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New approach for bio-jet fuels production by hydrodeoxygenation of higher alcohols derived from C-C coupling of bio-ethanol

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  • Liao, Junwei
  • Zhong, Quanwang
  • Gu, Juwen
  • Qiu, Songbai
  • Meng, Qingwei
  • Zhang, Qian
  • Wang, Tiejun

Abstract

A new approach for the synthesis of jet fuel hydrocarbon from bio-ethanol was developed, the integrated catalytic process of ethanol C-C coupling and heavy alcohols hydrodeoxygenation (HDO) was reported. The initial bio-ethanol C-C coupling process was fulfilled directly in aqueous environment over Na/Ni@C catalyst. The obtained high-carbon alcohols can be separated into C4-C7 and C8-C16 alcohols respectively through convenient fractional distillation. The obtained C8-C16 alcohols mainly consist of β-branched primary alcohol, which are desired precursors for jet fuel hydrocarbons. To maintain the branched carbon skeleton in the subsequent alcohol HDO process, the Co-Mo2C catalyst with excellent C-O bonds cleavage and carbon skeleton retention ability were developed. Jet fuel hydrocarbons of 56.7% yield obtained from this approach is mainly C8-C16 branched alkanes, which is beneficial for the cold flow properties. This strategy creates new opportunities for producing alternative jet fuel from the mature bio-ethanol industry.

Suggested Citation

  • Liao, Junwei & Zhong, Quanwang & Gu, Juwen & Qiu, Songbai & Meng, Qingwei & Zhang, Qian & Wang, Tiejun, 2022. "New approach for bio-jet fuels production by hydrodeoxygenation of higher alcohols derived from C-C coupling of bio-ethanol," Applied Energy, Elsevier, vol. 324(C).
    • Handle: RePEc:eee:appene:v:324:y:2022:i:c:s0306261922011126
    DOI: 10.1016/j.apenergy.2022.119843
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