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How much can novel solid sorbents reduce the cost of post-combustion CO2 capture? A techno-economic investigation on the cost limits of pressure–vacuum swing adsorption

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  • Subraveti, Sai Gokul
  • Roussanaly, Simon
  • Anantharaman, Rahul
  • Riboldi, Luca
  • Rajendran, Arvind

Abstract

This paper focuses on identifying the cost limits of two single-stage pressure–vacuum swing adsorption (PVSA) cycles for post-combustion CO2 capture if the “ideal” zero-cost adsorbent can be discovered. Through an integrated techno-economic optimisation, we simultaneously optimise the adsorbent properties (adsorption isotherms and particle morphology) and process design variables to determine the lowest possible cost of CO2 avoided (excluding the CO2 conditioning, transport and storage) for different industrial flue gas CO2 compositions and flow rates. The CO2 avoided cost for PVSA ranges from 87.1 to 10.4 € per tonne of CO2 avoided, corresponding to CO2 feed compositions of 3.5 mol% to 30 mol %, respectively. The corresponding costs for a monoethanolamine based absorption process, using heat from a natural gas plant, are 76.8 to 54.8 € per tonne of CO2 avoided, respectively showing that PVSA can be attractive for flue gas streams with high CO2 compositions. The “ideal” adsorbents needed to attain the lowest possible CO2 avoided costs have a range of CO2 affinities with close to zero N2 adsorption, demonstrating promise for adsorbent discovery and development. The need for simultaneously optimising the particle morphology and the process conditions are emphasised.

Suggested Citation

  • Subraveti, Sai Gokul & Roussanaly, Simon & Anantharaman, Rahul & Riboldi, Luca & Rajendran, Arvind, 2022. "How much can novel solid sorbents reduce the cost of post-combustion CO2 capture? A techno-economic investigation on the cost limits of pressure–vacuum swing adsorption," Applied Energy, Elsevier, vol. 306(PA).
    • Handle: RePEc:eee:appene:v:306:y:2022:i:pa:s0306261921012605
    DOI: 10.1016/j.apenergy.2021.117955
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    References listed on IDEAS

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    1. Stefania Osk Gardarsdottir & Edoardo De Lena & Matteo Romano & Simon Roussanaly & Mari Voldsund & José-Francisco Pérez-Calvo & David Berstad & Chao Fu & Rahul Anantharaman & Daniel Sutter & Matteo Gaz, 2019. "Comparison of Technologies for CO 2 Capture from Cement Production—Part 2: Cost Analysis," Energies, MDPI, vol. 12(3), pages 1-20, February.
    2. Mari Voldsund & Stefania Osk Gardarsdottir & Edoardo De Lena & José-Francisco Pérez-Calvo & Armin Jamali & David Berstad & Chao Fu & Matteo Romano & Simon Roussanaly & Rahul Anantharaman & Helmut Hopp, 2019. "Comparison of Technologies for CO 2 Capture from Cement Production—Part 1: Technical Evaluation," Energies, MDPI, vol. 12(3), pages 1-33, February.
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    Cited by:

    1. Ji, Y. & Liu, W. & Yong, J.Y. & Zhang, X.J. & Jiang, L., 2023. "Solar-assisted temperature vacuum swing adsorption for direct air capture: Effect of relative humidity," Applied Energy, Elsevier, vol. 348(C).
    2. Akinola, Toluleke E. & Bonilla Prado, Phebe L. & Wang, Meihong, 2022. "Experimental studies, molecular simulation and process modelling\simulation of adsorption-based post-combustion carbon capture for power plants: A state-of-the-art review," Applied Energy, Elsevier, vol. 317(C).
    3. A. G. Olabi & Tabbi Wilberforce & Enas Taha Sayed & Nabila Shehata & Abdul Hai Alami & Hussein M. Maghrabie & Mohammad Ali Abdelkareem, 2022. "Prospect of Post-Combustion Carbon Capture Technology and Its Impact on the Circular Economy," Energies, MDPI, vol. 15(22), pages 1-38, November.

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