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Performance of alkali and Ni-modified ZSM-5 during catalytic pyrolysis of extracted hemicellulose from rice straw for the production of aromatic hydrocarbons

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  • Nishu,
  • Li, Chong
  • Chai, Meiyun
  • Rahman, Md. Maksudur
  • Li, Yingkai
  • Sarker, Manobendro
  • Liu, Ronghou

Abstract

Hemicellulose was extracted from rice straw, and catalyst ZSM-5 was modified by NaOH and Ni over alkaline treatment and wet impregnation method, respectively. To investigate the effects of modified ZSM-5 on selectivity of aromatic hydrocarbons, catalytic pyrolysis of hemicellulose was studied via Py-GC/MS. Significant effect has been reported for product selectivity and composition over the modified catalysts. All the modified catalysts showed better aromatic selectivity than parent ZSM-5 (P-ZSM-5). Notably, alkali modified ZSM-5 with 0.4 M concentration of NaOH (0.4 M ZSM-5) showed 36% selectivity towards aromatics with the share of benzene, toluene, and xylene (58%) and share of polyaromatics (15%) compared to others. Meanwhile, 8 wt% Ni-ZSM-5 showed the highest selectivity of aromatic hydrocarbons of 54% where the share of benzene, toluene, and xylene was 70%. This research revealed that metal modified ZSM-5 significantly influences the aromatics yield, which is essential for the production of liquid fuels and chemicals.

Suggested Citation

  • Nishu, & Li, Chong & Chai, Meiyun & Rahman, Md. Maksudur & Li, Yingkai & Sarker, Manobendro & Liu, Ronghou, 2021. "Performance of alkali and Ni-modified ZSM-5 during catalytic pyrolysis of extracted hemicellulose from rice straw for the production of aromatic hydrocarbons," Renewable Energy, Elsevier, vol. 175(C), pages 936-951.
    • Handle: RePEc:eee:renene:v:175:y:2021:i:c:p:936-951
    DOI: 10.1016/j.renene.2021.05.005
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    1. Nishu, & Li, Chong & Yellezuome, Dominic & Li, Yingkai & Liu, Ronghou, 2023. "Catalytic pyrolysis of rice straw for high yield of aromatics over modified ZSM-5 catalysts and its kinetics," Renewable Energy, Elsevier, vol. 209(C), pages 569-580.
    2. Wei, Xiaocui & Liu, Yanan & Cao, Yang & Li, Jin & Meng, Xianghao & Zhang, Zhao & Jiang, Zhongyi, 2022. "Hierarchical gallium-modified ZSM-5@SBA-15 for the catalytic pyrolysis of biomass into hydrocarbons," Renewable Energy, Elsevier, vol. 200(C), pages 1037-1046.
    3. Kostyniuk, Andrii & Bajec, David & Likozar, Blaž, 2022. "Catalytic hydrocracking reactions of tetralin biomass tar model compound to benzene, toluene and xylenes (BTX) over metal-modified ZSM-5 in ambient pressure reactor," Renewable Energy, Elsevier, vol. 188(C), pages 240-255.
    4. Douvartzides, Savvas & Charisiou, Nikolaos D. & Wang, Wen & Papadakis, Vagelis G. & Polychronopoulou, Kyriaki & Goula, Maria A., 2022. "Catalytic fast pyrolysis of agricultural residues and dedicated energy crops for the production of high energy density transportation biofuels. Part II: Catalytic research," Renewable Energy, Elsevier, vol. 189(C), pages 315-338.

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