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The Oxy-CaL process: A novel CO2 capture system by integrating partial oxy-combustion with the Calcium-Looping process

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  • Ortiz, C.
  • Valverde, J.M.
  • Chacartegui, R.
  • Benítez-Guerrero, M.
  • Perejón, A.
  • Romeo, L.M.

Abstract

This paper proposes a novel CO2 capture technology from the integration of partial oxy-combustion and the Calcium-Looping capture process based on the multicycle carbonation/calcination of limestone derived CaO. The concentration of CO2 in the carbonator reactor is increased by means of partial oxy-combustion, which enhances the multicycle CaO conversion according to thermogravimetric analysis results carried out in our work, thus improving the CO2 capture efficiency. On the other hand, energy consumption for partial oxy-combustion is substantially reduced as compared to total oxy-combustion. All in all, process simulations indicate that the integration of both processes has potential advantages mainly regarding power plant flexibility whereas the overall energy penalty is not increased. Thus, the resulting energy consumption per kilogram of CO2 avoided is kept smaller than 4MJ/kg CO2, which remains below the typical values reported for total oxy-combustion and amine based CO2 capture systems whereas CO2 capture efficiency is enhanced in comparison with the Calcium-Looping process.

Suggested Citation

  • Ortiz, C. & Valverde, J.M. & Chacartegui, R. & Benítez-Guerrero, M. & Perejón, A. & Romeo, L.M., 2017. "The Oxy-CaL process: A novel CO2 capture system by integrating partial oxy-combustion with the Calcium-Looping process," Applied Energy, Elsevier, vol. 196(C), pages 1-17.
    • Handle: RePEc:eee:appene:v:196:y:2017:i:c:p:1-17
    DOI: 10.1016/j.apenergy.2017.03.120
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    1. García-Luna, S. & Ortiz, C. & Chacartegui, R. & Pérez-Maqueda, L.A., 2023. "Large-scale oxygen-enriched air (OEA) production from polymeric membranes for partial oxycombustion processes," Energy, Elsevier, vol. 268(C).
    2. Benitez-Guerrero, Monica & Valverde, Jose Manuel & Perejon, Antonio & Sanchez-Jimenez, Pedro E. & Perez-Maqueda, Luis A., 2018. "Low-cost Ca-based composites synthesized by biotemplate method for thermochemical energy storage of concentrated solar power," Applied Energy, Elsevier, vol. 210(C), pages 108-116.
    3. Zhang, Shihan & Shen, Yao & Wang, Lidong & Chen, Jianmeng & Lu, Yongqi, 2019. "Phase change solvents for post-combustion CO2 capture: Principle, advances, and challenges," Applied Energy, Elsevier, vol. 239(C), pages 876-897.
    4. Ortiz, C. & García-Luna, S. & Carro, A. & Chacartegui, R. & Pérez-Maqueda, L., 2023. "Negative emissions power plant based on flexible calcium-looping process integrated with renewables and methane production," Renewable and Sustainable Energy Reviews, Elsevier, vol. 185(C).
    5. Niu, Yanqing & Yan, Bokang & Liu, Siqi & Liang, Yang & Dong, Ning & Hui, Shi'en, 2018. "Ultra-fine particulate matters (PMs) formation during air and oxy-coal combustion: Kinetics study," Applied Energy, Elsevier, vol. 218(C), pages 46-53.
    6. Zhang, Wan & Li, Yingjie & He, Zirui & Ma, Xiaotong & Song, Haiping, 2017. "CO2 capture by carbide slag calcined under high-concentration steam and energy requirement in calcium looping conditions," Applied Energy, Elsevier, vol. 206(C), pages 869-878.

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