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Effect of aging temperature on thermal stability of lithium-ion batteries: Part A – High-temperature aging

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  • Gao, Tianfeng
  • Bai, Jinlong
  • Ouyang, Dongxu
  • Wang, Zhirong
  • Bai, Wei
  • Mao, Ning
  • Zhu, Yu

Abstract

Aging and thermal runaway are two significant reasons why lithium-ion batteries are struggling to become more widely available. Aging at different temperatures causes differences in the aging mechanism and thermal runaway behaviour of lithium-ion batteries. In this paper, four sets of commercial lithium-ion batteries are aged at 25 °C, 40 °C, 60 °C and 80 °C respectively for 100 cycles. Then the morphology and composition of the electrodes and separators are analysed in order to reveal the mechanism of changes in electrical performance and thermal stability due to aging at different temperatures. The differences in the decomposition products of the solid electrolyte intermediate (SEI) layer are an important factor in inducing changes in thermal runaway behaviour. At 60 °C, the accumulation of SEI decomposition products results in thicker SEI layers and shorter thermal runaway times. At 80 °C, the SEI decomposition products are heavily transformed into particles with a loose structure, generating a large amount of gas in the process, which further leads to the rupture of the aluminium-plastic film and the evaporation of the electrolyte, with a longer duration of thermal runaway and a lower maximum temperature.

Suggested Citation

  • Gao, Tianfeng & Bai, Jinlong & Ouyang, Dongxu & Wang, Zhirong & Bai, Wei & Mao, Ning & Zhu, Yu, 2023. "Effect of aging temperature on thermal stability of lithium-ion batteries: Part A – High-temperature aging," Renewable Energy, Elsevier, vol. 203(C), pages 592-600.
    • Handle: RePEc:eee:renene:v:203:y:2023:i:c:p:592-600
    DOI: 10.1016/j.renene.2022.12.092
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    References listed on IDEAS

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    1. Xiong, Rui & Pan, Yue & Shen, Weixiang & Li, Hailong & Sun, Fengchun, 2020. "Lithium-ion battery aging mechanisms and diagnosis method for automotive applications: Recent advances and perspectives," Renewable and Sustainable Energy Reviews, Elsevier, vol. 131(C).
    2. Jhu, Can-Yong & Wang, Yih-Wen & Wen, Chia-Yuan & Shu, Chi-Min, 2012. "Thermal runaway potential of LiCoO2 and Li(Ni1/3Co1/3Mn1/3)O2 batteries determined with adiabatic calorimetry methodology," Applied Energy, Elsevier, vol. 100(C), pages 127-131.
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    3. Fransson, Matilda & Broche, Ludovic & Reid, Hamish T. & Patel, Drasti & Rack, Alexander & Shearing, Paul R., 2024. "Investigating thermal runaway dynamics and integrated safety mechanisms of micro-batteries using high-speed X-ray imaging," Applied Energy, Elsevier, vol. 369(C).
    4. García, Antonio & Pastor, José V. & Monsalve-Serrano, Javier & Golke, Diego, 2024. "Cell-to-cell dispersion impact on zero-dimensional models for predicting thermal runaway parameters of NCA and NMC811," Applied Energy, Elsevier, vol. 369(C).
    5. Wang, Meng & Wu, Senming & Chen, Ying & Luan, Weiling, 2025. "The snowball effect in electrochemical degradation and safety evolution of lithium-ion batteries during long-term cycling," Applied Energy, Elsevier, vol. 378(PB).
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    7. Wang, Zhi & Zhao, Qingjie & Sun, Feng & Yin, Bo & An, Weiguang & Shi, Bobo, 2024. "Influence of temperature dependent short-term storage on thermal runaway characteristics in lithium-ion batteries," Renewable Energy, Elsevier, vol. 232(C).

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