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Transport phenomena of convergent and divergent serpentine flow fields for PEMFC

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  • Chowdhury, Mohammad Ziauddin
  • Timurkutluk, Bora

Abstract

Reactive species and water transport are crucial for the proton exchange membrane fuel cell operation and performance, and for this, effective flow field design can facilitate the desired transport characteristics of species. From this motivation, the conventional single serpentine flow field pattern is modified by convergent and divergent design concepts and the complex transport phenomena of the newly developed flow field designs are investigated by a numerical approach. For the numerical analyses, an experimentally validated mathematical model is developed to predict the current density, oxygen mass transport, water concentration and pressure distribution. The different configurations of modified convergent and divergent serpentine flow fields are then numerically solved and the results are compared with the conventional serpentine flow field pattern. The transport of reactive species and water concentration are analyzed from the different perspectives including cathode domains and surfaces with a quantitative formulation of the transport species. The numerical results reveals that the modified convergent serpentine flow fields yield to a uniform current density due to the lower mass fraction of water concentration over the reaction zone facilitating better oxygen mass transport and also higher channel pressure distribution along the flow field comparing the conventional and divergent type serpentine flow fields.

Suggested Citation

  • Chowdhury, Mohammad Ziauddin & Timurkutluk, Bora, 2018. "Transport phenomena of convergent and divergent serpentine flow fields for PEMFC," Energy, Elsevier, vol. 161(C), pages 104-117.
  • Handle: RePEc:eee:energy:v:161:y:2018:i:c:p:104-117
    DOI: 10.1016/j.energy.2018.07.143
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    1. Wu, Horng-Wen, 2016. "A review of recent development: Transport and performance modeling of PEM fuel cells," Applied Energy, Elsevier, vol. 165(C), pages 81-106.
    2. Thomas, Sobi & Bates, Alex & Park, Sam & Sahu, A.K. & Lee, Sang C. & Son, Byung Rak & Kim, Joo Gon & Lee, Dong-Ha, 2016. "An experimental and simulation study of novel channel designs for open-cathode high-temperature polymer electrolyte membrane fuel cells," Applied Energy, Elsevier, vol. 165(C), pages 765-776.
    3. Hong, Po & Xu, Liangfei & Li, Jianqiu & Ouyang, Minggao, 2017. "Modeling of membrane electrode assembly of PEM fuel cell to analyze voltage losses inside," Energy, Elsevier, vol. 139(C), pages 277-288.
    4. Xing, Lei & Liu, Xiaoteng & Alaje, Taiwo & Kumar, Ravi & Mamlouk, Mohamed & Scott, Keith, 2014. "A two-phase flow and non-isothermal agglomerate model for a proton exchange membrane (PEM) fuel cell," Energy, Elsevier, vol. 73(C), pages 618-634.
    5. Lin, R. & Ren, Y.S. & Lin, X.W. & Jiang, Z.H. & Yang, Z. & Chang, Y.T., 2017. "Investigation of the internal behavior in segmented PEMFCs of different flow fields during cold start process," Energy, Elsevier, vol. 123(C), pages 367-377.
    6. Carton, J.G. & Lawlor, V. & Olabi, A.G. & Hochenauer, C. & Zauner, G., 2012. "Water droplet accumulation and motion in PEM (Proton Exchange Membrane) fuel cell mini-channels," Energy, Elsevier, vol. 39(1), pages 63-73.
    7. Ramiar, A. & Mahmoudi, A.H. & Esmaili, Q. & Abdollahzadeh, M., 2016. "Influence of cathode flow pulsation on performance of proton exchange membrane fuel cell with interdigitated gas distributors," Energy, Elsevier, vol. 94(C), pages 206-217.
    8. Arun Saco, S. & Thundil Karuppa Raj, R. & Karthikeyan, P., 2016. "A study on scaled up proton exchange membrane fuel cell with various flow channels for optimizing power output by effective water management using numerical technique," Energy, Elsevier, vol. 113(C), pages 558-573.
    9. Chen, Ben & Wang, Jun & Yang, Tianqi & Cai, Yonghua & Zhang, Caizhi & Chan, Siew Hwa & Yu, Yi & Tu, Zhengkai, 2016. "Carbon corrosion and performance degradation mechanism in a proton exchange membrane fuel cell with dead-ended anode and cathode," Energy, Elsevier, vol. 106(C), pages 54-62.
    10. Karvelas, E.G. & Koubogiannis, D.G. & Hatziapostolou, A. & Sarris, I.E., 2016. "The effect of anode bed geometry on the hydraulic behaviour of PEM fuel cells," Renewable Energy, Elsevier, vol. 93(C), pages 269-279.
    11. Iranzo, Alfredo & Boillat, Pierre & Biesdorf, Johannes & Salva, Antonio, 2015. "Investigation of the liquid water distributions in a 50 cm2 PEM fuel cell: Effects of reactants relative humidity, current density, and cathode stoichiometry," Energy, Elsevier, vol. 82(C), pages 914-921.
    12. Wang, Junye, 2015. "Theory and practice of flow field designs for fuel cell scaling-up: A critical review," Applied Energy, Elsevier, vol. 157(C), pages 640-663.
    13. Xing, Lei & Cai, Qiong & Xu, Chenxi & Liu, Chunbo & Scott, Keith & Yan, Yongsheng, 2016. "Numerical study of the effect of relative humidity and stoichiometric flow ratio on PEM (proton exchange membrane) fuel cell performance with various channel lengths: An anode partial flooding modelli," Energy, Elsevier, vol. 106(C), pages 631-645.
    14. khazaee, I. & Sabadbafan, H., 2016. "Effect of humidity content and direction of the flow of reactant gases on water management in the 4-serpentine and 1-serpentine flow channel in a PEM (proton exchange membrane) fuel cell," Energy, Elsevier, vol. 101(C), pages 252-265.
    15. Damian-Ascencio, Cesar E. & Saldaña-Robles, Adriana & Hernandez-Guerrero, Abel & Cano-Andrade, Sergio, 2017. "Numerical modeling of a proton exchange membrane fuel cell with tree-like flow field channels based on an entropy generation analysis," Energy, Elsevier, vol. 133(C), pages 306-316.
    16. Afshari, E. & Mosharaf-Dehkordi, M. & Rajabian, H., 2017. "An investigation of the PEM fuel cells performance with partially restricted cathode flow channels and metal foam as a flow distributor," Energy, Elsevier, vol. 118(C), pages 705-715.
    17. Xing, Lei & Du, Shangfeng & Chen, Rui & Mamlouk, Mohamed & Scott, Keith, 2016. "Anode partial flooding modelling of proton exchange membrane fuel cells: Model development and validation," Energy, Elsevier, vol. 96(C), pages 80-95.
    18. Siegel, C., 2008. "Review of computational heat and mass transfer modeling in polymer-electrolyte-membrane (PEM) fuel cells," Energy, Elsevier, vol. 33(9), pages 1331-1352.
    19. Rostami, Leila & Mohamad Gholy Nejad, Puriya & Vatani, Ali, 2016. "A numerical investigation of serpentine flow channel with different bend sizes in polymer electrolyte membrane fuel cells," Energy, Elsevier, vol. 97(C), pages 400-410.
    20. Abdollahzadeh, M. & Pascoa, J.C. & Ranjbar, A.A. & Esmaili, Q., 2014. "Analysis of PEM (Polymer Electrolyte Membrane) fuel cell cathode two-dimensional modeling," Energy, Elsevier, vol. 68(C), pages 478-494.
    21. Salva, J. Antonio & Iranzo, Alfredo & Rosa, Felipe & Tapia, Elvira, 2016. "Validation of cell voltage and water content in a PEM (polymer electrolyte membrane) fuel cell model using neutron imaging for different operating conditions," Energy, Elsevier, vol. 101(C), pages 100-112.
    22. Unknown, 2004. "End Materials," Choices: The Magazine of Food, Farm, and Resource Issues, Agricultural and Applied Economics Association, vol. 19(4), pages 1-1.
    23. Andersson, M. & Beale, S.B. & Espinoza, M. & Wu, Z. & Lehnert, W., 2016. "A review of cell-scale multiphase flow modeling, including water management, in polymer electrolyte fuel cells," Applied Energy, Elsevier, vol. 180(C), pages 757-778.
    24. Carton, J.G. & Olabi, A.G., 2017. "Three-dimensional proton exchange membrane fuel cell model: Comparison of double channel and open pore cellular foam flow plates," Energy, Elsevier, vol. 136(C), pages 185-195.
    25. Mortazavi, Mehdi & Tajiri, Kazuya, 2015. "Two-phase flow pressure drop in flow channels of proton exchange membrane fuel cells: Review of experimental approaches," Renewable and Sustainable Energy Reviews, Elsevier, vol. 45(C), pages 296-317.
    26. Li, Wenkai & Zhang, Qinglei & Wang, Chao & Yan, Xiaohui & Shen, Shuiyun & Xia, Guofeng & Zhu, Fengjuan & Zhang, Junliang, 2017. "Experimental and numerical analysis of a three-dimensional flow field for PEMFCs," Applied Energy, Elsevier, vol. 195(C), pages 278-288.
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    Cited by:

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    3. Perng, Shiang-Wuu & Wu, Horng-Wen, 2022. "Influence of inlet-nozzle and outlet-diffuser mounted in the plate-shape reactor on PEMFC net power output and methanol steam reforming performance," Applied Energy, Elsevier, vol. 323(C).
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    5. Suprava Chakraborty & Devaraj Elangovan & Karthikeyan Palaniswamy & Ashley Fly & Dineshkumar Ravi & Denis Ashok Sathia Seelan & Thundil Karuppa Raj Rajagopal, 2022. "A Review on the Numerical Studies on the Performance of Proton Exchange Membrane Fuel Cell (PEMFC) Flow Channel Designs for Automotive Applications," Energies, MDPI, vol. 15(24), pages 1-21, December.
    6. Hwang, Jenn-Jiang & Dlamini, Mangaliso Menzi & Weng, Fang-Bor & Chang, Tseng & Lin, Chih-Hong & Weng, Shih-Cheng, 2022. "Simulation of fine mesh implementation on the cathode for proton exchange membrane fuel cell (PEMFC)," Energy, Elsevier, vol. 244(PA).
    7. Yin, Yan & Wu, Shiyu & Qin, Yanzhou & Otoo, Obed Nenyi & Zhang, Junfeng, 2020. "Quantitative analysis of trapezoid baffle block sloping angles on oxygen transport and performance of proton exchange membrane fuel cell," Applied Energy, Elsevier, vol. 271(C).
    8. Xiong, Kangning & Wu, Wei & Wang, Shuangfeng & Zhang, Lin, 2021. "Modeling, design, materials and fabrication of bipolar plates for proton exchange membrane fuel cell: A review," Applied Energy, Elsevier, vol. 301(C).

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