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CO2 hydrate formation at atmospheric pressure using high efficiency absorbent and surfactants

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  • Choi, Jae Woo
  • Chung, Jin Tack
  • Kang, Yong Tae

Abstract

CO2 hydrate slurry can be used in a lot of practical applications such as CO2 capture, CO2 storage-transportation and CO2 sequestration processes. However, CO2 hydrate slurry is generally formed at low temperature and high pressure. The objectives of this study are to develop new absorbents to form CO2 hydrate at atmospheric pressure, and to evaluate the effects of surfactants and additives on the formation rate and the induction time of CO2 hydrate. THF (Tetrahydrofuran) is used as a surfactant and SDS (Sodium dodecyl sulfate) and nano particles such as Al2O3 are used as the additives. It is found that the maximum CO2 hydrate formation rate is enhanced up to 3.74 times by adding 0.6 wt% of SDS and 0.2 wt% of Al2O3 nanoparticles compared to the formation rate without the surfactants. Finally, it is concluded that THF 10 wt% and SDS 0.6 wt% with Al2O3 0.2 wt% is the optimum condition for CO2 hydrate formation rate enhancement.

Suggested Citation

  • Choi, Jae Woo & Chung, Jin Tack & Kang, Yong Tae, 2014. "CO2 hydrate formation at atmospheric pressure using high efficiency absorbent and surfactants," Energy, Elsevier, vol. 78(C), pages 869-876.
    • Handle: RePEc:eee:energy:v:78:y:2014:i:c:p:869-876
    DOI: 10.1016/j.energy.2014.10.081
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    References listed on IDEAS

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    1. Wang, Xiaolin & Dennis, Mike & Hou, Liangzhuo, 2014. "Clathrate hydrate technology for cold storage in air conditioning systems," Renewable and Sustainable Energy Reviews, Elsevier, vol. 36(C), pages 34-51.
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    Cited by:

    1. Sun, Qibei & Kang, Yong Tae, 2016. "Review on CO2 hydrate formation/dissociation and its cold energy application," Renewable and Sustainable Energy Reviews, Elsevier, vol. 62(C), pages 478-494.
    2. Cheng, Zucheng & Li, Shaohua & Liu, Yu & Zhang, Yi & Ling, Zheng & Yang, Mingjun & Jiang, Lanlan & Song, Yongchen, 2022. "Post-combustion CO2 capture and separation in flue gas based on hydrate technology：A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 154(C).
    3. Wang, Xiaolin & Zhang, Fengyuan & Lipiński, Wojciech, 2020. "Research progress and challenges in hydrate-based carbon dioxide capture applications," Applied Energy, Elsevier, vol. 269(C).
    4. Shuo Yan & Wenjie Dai & Shuli Wang & Yongchao Rao & Shidong Zhou, 2018. "Graphene Oxide: An Effective Promoter for CO 2 Hydrate Formation," Energies, MDPI, vol. 11(7), pages 1-13, July.
    5. Pivezhani, Farzane & Roosta, Hadi & Dashti, Ali & Mazloumi, S. Hossein, 2016. "Investigation of CO2 hydrate formation conditions for determining the optimum CO2 storage rate and energy: Modeling and experimental study," Energy, Elsevier, vol. 113(C), pages 215-226.
    6. Sun, Qibei & Kim, Shol & Kang, Yong Tae, 2017. "Study on dissociation characteristics of CO2 hydrate with THF for cooling application," Applied Energy, Elsevier, vol. 190(C), pages 249-256.
    7. Liu, Ni & Chen, Litao & Liu, Caixia & Yang, Liang & Liu, Daoping, 2020. "Experimental study of carbon dioxide hydrate formation in the presence of graphene oxide," Energy, Elsevier, vol. 211(C).
    8. Choi, Sung & Park, Jungjoon & Kang, Yong Tae, 2019. "Experimental investigation on CO2 hydrate formation/dissociation for cold thermal energy harvest and transportation applications," Applied Energy, Elsevier, vol. 242(C), pages 1358-1368.
    9. Li, Airong & Jiang, Lele & Tang, Siyao, 2017. "An experimental study on carbon dioxide hydrate formation using a gas-inducing agitated reactor," Energy, Elsevier, vol. 134(C), pages 629-637.
    10. Yang, Mingjun & Zheng, Jianan & Liu, Weiguo & Liu, Yu & Song, Yongchen, 2015. "Effects of C3H8 on hydrate formation and dissociation for integrated CO2 capture and desalination technology," Energy, Elsevier, vol. 93(P2), pages 1971-1979.
    11. Bi, Yuehong & Chen, Jie & Miao, Zhen, 2016. "Thermodynamic optimization for dissociation process of gas hydrates," Energy, Elsevier, vol. 106(C), pages 270-276.
    12. Theo, Wai Lip & Lim, Jeng Shiun & Hashim, Haslenda & Mustaffa, Azizul Azri & Ho, Wai Shin, 2016. "Review of pre-combustion capture and ionic liquid in carbon capture and storage," Applied Energy, Elsevier, vol. 183(C), pages 1633-1663.
    13. Liu, Fa-Ping & Li, Ai-Rong & Qing, Sheng-Lan & Luo, Ze-Dong & Ma, Yu-Ling, 2022. "Formation kinetics, mechanism of CO2 hydrate and its applications," Renewable and Sustainable Energy Reviews, Elsevier, vol. 159(C).
    14. Nguyen, Ngoc N. & La, Vinh T. & Huynh, Chinh D. & Nguyen, Anh V., 2022. "Technical and economic perspectives of hydrate-based carbon dioxide capture," Applied Energy, Elsevier, vol. 307(C).
    15. Kim, Shol & Lee, Seong Hyuk & Kang, Yong Tae, 2017. "Characteristics of CO2 hydrate formation/dissociation in H2O + THF aqueous solution and estimation of CO2 emission reduction by district cooling application," Energy, Elsevier, vol. 120(C), pages 362-373.
    16. Sun, Qibei & Kang, Yong Tae, 2015. "Experimental correlation for the formation rate of CO2 hydrate with THF (tetrahydrofuran) for cooling application," Energy, Elsevier, vol. 91(C), pages 712-719.
    17. Cheng, Chuanxiao & Wang, Fan & Tian, Yongjia & Wu, Xuehong & Zheng, Jili & Zhang, Jun & Li, Longwei & Yang, Penglin & Zhao, Jiafei, 2020. "Review and prospects of hydrate cold storage technology," Renewable and Sustainable Energy Reviews, Elsevier, vol. 117(C).

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    Keywords

    CO2 hydrate; Formation rate; Induction time; Surfactants;
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