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Decarbonization of cement production in a hydrogen economy

Author

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  • Nhuchhen, Daya R.
  • Sit, Song P.
  • Layzell, David B.

Abstract

The transition to net-zero emission energy systems creates synergistic opportunities across sectors. For example, fuel hydrogen production from water electrolysis generates by-product oxygen that could be used to reduce the cost of carbon capture and storage (CCS) essential in the decarbonization of clinker production in cement making. To assess this opportunity, a techno-economic assessment was carried out for the production of clinker using oxy-combustion in a natural gas-fueled plant coupled to CCS. Material and energy flows were assessed in a reference case for clinker production (oxygen from air, no CCS), and compared to oxy-combustion clinker production from either an air separation unit (ASU, 95% O2), or water electrolysis (100% O2), both coupled to CCS. Compared to the reference, air-combusted clinker plant, oxy-combustion increases thermal energy demand by 7% and electricity demand by 137% for ASU and 67% for electrolytic oxygen. The levelized cost of oxygen supply ranges from $49/tO2 for an on-site ASU to pipelined electrolytic O2 at $35/tO2 (200 km) or $13/t O2 (20 km). The cost of clinker for the reference plant without CCS increases linearly from $84/t clinker to $193/t clinker at a carbon price of $0/tCO2 to $150/tCO2, respectively. With oxy-combustion and CCS, the clinker production cost ranges from $119 to $122/t clinker, reflecting a breakeven carbon price of $39 to $53/tCO2 compared to the reference case. The lower cost for the electrolytic supply of by-product oxygen compared to ASU oxygen must be balanced against the reliability of supply, the pipeline transport distance and the charges that may be added by the hydrogen producer.

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  • Nhuchhen, Daya R. & Sit, Song P. & Layzell, David B., 2022. "Decarbonization of cement production in a hydrogen economy," Applied Energy, Elsevier, vol. 317(C).
    • Handle: RePEc:eee:appene:v:317:y:2022:i:c:s0306261922005529
    DOI: 10.1016/j.apenergy.2022.119180
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    2. Otavio Cavalett & Marcos D. B. Watanabe & Mari Voldsund & Simon Roussanaly & Francesco Cherubini, 2024. "Paving the way for sustainable decarbonization of the European cement industry," Nature Sustainability, Nature, vol. 7(5), pages 568-580, May.
    3. Nehdi, Moncef L. & Marani, Afshin & Zhang, Lei, 2024. "Is net-zero feasible: Systematic review of cement and concrete decarbonization technologies," Renewable and Sustainable Energy Reviews, Elsevier, vol. 191(C).
    4. Goran Durakovic & Hongyu Zhang & Brage Rugstad Knudsen & Asgeir Tomasgard & Pedro Crespo del Granado, 2023. "Decarbonizing the European energy system in the absence of Russian gas: Hydrogen uptake and carbon capture developments in the power, heat and industry sectors," Papers 2308.08953, arXiv.org.
    5. Martin Greco-Coppi & Carina Hofmann & Diethelm Walter & Jochen Ströhle & Bernd Epple, 2023. "Negative CO2 emissions in the lime production using an indirectly heated carbonate looping process," Mitigation and Adaptation Strategies for Global Change, Springer, vol. 28(6), pages 1-32, August.
    6. Hosseini Dehshiri, Seyyed Shahabaddin & Firoozabadi, Bahar, 2024. "Wind energy integrated green hydrogen system as sustainable solution to decarbonize Iranian Industrial Cities," Energy, Elsevier, vol. 306(C).
    7. Bi, Zhenhui & Guo, Yintong & Yang, Chunhe & Yang, Hanzhi & Wang, Lei & He, Yuting & Guo, Wuhao, 2025. "Numerical investigation of fluid dynamics in aquifers for seasonal large-scale hydrogen storage using compositional simulations," Renewable Energy, Elsevier, vol. 239(C).
    8. Lifeng Du & Yanmei Yang & Luli Zhou & Min Liu, 2024. "Greenhouse Gas Reduction Potential and Economics of Green Hydrogen via Water Electrolysis: A Systematic Review of Value-Chain-Wide Decarbonization," Sustainability, MDPI, vol. 16(11), pages 1-37, May.
    9. Zhu, Yongxian & Keoleian, Gregory A. & Cooper, Daniel R., 2025. "The role of hydrogen in decarbonizing U.S. industry: A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 214(C).

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