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Thermal runaway potential of LiCoO2 and Li(Ni1/3Co1/3Mn1/3)O2 batteries determined with adiabatic calorimetry methodology

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  • Jhu, Can-Yong
  • Wang, Yih-Wen
  • Wen, Chia-Yuan
  • Shu, Chi-Min

Abstract

Thermal runaway hazards related to adiabatic runaway reactions in various 18650 Li-ion batteries were studied in an adiabatic calorimeter with vent sizing package 2 (VSP2). We selected two cathode types, LiCoO2 and Li(Ni1/3Co1/3Mn1/3)O2, and tested Li-ion batteries to determine the thermal runaway features. The charged 18650 Li-ion batteries were tested to evaluate the thermal hazard characteristics, such as the initial exothermic temperature (T0), self-heating rate (dT/dt), pressure rise rate (dP/dt), pressure–temperature profiles, maximum temperature (Tmax) and pressure (Pmax), which are measured by VSP2 with a customized stainless steel test can. The thermal reaction behaviors of the Li-ion battery packs were shown to be an important safety concern for energy storage systems for power supply applications. The thermal abuse trials of the adiabatic calorimetry methodology used to classify the self-reactive ratings of the various cathodes for Li-ion batteries provided the safety design considerations.

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  • Jhu, Can-Yong & Wang, Yih-Wen & Wen, Chia-Yuan & Shu, Chi-Min, 2012. "Thermal runaway potential of LiCoO2 and Li(Ni1/3Co1/3Mn1/3)O2 batteries determined with adiabatic calorimetry methodology," Applied Energy, Elsevier, vol. 100(C), pages 127-131.
    • Handle: RePEc:eee:appene:v:100:y:2012:i:c:p:127-131
    DOI: 10.1016/j.apenergy.2012.05.064
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    Cited by:

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    12. Chen, Jie & Ren, Dongsheng & Hsu, Hungjen & Wang, Li & He, Xiangming & Zhang, Caiping & Feng, Xuning & Ouyang, Minggao, 2021. "Investigating the thermal runaway features of lithium-ion batteries using a thermal resistance network model," Applied Energy, Elsevier, vol. 295(C).
    13. Liu, Tong & Tao, Changfa & Wang, Xishi, 2020. "Cooling control effect of water mist on thermal runaway propagation in lithium ion battery modules," Applied Energy, Elsevier, vol. 267(C).
    14. Oh, Ki-Yong & Epureanu, Bogdan I., 2016. "Characterization and modeling of the thermal mechanics of lithium-ion battery cells," Applied Energy, Elsevier, vol. 178(C), pages 633-646.
    15. Mao, Ning & Zhang, Teng & Wang, Zhirong & Gadkari, Siddharth & Wang, Junling & He, Tengfei & Gao, Tianfeng & Cai, Qiong, 2023. "Revealing the thermal stability and component heat contribution ratio of overcharged lithium-ion batteries during thermal runaway," Energy, Elsevier, vol. 263(PD).
    16. Ankur Bhattacharjee & Rakesh K. Mohanty & Aritra Ghosh, 2020. "Design of an Optimized Thermal Management System for Li-Ion Batteries under Different Discharging Conditions," Energies, MDPI, vol. 13(21), pages 1-21, October.
    17. Eddahech, Akram & Briat, Olivier & Vinassa, Jean-Michel, 2013. "Thermal characterization of a high-power lithium-ion battery: Potentiometric and calorimetric measurement of entropy changes," Energy, Elsevier, vol. 61(C), pages 432-439.
    18. Wang, Tao & Tseng, K.J. & Zhao, Jiyun & Wei, Zhongbao, 2014. "Thermal investigation of lithium-ion battery module with different cell arrangement structures and forced air-cooling strategies," Applied Energy, Elsevier, vol. 134(C), pages 229-238.
    19. Wang, Zhi & Wang, Jian, 2020. "Investigation of external heating-induced failure propagation behaviors in large-size cell modules with different phase change materials," Energy, Elsevier, vol. 204(C).
    20. Wang, Qian & Jiang, Bin & Li, Bo & Yan, Yuying, 2016. "A critical review of thermal management models and solutions of lithium-ion batteries for the development of pure electric vehicles," Renewable and Sustainable Energy Reviews, Elsevier, vol. 64(C), pages 106-128.
    21. Huang, Peifeng & Ping, Ping & Li, Ke & Chen, Haodong & Wang, Qingsong & Wen, Jennifer & Sun, Jinhua, 2016. "Experimental and modeling analysis of thermal runaway propagation over the large format energy storage battery module with Li4Ti5O12 anode," Applied Energy, Elsevier, vol. 183(C), pages 659-673.
    22. Gao, Tianfeng & Bai, Jinlong & Ouyang, Dongxu & Wang, Zhirong & Bai, Wei & Mao, Ning & Zhu, Yu, 2023. "Effect of aging temperature on thermal stability of lithium-ion batteries: Part A – High-temperature aging," Renewable Energy, Elsevier, vol. 203(C), pages 592-600.
    23. Ye, Jiana & Chen, Haodong & Wang, Qingsong & Huang, Peifeng & Sun, Jinhua & Lo, Siuming, 2016. "Thermal behavior and failure mechanism of lithium ion cells during overcharge under adiabatic conditions," Applied Energy, Elsevier, vol. 182(C), pages 464-474.

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