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Pd-based composite membrane and its high-pressure module for pre-combustion CO2 capture

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  • Ryi, Shin-Kun
  • Lee, Chun-Boo
  • Lee, Sung-Wook
  • Park, Jong-Soo

Abstract

This study investigates configuration of a module for withstanding high pressure and temperature for CO2 capture from a coal gasifier. In order to increase the durability of the module at high pressure and temperature, a flange-type unit-cell module was installed in a high-pressure chamber. Hydrogen permeation and N2 leakage tests showed that H2/N2 selectivity remained at ∼4000 after ∼300 h at a pressure difference of 2000 kPa (∼20 bar) and 673 K. A CO2 capturing test was carried out at 673 K and a pressure difference of 2000 kPa with a 40% CO2 + 60% H2 feed gas mixture, which is similar to the composition in a coal gasifier after shift reaction and H2O removal. It was shown that CO2 could be enriched up to 78–95% with a hydrogen recovery ratio of 82–97% when the feed flow rate was 0.05–0.17 Nm3 h−1 with a membrane surface area of 16. 6 cm2.

Suggested Citation

  • Ryi, Shin-Kun & Lee, Chun-Boo & Lee, Sung-Wook & Park, Jong-Soo, 2013. "Pd-based composite membrane and its high-pressure module for pre-combustion CO2 capture," Energy, Elsevier, vol. 51(C), pages 237-242.
    • Handle: RePEc:eee:energy:v:51:y:2013:i:c:p:237-242
    DOI: 10.1016/j.energy.2012.12.039
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    References listed on IDEAS

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    1. Bounaceur, Roda & Lape, Nancy & Roizard, Denis & Vallieres, Cécile & Favre, Eric, 2006. "Membrane processes for post-combustion carbon dioxide capture: A parametric study," Energy, Elsevier, vol. 31(14), pages 2556-2570.
    2. Ryi, Shin-Kun & Lee, Chun-Boo & Lee, Sung-Wook & Hwang, Kyung-Ran & Park, Jong-Soo, 2012. "Hydrogen recovery from ethylene mixture with PD-AU composite membrane," Energy, Elsevier, vol. 47(1), pages 3-10.
    3. Davison, John, 2007. "Performance and costs of power plants with capture and storage of CO2," Energy, Elsevier, vol. 32(7), pages 1163-1176.
    Full references (including those not matched with items on IDEAS)

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    Cited by:

    1. Lee, Sung-Wook & Park, Jong-Soo & Lee, Chun-Boo & Lee, Dong-Wook & Kim, Hakjoo & Ra, Ho Won & Kim, Sung-Hyun & Ryi, Shin-Kun, 2014. "H2 recovery and CO2 capture after water–gas shift reactor using synthesis gas from coal gasification," Energy, Elsevier, vol. 66(C), pages 635-642.
    2. Theo, Wai Lip & Lim, Jeng Shiun & Hashim, Haslenda & Mustaffa, Azizul Azri & Ho, Wai Shin, 2016. "Review of pre-combustion capture and ionic liquid in carbon capture and storage," Applied Energy, Elsevier, vol. 183(C), pages 1633-1663.
    3. Song, Chunfeng & Kitamura, Yutaka & Li, Shuhong, 2014. "Energy analysis of the cryogenic CO2 capture process based on Stirling coolers," Energy, Elsevier, vol. 65(C), pages 580-589.

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