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Alternative production of methanol from industrial CO2

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  • Meunier, Nicolas
  • Chauvy, Remi
  • Mouhoubi, Seloua
  • Thomas, Diane
  • De Weireld, Guy

Abstract

Carbon dioxide valorization into value added products have become subject to much study to reduce industrial CO2 emissions and fossil energy resource consumption. In this context, the purpose of this study is to evaluate and highlight the interest of CO2 conversion into methanol through a complete techno-economic and environmental assessment of the entire process chain. The integrated process, successfully implemented in Aspen Plus®, is designed to treat the CO2 coming from a conventional cement plant. A MEA-based CO2 capture process is considered, and the captured CO2 is then directly sent to the conversion unit for its catalytic conversion. Consequently, combining the two units leads to relevant integrations, especially regarding the reuse of the heat provided by the exothermal methanol reactions for the regeneration of the CO2 capture solvent. An economic assessment is proposed to estimate the operational and investment costs, as well as the net present value, which demonstrates that the economic feasibility strongly depends on electricity and H2 production costs. A Life Cycle Analysis method is finally performed to identify the main environmental hotspots. The underlying process design offers a significant reduction in greenhouse gases (besides other categories) when compared to the conventional fossil production from natural gas.

Suggested Citation

  • Meunier, Nicolas & Chauvy, Remi & Mouhoubi, Seloua & Thomas, Diane & De Weireld, Guy, 2020. "Alternative production of methanol from industrial CO2," Renewable Energy, Elsevier, vol. 146(C), pages 1192-1203.
    • Handle: RePEc:eee:renene:v:146:y:2020:i:c:p:1192-1203
    DOI: 10.1016/j.renene.2019.07.010
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    References listed on IDEAS

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    1. Oh, Se-Young & Binns, Michael & Cho, Habin & Kim, Jin-Kuk, 2016. "Energy minimization of MEA-based CO2 capture process," Applied Energy, Elsevier, vol. 169(C), pages 353-362.
    2. Bruhn, Thomas & Naims, Henriette & Olfe-Kräutlein, Barbara, 2016. "Separating the debate on CO2 utilisation from carbon capture and storage," Environmental Science & Policy, Elsevier, vol. 60(C), pages 38-43.
    3. Pérez-Fortes, Mar & Schöneberger, Jan C. & Boulamanti, Aikaterini & Tzimas, Evangelos, 2016. "Methanol synthesis using captured CO2 as raw material: Techno-economic and environmental assessment," Applied Energy, Elsevier, vol. 161(C), pages 718-732.
    4. Li, Bao-Hong & Zhang, Nan & Smith, Robin, 2016. "Simulation and analysis of CO2 capture process with aqueous monoethanolamine solution," Applied Energy, Elsevier, vol. 161(C), pages 707-717.
    5. Niall Mac Dowell & Paul S. Fennell & Nilay Shah & Geoffrey C. Maitland, 2017. "The role of CO2 capture and utilization in mitigating climate change," Nature Climate Change, Nature, vol. 7(4), pages 243-249, April.
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