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High-efficiency negative-carbon emission power generation from integrated solid-oxide fuel cell and calciner

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  • Hanak, Dawid P.
  • Jenkins, Barrie G.
  • Kruger, Tim
  • Manovic, Vasilije

Abstract

Direct air capture of CO2 has the potential to help meet the ambitious environmental targets established by the Paris Agreement. This study assessed the techno-economic feasibility of a process for simultaneous power generation and CO2 removal from the air using solid sorbents. The process uses a solid-oxide fuel cell to convert the chemical energy of fuel to electricity and high-grade heat, the latter of which can be utilised to calcine a carbonate material that, in turn, can remove CO2 from the air. The proposed process was shown to operate with a net thermal efficiency of 43.7–47.7%LHV and to have the potential to remove 463.5–882.3 gCO2/kWelh, depending on the fresh material used in the calciner. Importantly, the estimated capital cost of the proposed process (1397.9–1740.5 £/kWel,gross) was found to be lower than that for other low-carbon emission power generation systems using fossil fuels. The proposed process was also shown to achieve a levelised cost of electricity of 50 £/MWelh, which is competitive with other low-carbon power generation technologies, for a carbon tax varying between 39.2 and 74.9 £/tCO2. Such figure associated with the levelised cost of CO2 capture from air is lower than for other direct air concepts.

Suggested Citation

  • Hanak, Dawid P. & Jenkins, Barrie G. & Kruger, Tim & Manovic, Vasilije, 2017. "High-efficiency negative-carbon emission power generation from integrated solid-oxide fuel cell and calciner," Applied Energy, Elsevier, vol. 205(C), pages 1189-1201.
    • Handle: RePEc:eee:appene:v:205:y:2017:i:c:p:1189-1201
    DOI: 10.1016/j.apenergy.2017.08.090
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