure-enhanced phase change material modules with flame retardant additives

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  • Weng, Jingwen
  • Xiao, Changren
  • Ouyang, Dongxu
  • Yang, Xiaoqing
  • Chen, Mingyi
  • Zhang, Guoqing
  • Yuen, Richard Kwok Kit
  • Wang, Jian

Abstract

Majority existing organic composite phase change materials (CPCMs) are flammable that result in thermal hazards such as fire and explosions in battery modules. Furthermore, the performance of PCM-based battery modules in extreme conditions like thermal runaway has not been studied adequately. In this study, a tubular CPCM-cell structure is designed using physically flame-retardant-modified CPCMs, and a series of experiments on the CPCMs with/without real cells is conducted with calorimeter tests and SEM analysis on morphology structure. First, the calorimeter tests and comparison on the heat release rate (HRR) are conducted on the CPCMs with and without flame retardant additives. Results show that the addition of Al(OH)3 reduced the HRR from 242.5 to 204.4 kW/m2 with 15 wt% additives. Besides, the analysis of the mitigating performances of structure-enhanced tubular module and traditional cuboid module with real batteries is conducted. A factor of safety (FOS) parameter is defined to evaluate the safety degree of thermal runaway domino with energy density. The FOS of blank, CPCM–0C, and CPCM–15C modules are 0, 3.59, and 16.67, respectively, while that of CPCM-15T reaches 21.01, indicating a significant improvement on mitigating effects by structure enhancement compared to adding flame retardant additives. This study brings novelty in the design of PCM-based battery modules, particularly from the thermal safety prospect.

Suggested Citation

  • Weng, Jingwen & Xiao, Changren & Ouyang, Dongxu & Yang, Xiaoqing & Chen, Mingyi & Zhang, Guoqing & Yuen, Richard Kwok Kit & Wang, Jian, 2022. "Mitigation effects on thermal runaway propagation of structure-enhanced phase change material modules with flame retardant additives," Energy, Elsevier, vol. 239(PC).
    • Handle: RePEc:eee:energy:v:239:y:2022:i:pc:s0360544221023355
    DOI: 10.1016/j.energy.2021.122087
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    1. Yilin Cui & Yin Chen & Luyao Zhao & Fang Zhu & Lixia Li & Qinghong Kong & Mingyi Chen, 2023. "Investigation on the Properties of Flame-Retardant Phase Change Material and Its Application in Battery Thermal Management," Energies, MDPI, vol. 16(1), pages 1-17, January.
    2. Hong Shi & Mengmeng Cheng & Yi Feng & Chenghui Qiu & Caiyue Song & Nenglin Yuan & Chuanzhi Kang & Kaijie Yang & Jie Yuan & Yonghao Li, 2023. "Thermal Management Techniques for Lithium-Ion Batteries Based on Phase Change Materials: A Systematic Review and Prospective Recommendations," Energies, MDPI, vol. 16(2), pages 1-23, January.
    3. Jia, Zhuangzhuang & Huang, Zonghou & Zhai, Hongju & Qin, Pen & Zhang, Yue & Li, Yawen & Wang, Qingsong, 2022. "Experimental investigation on thermal runaway propagation of 18,650 lithium-ion battery modules with two cathode materials at low pressure," Energy, Elsevier, vol. 251(C).
    4. Fan, Zhaohui & Gao, Renjing & Liu, Shutian, 2022. "Thermal conductivity enhancement and thermal saturation elimination designs of battery thermal management system for phase change materials based on triply periodic minimal surface," Energy, Elsevier, vol. 259(C).
    5. Hongxu Li & Qing Gao & Yan Wang, 2023. "Experimental Investigation of the Thermal Runaway Propagation Characteristics and Thermal Failure Prediction Parameters of Six-Cell Lithium-Ion Battery Modules," Energies, MDPI, vol. 16(13), pages 1-14, July.

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