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In situ investigation of proton exchange membrane fuel cell performance with novel segmented cell design and a two-phase flow model

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  • Yin, Cong
  • Gao, Jianlong
  • Wen, Xuhui
  • Xie, Guangyou
  • Yang, Chunhua
  • Fang, Honglin
  • Tang, Hao

Abstract

A novel segmented fuel cell device based on the multi-layered printed circuit board (PCB) flow field plates is designed to study the localized fuel cell performance with various operation conditions. With embedded sensors, distributions of current density, relative humidity (RH) and temperature for both anode and cathode are measured simultaneously along the direction of straight parallel flow channels. Meanwhile, a stationary two-phase flow fuel cell model is developed to study the internal reaction parameter distributions and the results are compared with the in situ experimental measurements. In the co-flow operation mode of hydrogen and air, current density and reactants' RH distributions are sensitive to the stoichiometry of air but the effect from hydrogen is minor. Water transfer behavior, local reactants' RH status, temperature gradients and their impacts on current distributions are analyzed based on the in situ measurements and the coupled model analysis. The segmented cell device discussed in this paper, as well as the experimental and modeling results can be employed to optimize stack design and operating parameters with “visible” internal distributions of water, RH and temperature inside membrane electrode assembly (MEA). Further investigation on fuel cell performance and lifetime with different reactant flow directions is also suggested.

Suggested Citation

  • Yin, Cong & Gao, Jianlong & Wen, Xuhui & Xie, Guangyou & Yang, Chunhua & Fang, Honglin & Tang, Hao, 2016. "In situ investigation of proton exchange membrane fuel cell performance with novel segmented cell design and a two-phase flow model," Energy, Elsevier, vol. 113(C), pages 1071-1089.
    • Handle: RePEc:eee:energy:v:113:y:2016:i:c:p:1071-1089
    DOI: 10.1016/j.energy.2016.06.097
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    References listed on IDEAS

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    1. Xing, Lei & Liu, Xiaoteng & Alaje, Taiwo & Kumar, Ravi & Mamlouk, Mohamed & Scott, Keith, 2014. "A two-phase flow and non-isothermal agglomerate model for a proton exchange membrane (PEM) fuel cell," Energy, Elsevier, vol. 73(C), pages 618-634.
    2. Carton, J.G. & Lawlor, V. & Olabi, A.G. & Hochenauer, C. & Zauner, G., 2012. "Water droplet accumulation and motion in PEM (Proton Exchange Membrane) fuel cell mini-channels," Energy, Elsevier, vol. 39(1), pages 63-73.
    3. Wang, Yun & Chen, Ken S. & Mishler, Jeffrey & Cho, Sung Chan & Adroher, Xavier Cordobes, 2011. "A review of polymer electrolyte membrane fuel cells: Technology, applications, and needs on fundamental research," Applied Energy, Elsevier, vol. 88(4), pages 981-1007, April.
    4. Xing, Lei & Mamlouk, Mohamed & Scott, Keith, 2013. "A two dimensional agglomerate model for a proton exchange membrane fuel cell," Energy, Elsevier, vol. 61(C), pages 196-210.
    5. Pérez, Luis C. & Brandão, Lúcia & Sousa, José M. & Mendes, Adélio, 2011. "Segmented polymer electrolyte membrane fuel cells--A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 15(1), pages 169-185, January.
    6. Rakhshanpouri, S. & Rowshanzamir, S., 2013. "Water transport through a PEM (proton exchange membrane) fuel cell in a seven-layer model," Energy, Elsevier, vol. 50(C), pages 220-231.
    7. Perng, Shiang-Wuu & Wu, Horng-Wen & Shih, Gin-Jang, 2015. "Effect of prominent gas diffusion layer (GDL) on non-isothermal transport characteristics and cell performance of a proton exchange membrane fuel cell (PEMFC)," Energy, Elsevier, vol. 88(C), pages 126-138.
    8. Kang, Sanggyu, 2015. "Quasi-three dimensional dynamic modeling of a proton exchange membrane fuel cell with consideration of two-phase water transport through a gas diffusion layer," Energy, Elsevier, vol. 90(P2), pages 1388-1400.
    9. Djilali, N., 2007. "Computational modelling of polymer electrolyte membrane (PEM) fuel cells: Challenges and opportunities," Energy, Elsevier, vol. 32(4), pages 269-280.
    10. Carton, J.G. & Olabi, A.G., 2010. "Design of experiment study of the parameters that affect performance of three flow plate configurations of a proton exchange membrane fuel cell," Energy, Elsevier, vol. 35(7), pages 2796-2806.
    11. Cano-Andrade, S. & Hernandez-Guerrero, A. & von Spakovsky, M.R. & Damian-Ascencio, C.E. & Rubio-Arana, J.C., 2010. "Current density and polarization curves for radial flow field patterns applied to PEMFCs (Proton Exchange Membrane Fuel Cells)," Energy, Elsevier, vol. 35(2), pages 920-927.
    12. Xing, Lei & Du, Shangfeng & Chen, Rui & Mamlouk, Mohamed & Scott, Keith, 2016. "Anode partial flooding modelling of proton exchange membrane fuel cells: Model development and validation," Energy, Elsevier, vol. 96(C), pages 80-95.
    13. Siegel, C., 2008. "Review of computational heat and mass transfer modeling in polymer-electrolyte-membrane (PEM) fuel cells," Energy, Elsevier, vol. 33(9), pages 1331-1352.
    14. Rostami, Leila & Mohamad Gholy Nejad, Puriya & Vatani, Ali, 2016. "A numerical investigation of serpentine flow channel with different bend sizes in polymer electrolyte membrane fuel cells," Energy, Elsevier, vol. 97(C), pages 400-410.
    15. Abdollahzadeh, M. & Pascoa, J.C. & Ranjbar, A.A. & Esmaili, Q., 2014. "Analysis of PEM (Polymer Electrolyte Membrane) fuel cell cathode two-dimensional modeling," Energy, Elsevier, vol. 68(C), pages 478-494.
    16. Iranzo, Alfredo & Boillat, Pierre & Oberholzer, Pierre & Guerra, José, 2014. "A novel approach coupling neutron imaging and numerical modelling for the analysis of the impact of water on fuel cell performance," Energy, Elsevier, vol. 68(C), pages 971-981.
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    Cited by:

    1. Yin, Cong & Gao, Yan & Li, Ting & Xie, Guangyou & Li, Kai & Tang, Hao, 2020. "Study of internal multi-parameter distributions of proton exchange membrane fuel cell with segmented cell device and coupled three-dimensional model," Renewable Energy, Elsevier, vol. 147(P1), pages 650-662.
    2. Yin, Cong & Cao, Jishen & Tang, Qilin & Su, Yanghuai & Wang, Renkang & Li, Kai & Tang, Hao, 2022. "Study of internal performance of commercial-size fuel cell stack with 3D multi-physical model and high resolution current mapping," Applied Energy, Elsevier, vol. 323(C).
    3. Zhao, Junjie & Tu, Zhengkai & Chan, Siew Hwa, 2022. "In-situ measurement of humidity distribution and its effect on the performance of a proton exchange membrane fuel cell," Energy, Elsevier, vol. 239(PD).
    4. Pan, Mingzhang & Pan, Chengjie & Li, Chao & Zhao, Jian, 2021. "A review of membranes in proton exchange membrane fuel cells: Transport phenomena, performance and durability," Renewable and Sustainable Energy Reviews, Elsevier, vol. 141(C).
    5. Lin, Zi & Liu, Xiaolei & Lao, Liyun & Liu, Hengxu, 2020. "Prediction of two-phase flow patterns in upward inclined pipes via deep learning," Energy, Elsevier, vol. 210(C).
    6. Kim, Young Sang & Kim, Dong Kyu & Ahn, Kook Young & Kim, Min Soo, 2020. "Real-time analysis of dry start-up characteristics of polymer electrolyte membrane fuel cell with water storage process under pressurized condition," Energy, Elsevier, vol. 199(C).

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