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Effect of gas-diffusion electrode material heterogeneity on the structural integrity of polymer electrolyte fuel cell

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  • Poornesh, K.K.
  • Cho, Chongdu
  • Kim, Do-Young
  • Tak, Yongsug

Abstract

In polymer electrolyte fuel cell (PEFC), gas-diffusion electrode (GDE) plays very significant role in force transmission from bipolar plate to the membrane. This paper investigates the effects of material heterogeneities of gas-diffusion electrode layer (gas-diffusion layer (GDL) and catalyst layer (CL)) on the assembly stress levels of single PEFC stack. In addition, we adopt a force transfer mechanism in a single fuel cell stack based on material heterogeneities of GDL and CL to understand the limitations and advantages associated with it through numerical analyses. Nanoscale heterogeneities in GDE are effectively implemented in the simulation cases along with the membrane swelling. Influence of presence or absence of CL interlayer in the numerical environment is found to have significant impact on the adjacent layers as well as interfaces.

Suggested Citation

  • Poornesh, K.K. & Cho, Chongdu & Kim, Do-Young & Tak, Yongsug, 2010. "Effect of gas-diffusion electrode material heterogeneity on the structural integrity of polymer electrolyte fuel cell," Energy, Elsevier, vol. 35(12), pages 5241-5249.
    • Handle: RePEc:eee:energy:v:35:y:2010:i:12:p:5241-5249
    DOI: 10.1016/j.energy.2010.07.041
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    References listed on IDEAS

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    1. Taymaz, Imdat & Benli, Merthan, 2010. "Numerical study of assembly pressure effect on the performance of proton exchange membrane fuel cell," Energy, Elsevier, vol. 35(5), pages 2134-2140.
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    Cited by:

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    2. Boyaci San, Fatma Gül & Isik-Gulsac, Isil & Okur, Osman, 2013. "Analysis of the polymer composite bipolar plate properties on the performance of PEMFC (polymer electrolyte membrane fuel cells) by RSM (response surface methodology)," Energy, Elsevier, vol. 55(C), pages 1067-1075.
    3. Ren, Zhijun & Zhang, Dongming & Wang, Zaiyi, 2012. "Stacks with TiN/titanium as the bipolar plate for PEMFCs," Energy, Elsevier, vol. 48(1), pages 577-581.
    4. Ye, Luhan & Lv, Weiqiang & Zhang, Kelvin H.L. & Wang, Xiaoning & Yan, Pengfei & Dickerson, James H. & He, Weidong, 2015. "A new insight into the oxygen diffusion in porous cathodes of lithium-air batteries," Energy, Elsevier, vol. 83(C), pages 669-673.
    5. Liu, Jiaran & Tan, Jinzhu & Yang, Weizhan & Li, Yang & Wang, Chao, 2021. "Better electrochemical performance of PEMFC under a novel pneumatic clamping mechanism," Energy, Elsevier, vol. 229(C).
    6. Kim, Ah-Reum & Shin, Seungho & Um, Sukkee, 2016. "Multidisciplinary approaches to metallic bipolar plate design with bypass flow fields through deformable gas diffusion media of polymer electrolyte fuel cells," Energy, Elsevier, vol. 106(C), pages 378-389.
    7. Kim, Jaeyeon & Kim, Hyeok & Song, Hyeonjun & Kim, Dasol & Kim, Geon Hwi & Im, Dasom & Jeong, Youngjin & Park, Taehyun, 2021. "Carbon nanotube sheet as a microporous layer for proton exchange membrane fuel cells," Energy, Elsevier, vol. 227(C).

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