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Cr2O3/C composite coatings on stainless steel 304 as bipolar plate for proton exchange membrane fuel cell

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  • Huang, Kaikai
  • Zhang, Dongming
  • Hu, Mingming
  • Hu, Qinghui

Abstract

Stainless steel 304 (SS304) is a potential material as the bipolar plate for PEMFC (proton exchange membrane fuel cell). However, its interfacial contact resistance is too high and the corrosion resistance is too low to survive in the hostile environment. A novel approach of preparing the composite coating layers by in-situ method is reported in this manuscript. The plate is first treated in acid solution, and then heat treated at low temperature, finally it is treated by electrochemical method. The ICR (interfacial contact resistance) for the treated plate is 9.8 mΩ cm2 at the compaction force of 240 N cm−2, and the corrosion current density is 3 × 10−7 A cm−2. Microstructures for differential treatments have been analyzed by FESEM (field emission scanning electron microscope), XPS (X-ray photoelectron spectroscopy) and AES (Auger electron spectroscopy). The results indicate that a protectively layer with Cr2O3/carbon is formed on the SS304 surface, which improves the performance of bipolar plate effectively.

Suggested Citation

  • Huang, Kaikai & Zhang, Dongming & Hu, Mingming & Hu, Qinghui, 2014. "Cr2O3/C composite coatings on stainless steel 304 as bipolar plate for proton exchange membrane fuel cell," Energy, Elsevier, vol. 76(C), pages 816-821.
    • Handle: RePEc:eee:energy:v:76:y:2014:i:c:p:816-821
    DOI: 10.1016/j.energy.2014.08.076
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    1. Kariya, Tetsuro & Yanagimoto, Katsu & Funakubo, Hiroshi & Shudo, Toshio, 2015. "Effects of porous flow field type separators using sintered Ni-based alloy powders on interfacial contact resistances and fuel cell performances," Energy, Elsevier, vol. 87(C), pages 134-141.
    2. Bhosale, Amit C. & Rengaswamy, Raghunathan, 2019. "Interfacial contact resistance in polymer electrolyte membrane fuel cells: Recent developments and challenges," Renewable and Sustainable Energy Reviews, Elsevier, vol. 115(C).
    3. Hu, Qinghui & Zhang, Dongming & Fu, Hao, 2015. "Effect of flow-field dimensions on the formability of Fe–Ni–Cr alloy as bipolar plate for PEM (proton exchange membrane) fuel cell," Energy, Elsevier, vol. 83(C), pages 156-163.
    4. Kim, Ah-Reum & Shin, Seungho & Um, Sukkee, 2016. "Multidisciplinary approaches to metallic bipolar plate design with bypass flow fields through deformable gas diffusion media of polymer electrolyte fuel cells," Energy, Elsevier, vol. 106(C), pages 378-389.
    5. Ren, Peng & Pei, Pucheng & Chen, Dongfang & Zhang, Lu & Li, Yuehua & Song, Xin & Wang, Mingkai & Wang, He, 2022. "Corrosion of metallic bipolar plates accelerated by operating conditions in a simulated PEM fuel cell cathode environment," Renewable Energy, Elsevier, vol. 194(C), pages 1277-1287.
    6. Li, Yuee & Zhang, Dongming, 2017. "Preparation of DB film in the channel of SS304 bipolar plate to improve its water liquidity," Energy, Elsevier, vol. 128(C), pages 19-27.
    7. Zhang, Weixin & Yi, Peiyun & Peng, Linfa & Lai, Xinmin, 2018. "Strategy of alternating bias voltage on corrosion resistance and interfacial conductivity enhancement of TiCx/a-C coatings on metallic bipolar plates in PEMFCs," Energy, Elsevier, vol. 162(C), pages 933-943.
    8. Chen, Chen-Yu & Su, Sheng-Chun, 2018. "Effects of assembly torque on a proton exchange membrane fuel cell with stamped metallic bipolar plates," Energy, Elsevier, vol. 159(C), pages 440-447.
    9. Fan, Hong-Qiang & Wu, Yuan-Min & Su, Shuo & Shi, Dong-Dong & Wang, Xian-Zong & Behnamian, Yashar & Zhang, Jie-Yu & Li, Qian, 2022. "Solution acidity and temperature induced anodic dissolution and degradation of through-plane electrical conductivity of Au/TiN coated metal bipolar plates used in PEMFC," Energy, Elsevier, vol. 254(PC).

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