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Investigation of CO2 hydrate formation conditions for determining the optimum CO2 storage rate and energy: Modeling and experimental study

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  • Pivezhani, Farzane
  • Roosta, Hadi
  • Dashti, Ali
  • Mazloumi, S. Hossein

Abstract

In this study, optimum conditions for CO2 hydrate formation are investigated in order to determine the maximum CO2 storage rate and optimum energy consumption. First, a wide range of new experiments are carried out by using three-blade, six-blade and anchor impellers. For each experiment, a mass transfer model and a semi-empirical equation are utilized and the amount of energy consumption is measured. Temperature, impeller speed, initial pressure and volume of water, surface tension and the diffusion coefficient of CO2 are considered as the factors that affect the kinetics of CO2 hydrate. Maximum energy savings is achieved with maximum hydrate formation rate. It is found that the impeller speed is the most effective factor here. Moreover, at a given impeller speed, the hydrate formation rate is four times greater than the three-blade impeller when a combination of six-blade and anchor impellers is used. In addition, the rate of hydrate formation becomes 2, 1.6 and 3 times greater by reducing the volume of water, increasing the temperature and initial pressure and increasing the concentration of surfactant up to its optimum concentration in such a way that the energy consumption reduces from 1.92 kWh to 0.08 kWh when these effective parameters are changed.

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  • Pivezhani, Farzane & Roosta, Hadi & Dashti, Ali & Mazloumi, S. Hossein, 2016. "Investigation of CO2 hydrate formation conditions for determining the optimum CO2 storage rate and energy: Modeling and experimental study," Energy, Elsevier, vol. 113(C), pages 215-226.
    • Handle: RePEc:eee:energy:v:113:y:2016:i:c:p:215-226
    DOI: 10.1016/j.energy.2016.07.043
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    References listed on IDEAS

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    3. Liu, Fa-Ping & Li, Ai-Rong & Qing, Sheng-Lan & Luo, Ze-Dong & Ma, Yu-Ling, 2022. "Formation kinetics, mechanism of CO2 hydrate and its applications," Renewable and Sustainable Energy Reviews, Elsevier, vol. 159(C).
    4. Wang, Xiaolin & Zhang, Fengyuan & Lipiński, Wojciech, 2020. "Research progress and challenges in hydrate-based carbon dioxide capture applications," Applied Energy, Elsevier, vol. 269(C).
    5. Wang, Yiwei & Deng, Ye & Guo, Xuqiang & Sun, Qiang & Liu, Aixian & Zhang, Guangqing & Yue, Gang & Yang, Lanying, 2018. "Experimental and modeling investigation on separation of methane from coal seam gas (CSG) using hydrate formation," Energy, Elsevier, vol. 150(C), pages 377-395.
    6. Jyoti Shanker Pandey & Yousef Jouljamal Daas & Adam Paul Karcz & Nicolas von Solms, 2020. "Enhanced Hydrate-Based Geological CO 2 Capture and Sequestration as a Mitigation Strategy to Address Climate Change," Energies, MDPI, vol. 13(21), pages 1-28, October.
    7. Zhang, Kai & Lau, Hon Chung, 2022. "Sequestering CO2 as CO2 hydrate in an offshore saline aquifer by reservoir pressure management," Energy, Elsevier, vol. 239(PC).
    8. Liu, Fa-Ping & Li, Ai-Rong & Wang, Cheng & Ma, Yu-Ling, 2023. "Controlling and tuning CO2 hydrate nucleation and growth by metal-based ionic liquids," Energy, Elsevier, vol. 269(C).
    9. Sina Eslami & Behnam Farhangdoost & Hamidreza Shahverdi & Mohsen Mohammadi, 2021. "Surface grafting of silica nanoparticles using 3‐aminopropyl (triethoxysilane) to improve the CO2 absorption and enhance the gas consumption during the CO2 hydrate formation," Greenhouse Gases: Science and Technology, Blackwell Publishing, vol. 11(5), pages 939-953, October.
    10. Foroutan, Shima & Mohsenzade, Hanie & Dashti, Ali & Roosta, Hadi, 2021. "New insights into the evaluation of kinetic hydrate inhibitors and energy consumption in rocking and stirred cells," Energy, Elsevier, vol. 218(C).

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