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Long-term performance degradation study of solid oxide carbon fuel cells integrated with a steam gasifier

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  • Mehran, Muhammad Taqi
  • Lim, Tak-Hyoung
  • Lee, Seung-Bok
  • Lee, Jong-Won
  • Park, Seok-Ju
  • Song, Rak-Hyun

Abstract

We investigated the long-term performance degradation in a solid oxide carbon fuel cell (SO-CFC) integrated with a steam gasifier that used activated carbon as a fuel. The steam gasifier-integrated SO-CFC was continuously operated for 2000 h at 750 °C under galvanostatic conditions. Fuel analysis, in-situ electrochemical tests, and post-mortem characterization were performed to determine the dominant degradation factors during the extended operation of the SO-CFC. During the 2000 h continuous operation, the overall degradation rate of the SO-CFC was 0.108 V per 1000 h. Electrochemical impedance spectroscopy analysis showed that the polarization and ohmic resistance of the SO-CFC increased gradually with the operation time. The post-mortem diagnosis via SEM, XRD, EDS, and XPS analyses revealed that the increased Ni particle coarsening and carbon deposition at the anode functional layer induced increased performance degradation in the SO-CFC. The long-term durability study of the SO-CFC with a steam gasifier confirmed that conventional anode materials result in rapid performance degradation during 2000 h continuous operation, and further development of anode materials will be necessary for the long and durable operation of SO-CFCs.

Suggested Citation

  • Mehran, Muhammad Taqi & Lim, Tak-Hyoung & Lee, Seung-Bok & Lee, Jong-Won & Park, Seok-Ju & Song, Rak-Hyun, 2016. "Long-term performance degradation study of solid oxide carbon fuel cells integrated with a steam gasifier," Energy, Elsevier, vol. 113(C), pages 1051-1061.
    • Handle: RePEc:eee:energy:v:113:y:2016:i:c:p:1051-1061
    DOI: 10.1016/j.energy.2016.07.087
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    References listed on IDEAS

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    Cited by:

    1. Rashid, Kashif & Dong, Sang Keun & Mehran, Muhammad Taqi, 2017. "Numerical investigations to determine the optimal operating conditions for 1 kW-class flat-tubular solid oxide fuel cell stack," Energy, Elsevier, vol. 141(C), pages 673-691.
    2. Eom, Seongyong & Ahn, Seongyool & Kang, Kijoong & Choi, Gyungmin, 2017. "Correlations between electrochemical resistances and surface properties of acid-treated fuel in coal fuel cells," Energy, Elsevier, vol. 140(P1), pages 885-892.
    3. Yan, Dong & Liang, Lingjiang & Yang, Jiajun & Zhang, Tao & Pu, Jian & Chi, Bo & Li, Jian, 2017. "Performance degradation and analysis of 10-cell anode-supported SOFC stack with external manifold structure," Energy, Elsevier, vol. 125(C), pages 663-670.
    4. Mushtaq, Usman & Mehran, Muhammad Taqi & Kim, Sun-Kyoung & Lim, Tak-Hyoung & Naqvi, Syed Asad Ali & Lee, Jong-Won & Lee, Seung-Bok & Park, Seok-Joo & Song, Rak-Hyun, 2017. "Evaluation of steady-state characteristics for solid oxide carbon fuel cell short-stacks," Applied Energy, Elsevier, vol. 187(C), pages 886-898.
    5. Yang, JiaJun & Yan, Dong & Huang, Wei & Li, Jun & Pu, Jian & Chi, Bo & Jian, Li, 2018. "Improvement on durability and thermal cycle performance for solid oxide fuel cell stack with external manifold structure," Energy, Elsevier, vol. 149(C), pages 903-913.
    6. Mehran, Muhammad Taqi & Yu, Seong-Bin & Lee, Dong-Young & Hong, Jong-Eun & Lee, Seung-Bok & Park, Seok-Joo & Song, Rak-Hyun & Lim, Tak-Hyoung, 2018. "Production of syngas from H2O/CO2 by high-pressure coelectrolysis in tubular solid oxide cells," Applied Energy, Elsevier, vol. 212(C), pages 759-770.
    7. Tanveer, Waqas Hassan & Abdelkareem, Mohammad Ali & Kolosz, Ben W. & Rezk, Hegazy & Andresen, John & Cha, Suk Won & Sayed, Enas Taha, 2021. "The role of vacuum based technologies in solid oxide fuel cell development to utilize industrial waste carbon for power production," Renewable and Sustainable Energy Reviews, Elsevier, vol. 142(C).
    8. Lee, Dong-Young & Mehran, Muhammad Taqi & Kim, Jonghwan & Kim, Sangcho & Lee, Seung-Bok & Song, Rak-Hyun & Ko, Eun-Yong & Hong, Jong-Eun & Huh, Joo-Youl & Lim, Tak-Hyoung, 2020. "Scaling up syngas production with controllable H2/CO ratio in a highly efficient, compact, and durable solid oxide coelectrolysis cell unit-bundle," Applied Energy, Elsevier, vol. 257(C).
    9. Tanveer, Waqas Hassan & Rezk, Hegazy & Nassef, Ahmed & Abdelkareem, Mohammad Ali & Kolosz, Ben & Karuppasamy, K. & Aslam, Jawad & Gilani, Syed Omer, 2020. "Improving fuel cell performance via optimal parameters identification through fuzzy logic based-modeling and optimization," Energy, Elsevier, vol. 204(C).

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