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Simulation and analysis of CO2 capture process with aqueous monoethanolamine solution

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  • Li, Bao-Hong
  • Zhang, Nan
  • Smith, Robin

Abstract

An improved rate-based model of the typical CO2 capture process by aqueous MonoEthanolAmine (MEA) solution is built within Aspen Plus V8.0 software in this study. The improved model is built on the basis of an example model coming along with Aspen Plus V8.0, and thermodynamic model of ENRTL-RK is adopted. Improvements include the washing section of the absorption column is strictly modelled by a separate column, and the error on mass balance of MEA is greatly reduced. The new model is validated by the recently published pilot-scale experimental results of the absorption of CO2 by MEA solution, in which both absorption and desorption columns are equipped with the structured packing Sulzer Mellapak 250.Y™. It predicts the experimental profiles of the temperature and the concentration of CO2 in the liquid phase with an accuracy of ±4%, and obviously much better than recently reported model with an accuracy of ±8%. Important insights have been obtained on the function of washing sections on the top of both absorber and desorption column, the factors to determine the flowrates of make-up water and recycle water around the washing section of the absorber are first analyzed.

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  • Li, Bao-Hong & Zhang, Nan & Smith, Robin, 2016. "Simulation and analysis of CO2 capture process with aqueous monoethanolamine solution," Applied Energy, Elsevier, vol. 161(C), pages 707-717.
    • Handle: RePEc:eee:appene:v:161:y:2016:i:c:p:707-717
    DOI: 10.1016/j.apenergy.2015.07.010
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    1. Zhang, Minkai & Guo, Yincheng, 2013. "Rate based modeling of absorption and regeneration for CO2 capture by aqueous ammonia solution," Applied Energy, Elsevier, vol. 111(C), pages 142-152.
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    15. Juan Camilo Solarte-Toro & Carlos Ariel Cardona Alzate, 2023. "Sustainability of Biorefineries: Challenges and Perspectives," Energies, MDPI, vol. 16(9), pages 1-24, April.
    16. Farajollahi, Hossein & Hossainpour, Siamak, 2017. "Application of organic Rankine cycle in integration of thermal power plant with post-combustion CO2 capture and compression," Energy, Elsevier, vol. 118(C), pages 927-936.
    17. Madeddu, Claudio & Errico, Massimiliano & Baratti, Roberto, 2018. "Process analysis for the carbon dioxide chemical absorption–regeneration system," Applied Energy, Elsevier, vol. 215(C), pages 532-542.
    18. Yi, Qun & Zhao, Yingjie & Huang, Yi & Wei, Guoqiang & Hao, Yanhong & Feng, Jie & Mohamed, Usama & Pourkashanian, Mohamed & Nimmo, William & Li, Wenying, 2018. "Life cycle energy-economic-CO2 emissions evaluation of biomass/coal, with and without CO2 capture and storage, in a pulverized fuel combustion power plant in the United Kingdom," Applied Energy, Elsevier, vol. 225(C), pages 258-272.
    19. Chuenphan, Thapanat & Yurata, Tarabordin & Sema, Teerawat & Chalermsinsuwan, Benjapon, 2022. "Techno-economic sensitivity analysis for optimization of carbon dioxide capture process by potassium carbonate solution," Energy, Elsevier, vol. 254(PA).
    20. Huang, Weijia & Zheng, Danxing & Xie, Hui & Li, Yun & Wu, Weize, 2019. "Hybrid physical-chemical absorption process for carbon capture with strategy of high-pressure absorption/medium-pressure desorption," Applied Energy, Elsevier, vol. 239(C), pages 928-937.
    21. Al-Kalbani, Haitham & Xuan, Jin & García, Susana & Wang, Huizhi, 2016. "Comparative energetic assessment of methanol production from CO2: Chemical versus electrochemical process," Applied Energy, Elsevier, vol. 165(C), pages 1-13.

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    Keywords

    CO2 capture; Reactive absorption; MEA; Simulation;
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