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Investigation of the internal behavior in segmented PEMFCs of different flow fields during cold start process

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  • Lin, R.
  • Ren, Y.S.
  • Lin, X.W.
  • Jiang, Z.H.
  • Yang, Z.
  • Chang, Y.T.

Abstract

In this study, we have researched the internal behavior in segmented proton exchange membrane fuel cells (PEMFCs) with three different flow fields during cold start process. The change of internal current density and temperature in fuel cells with different flow fields could be obviously shown by the printed circuit board (PCB) technology, and the study shows that the flow field is significant for enhancing the cold start ability and durability. Single serpentine flow field has the best cold start performance, while triple channel serpentine flow field has the best uniformity. It is found that without a robust temperature rising tendency, the cell temperature reaching 0 °C does not definitely mean a successful cold start because the cell temperature might drop down 0 °C again. Polarization curves show that there is almost no performance degradation after successful cold start, but the cell degrades quickly after the failed cold start at −7 °C and −10 °C. Based on these characteristics, we optimized the rapid cold start strategy by using electric heating and make it possible to start up the PEMFC at temperatures down to −20 °C within about 11 min.

Suggested Citation

  • Lin, R. & Ren, Y.S. & Lin, X.W. & Jiang, Z.H. & Yang, Z. & Chang, Y.T., 2017. "Investigation of the internal behavior in segmented PEMFCs of different flow fields during cold start process," Energy, Elsevier, vol. 123(C), pages 367-377.
    • Handle: RePEc:eee:energy:v:123:y:2017:i:c:p:367-377
    DOI: 10.1016/j.energy.2017.01.138
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    References listed on IDEAS

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    1. Wang, Junye, 2015. "Theory and practice of flow field designs for fuel cell scaling-up: A critical review," Applied Energy, Elsevier, vol. 157(C), pages 640-663.
    2. Xing, Lei & Cai, Qiong & Xu, Chenxi & Liu, Chunbo & Scott, Keith & Yan, Yongsheng, 2016. "Numerical study of the effect of relative humidity and stoichiometric flow ratio on PEM (proton exchange membrane) fuel cell performance with various channel lengths: An anode partial flooding modelli," Energy, Elsevier, vol. 106(C), pages 631-645.
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    Cited by:

    1. Zhong, Di & Lin, Rui & Jiang, Zhenghua & Zhu, Yike & Liu, Dengchen & Cai, Xin & Chen, Liang, 2020. "Low temperature durability and consistency analysis of proton exchange membrane fuel cell stack based on comprehensive characterizations," Applied Energy, Elsevier, vol. 264(C).
    2. Najmi, Aezid-Ul-Hassan & Anyanwu, Ikechukwu S. & Xie, Xu & Liu, Zhi & Jiao, Kui, 2021. "Experimental investigation and optimization of proton exchange membrane fuel cell using different flow fields," Energy, Elsevier, vol. 217(C).
    3. Li, Linjun & Wang, Shixue & Yue, Like & Wang, Guozhuo, 2019. "Cold-start method for proton-exchange membrane fuel cells based on locally heating the cathode," Applied Energy, Elsevier, vol. 254(C).
    4. Yang, Zirong & Jiao, Kui & Wu, Kangcheng & Shi, Weilong & Jiang, Shangfeng & Zhang, Longhai & Du, Qing, 2021. "Numerical investigations of assisted heating cold start strategies for proton exchange membrane fuel cell systems," Energy, Elsevier, vol. 222(C).
    5. Alizadeh, E. & Ghadimi, M. & Barzegari, M.M. & Momenifar, M. & Saadat, S.H.M., 2017. "Development of contact pressure distribution of PEM fuel cell's MEA using novel clamping mechanism," Energy, Elsevier, vol. 131(C), pages 92-97.
    6. Zhan, Zhigang & Yuan, Chong & Hu, Zhangrong & Wang, Hui & Sui, P.C. & Djilali, Ned & Pan, Mu, 2018. "Experimental study on different preheating methods for the cold-start of PEMFC stacks," Energy, Elsevier, vol. 162(C), pages 1029-1040.
    7. Liu, Ze & Xu, Sichuan & Zhao, Honghui & Wang, Yupeng, 2022. "Durability estimation and short-term voltage degradation forecasting of vehicle PEMFC system: Development and evaluation of machine learning models," Applied Energy, Elsevier, vol. 326(C).
    8. Chowdhury, Mohammad Ziauddin & Timurkutluk, Bora, 2018. "Transport phenomena of convergent and divergent serpentine flow fields for PEMFC," Energy, Elsevier, vol. 161(C), pages 104-117.
    9. Pourrahmani, Hossein & Van herle, Jan, 2022. "Water management of the proton exchange membrane fuel cells: Optimizing the effect of microstructural properties on the gas diffusion layer liquid removal," Energy, Elsevier, vol. 256(C).
    10. Maximilian Schmitz & Matthias Bahr & Sönke Gößling & Stefan Pischinger, 2023. "Analysis of Ice Formation during Start-Up of PEM Fuel Cells at Subzero Temperatures Using Experimental and Simulative Methods," Energies, MDPI, vol. 16(18), pages 1-26, September.
    11. Fathabadi, Hassan, 2018. "Novel fuel cell/battery/supercapacitor hybrid power source for fuel cell hybrid electric vehicles," Energy, Elsevier, vol. 143(C), pages 467-477.
    12. Zang, Linfeng & Hao, Liang & Zhu, Xiaojing, 2023. "Effect of the pore structure of cathode catalyst layer on the PEM fuel cell cold start process," Energy, Elsevier, vol. 271(C).
    13. Huo, Sen & Jiao, Kui & Park, Jae Wan, 2019. "On the water transport behavior and phase transition mechanisms in cold start operation of PEM fuel cell," Applied Energy, Elsevier, vol. 233, pages 776-788.
    14. Zhang, Weixin & Yi, Peiyun & Peng, Linfa & Lai, Xinmin, 2018. "Strategy of alternating bias voltage on corrosion resistance and interfacial conductivity enhancement of TiCx/a-C coatings on metallic bipolar plates in PEMFCs," Energy, Elsevier, vol. 162(C), pages 933-943.
    15. Lin, Rui & Zhu, Yike & Ni, Meng & Jiang, Zhenghua & Lou, Diming & Han, Lihang & Zhong, Di, 2019. "Consistency analysis of polymer electrolyte membrane fuel cell stack during cold start," Applied Energy, Elsevier, vol. 241(C), pages 420-432.
    16. Yuan, Xian Ming & Guo, Hang & Liu, Jia Xing & Ye, Fang & Ma, Chong Fang, 2018. "Influence of operation parameters on mode switching from electrolysis cell mode to fuel cell mode in a unitized regenerative fuel cell," Energy, Elsevier, vol. 162(C), pages 1041-1051.
    17. Liu, Dengcheng & Lin, Rui & Feng, Bowen & Han, Lihang & Zhang, Yu & Ni, Meng & Wu, Sai, 2019. "Localised electrochemical impedance spectroscopy investigation of polymer electrolyte membrane fuel cells using Print circuit board based interference-free system," Applied Energy, Elsevier, vol. 254(C).
    18. Liu, Jiaran & Tan, Jinzhu & Yang, Weizhan & Li, Yang & Wang, Chao, 2021. "Better electrochemical performance of PEMFC under a novel pneumatic clamping mechanism," Energy, Elsevier, vol. 229(C).

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