IDEAS home Printed from https://ideas.repec.org/a/eee/appene/v279y2020ics0306261920312915.html
   My bibliography  Save this article

On deconvolution for understanding synergistic effects in co-pyrolysis of pinewood and polypropylene

Author

Listed:
  • Liu, Xuan
  • Burra, Kiran G.
  • Wang, Zhiwei
  • Li, Jinhu
  • Che, Defu
  • Gupta, Ashwani K.

Abstract

The synergistic effects on syngas observed in co-pyrolysis of pinewood and polypropylene (PP) were systematically investigated on a fixed bed reactor with tailored feedstock configurations in this paper. The synergistic effects focused on evolutionary and cumulative behaviors of evolved syngas were quantified by juxtaposing the results from co-pyrolysis of pinewood-PP mixtures with weighted results from the pyrolysis of pinewood and PP as individual components. Examination of different feedstock configurations revealed quantified contributions on volatile interactions and catalytic effect of char to the overall synergy. Results showed that syngas yield, H2 yield and CO yield with co-pyrolysis were promoted by 27%, 80% and 63%, respectively, as compared to the weighted aggregates from individual pyrolysis. Reduced char residue and improved energy yield in co-pyrolysis contributed to a remarkable enhancement in apparent thermal efficiency from 69.93% to 80.67%. Interactions between volatiles evolved from pinewood and PP suppressed CnHm formation while significantly enhancing H2 and CO yields. Mutual interactions between the volatiles accelerated the evolution of each gas component during co-pyrolysis. Pinewood char showed a negligible catalytic effect in evenly mixed configuration, but this effect was pronounced in separated PP and pinewood char. The porous structure of pinewood char can be easily blocked by the fused PP during co-pyrolysis, which was responsible for the delayed CnHm and syngas evolution. This paper provides results that help assist to elucidate the detailed synergistic mechanism during co-pyrolysis of biomass and plastic wastes.

Suggested Citation

  • Liu, Xuan & Burra, Kiran G. & Wang, Zhiwei & Li, Jinhu & Che, Defu & Gupta, Ashwani K., 2020. "On deconvolution for understanding synergistic effects in co-pyrolysis of pinewood and polypropylene," Applied Energy, Elsevier, vol. 279(C).
    • Handle: RePEc:eee:appene:v:279:y:2020:i:c:s0306261920312915
    DOI: 10.1016/j.apenergy.2020.115811
    as

    Download full text from publisher

    File URL: http://www.sciencedirect.com/science/article/pii/S0306261920312915
    Download Restriction: Full text for ScienceDirect subscribers only
    File URL: https://libkey.io/10.1016/j.apenergy.2020.115811?utm_source=ideas
    LibKey link: if access is restricted and if your library uses this service, LibKey will redirect you to where you can use your library subscription to access this item
    ---><---

    As the access to this document is restricted, you may want to search for a different version of it.

    References listed on IDEAS

    as
    1. Long, Huiling & Li, Xiaobing & Wang, Hong & Jia, Jingdun, 2013. "Biomass resources and their bioenergy potential estimation: A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 26(C), pages 344-352.
    2. Wang, Zhiwei & Burra, Kiran G. & Zhang, Mengju & Li, Xueqin & He, Xiaofeng & Lei, Tingzhou & Gupta, Ashwani K., 2020. "Syngas evolution and energy efficiency in CO2-assisted gasification of pine bark," Applied Energy, Elsevier, vol. 269(C).
    3. Chan, Fan Liang & Tanksale, Akshat, 2014. "Review of recent developments in Ni-based catalysts for biomass gasification," Renewable and Sustainable Energy Reviews, Elsevier, vol. 38(C), pages 428-438.
    4. Burra, K.G. & Gupta, A.K., 2018. "Kinetics of synergistic effects in co-pyrolysis of biomass with plastic wastes," Applied Energy, Elsevier, vol. 220(C), pages 408-418.
    5. Burra, K.G. & Gupta, A.K., 2018. "Synergistic effects in steam gasification of combined biomass and plastic waste mixtures," Applied Energy, Elsevier, vol. 211(C), pages 230-236.
    6. Inayat, Muddasser & Sulaiman, Shaharin A. & Kurnia, Jundika Candra & Shahbaz, Muhammad, 2019. "Effect of various blended fuels on syngas quality and performance in catalytic co-gasification: A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 105(C), pages 252-267.
    7. Oladejo, Jumoke M. & Adegbite, Stephen & Pang, Cheng Heng & Liu, Hao & Parvez, Ashak M. & Wu, Tao, 2017. "A novel index for the study of synergistic effects during the co-processing of coal and biomass," Applied Energy, Elsevier, vol. 188(C), pages 215-225.
    8. Policella, Matteo & Wang, Zhiwei & Burra, Kiran. G. & Gupta, Ashwani K., 2019. "Characteristics of syngas from pyrolysis and CO2-assisted gasification of waste tires," Applied Energy, Elsevier, vol. 254(C).
    9. Ahmed, I.I. & Nipattummakul, N. & Gupta, A.K., 2011. "Characteristics of syngas from co-gasification of polyethylene and woodchips," Applied Energy, Elsevier, vol. 88(1), pages 165-174, January.
    10. Wei, Juntao & Guo, Qinghua & Ding, Lu & Yoshikawa, Kunio & Yu, Guangsuo, 2017. "Synergy mechanism analysis of petroleum coke and municipal solid waste (MSW)-derived hydrochar co-gasification," Applied Energy, Elsevier, vol. 206(C), pages 1354-1363.
    11. Singh, P. & Déparrois, N. & Burra, K.G. & Bhattacharya, S. & Gupta, A.K., 2019. "Energy recovery from cross-linked polyethylene wastes using pyrolysis and CO2 assisted gasification," Applied Energy, Elsevier, vol. 254(C).
    Full references (including those not matched with items on IDEAS)

    Citations

    Citations are extracted by the CitEc Project, subscribe to its RSS feed for this item.
    as


    Cited by:

    1. Li, Jinhu & Ye, Xinhao & Burra, Kiran G. & Lu, Wei & Wang, Zhiwei & Liu, Xuan & Gupta, Ashwani K., 2023. "Synergistic effects during co-pyrolysis and co-gasification of polypropylene and polystyrene," Applied Energy, Elsevier, vol. 336(C).
    2. Li, Moshan & Lu, Yiyu & Hu, Erfeng & Yang, Yang & Tian, Yishui & Dai, Chongyang & Li, Chenhao, 2023. "Fast co-pyrolysis characteristics of high-alkali coal and polyethylene using infrared rapid heating," Energy, Elsevier, vol. 266(C).
    3. Hou, Yanmei & Feng, Zixing & He, Yuyu & Gao, Qi & Ni, Liangmeng & Su, Mengfu & Ren, Hao & Liu, Zhijia & Hu, Wanhe, 2022. "Co-pyrolysis characteristics and synergistic interaction of bamboo residues and disposable face mask," Renewable Energy, Elsevier, vol. 194(C), pages 415-425.
    4. Changheng Li & Qing Huang & Haixiang Zhang & Qingqing Wang & Rixin Xue & Genmao Guo & Jie Hu & Tinghang Li & Junfeng Wang & Shan Hu, 2021. "Characterization of Biochars Produced by Co-Pyrolysis of Hami Melon (Cantaloupes) Straw Mixed with Polypropylene and Their Adsorption Properties of Cadmium," IJERPH, MDPI, vol. 18(21), pages 1-17, October.
    5. Mariyam, Sabah & Shahbaz, Muhammad & Al-Ansari, Tareq & Mackey, Hamish. R & McKay, Gordon, 2022. "A critical review on co-gasification and co-pyrolysis for gas production," Renewable and Sustainable Energy Reviews, Elsevier, vol. 161(C).
    6. Burra, Kiran Raj G. & Liu, Xuan & Wang, Zhiwei & Li, Jinhu & Che, Defu & Gupta, Ashwani K., 2021. "Quantifying the sources of synergistic effects in co-pyrolysis of pinewood and polystyrene," Applied Energy, Elsevier, vol. 302(C).

    Most related items

    These are the items that most often cite the same works as this one and are cited by the same works as this one.
    1. Li, Jinhu & Burra, Kiran Raj G. & Wang, Zhiwei & Liu, Xuan & Gupta, Ashwani K., 2021. "Co-gasification of high-density polyethylene and pretreated pine wood," Applied Energy, Elsevier, vol. 285(C).
    2. Li, Jinhu & Ye, Xinhao & Burra, Kiran G. & Lu, Wei & Wang, Zhiwei & Liu, Xuan & Gupta, Ashwani K., 2023. "Synergistic effects during co-pyrolysis and co-gasification of polypropylene and polystyrene," Applied Energy, Elsevier, vol. 336(C).
    3. Burra, Kiran Raj G. & Liu, Xuan & Wang, Zhiwei & Li, Jinhu & Che, Defu & Gupta, Ashwani K., 2021. "Quantifying the sources of synergistic effects in co-pyrolysis of pinewood and polystyrene," Applied Energy, Elsevier, vol. 302(C).
    4. Wang, Zhiwei & Burra, Kiran G. & Li, Xueqin & Zhang, Mengju & He, Xiaofeng & Lei, Tingzhou & Gupta, Ashwani K., 2020. "CO2-assisted gasification of polyethylene terephthalate with focus on syngas evolution and solid yield," Applied Energy, Elsevier, vol. 276(C).
    5. Dmitry Porshnov, 2022. "Evolution of pyrolysis and gasification as waste to energy tools for low carbon economy," Wiley Interdisciplinary Reviews: Energy and Environment, Wiley Blackwell, vol. 11(1), January.
    6. Buentello-Montoya, D.A. & Duarte-Ruiz, C.A. & Maldonado-Escalante, J.F., 2023. "Co-gasification of waste PET, PP and biomass for energy recovery: A thermodynamic model to assess the produced syngas quality," Energy, Elsevier, vol. 266(C).
    7. Mariyam, Sabah & Shahbaz, Muhammad & Al-Ansari, Tareq & Mackey, Hamish. R & McKay, Gordon, 2022. "A critical review on co-gasification and co-pyrolysis for gas production," Renewable and Sustainable Energy Reviews, Elsevier, vol. 161(C).
    8. Ajorloo, Mojtaba & Ghodrat, Maryam & Scott, Jason & Strezov, Vladimir, 2022. "Modelling and statistical analysis of plastic biomass mixture co-gasification," Energy, Elsevier, vol. 256(C).
    9. Déparrois, N. & Singh, P. & Burra, K.G. & Gupta, A.K., 2019. "Syngas production from co-pyrolysis and co-gasification of polystyrene and paper with CO2," Applied Energy, Elsevier, vol. 246(C), pages 1-10.
    10. Ong, Hwai Chyuan & Chen, Wei-Hsin & Farooq, Abid & Gan, Yong Yang & Lee, Keat Teong & Ashokkumar, Veeramuthu, 2019. "Catalytic thermochemical conversion of biomass for biofuel production: A comprehensive review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 113(C), pages 1-1.
    11. AlNouss, Ahmed & McKay, Gordon & Al-Ansari, Tareq, 2020. "Enhancing waste to hydrogen production through biomass feedstock blending: A techno-economic-environmental evaluation," Applied Energy, Elsevier, vol. 266(C).
    12. Huang, Jijiang & Veksha, Andrei & Chan, Wei Ping & Giannis, Apostolos & Lisak, Grzegorz, 2022. "Chemical recycling of plastic waste for sustainable material management: A prospective review on catalysts and processes," Renewable and Sustainable Energy Reviews, Elsevier, vol. 154(C).
    13. Patrik Šuhaj & Jakub Husár & Juma Haydary, 2020. "Gasification of RDF and Its Components with Tire Pyrolysis Char as Tar-Cracking Catalyst," Sustainability, MDPI, vol. 12(16), pages 1-14, August.
    14. Zaini, Ilman Nuran & Gomez-Rueda, Yamid & García López, Cristina & Ratnasari, Devy Kartika & Helsen, Lieve & Pretz, Thomas & Jönsson, Pär Göran & Yang, Weihong, 2020. "Production of H2-rich syngas from excavated landfill waste through steam co-gasification with biochar," Energy, Elsevier, vol. 207(C).
    15. David Antonio Buentello-Montoya & Miguel Ángel Armenta-Gutiérrez & Victor Manuel Maytorena-Soria, 2023. "Parametric Modelling Study to Determine the Feasibility of the Co-Gasification of Macroalgae and Plastics for the Production of Hydrogen-Rich Syngas," Energies, MDPI, vol. 16(19), pages 1-18, September.
    16. Inayat, Muddasser & Sulaiman, Shaharin A. & Kurnia, Jundika Candra & Shahbaz, Muhammad, 2019. "Effect of various blended fuels on syngas quality and performance in catalytic co-gasification: A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 105(C), pages 252-267.
    17. Sajid, Muhammad & Raheem, Abdul & Ullah, Naeem & Asim, Muhammad & Ur Rehman, Muhammad Saif & Ali, Nisar, 2022. "Gasification of municipal solid waste: Progress, challenges, and prospects," Renewable and Sustainable Energy Reviews, Elsevier, vol. 168(C).
    18. Burra, K.G. & Gupta, A.K., 2018. "Kinetics of synergistic effects in co-pyrolysis of biomass with plastic wastes," Applied Energy, Elsevier, vol. 220(C), pages 408-418.
    19. Yao, Dingding & Wang, Chi-Hwa, 2020. "Pyrolysis and in-line catalytic decomposition of polypropylene to carbon nanomaterials and hydrogen over Fe- and Ni-based catalysts," Applied Energy, Elsevier, vol. 265(C).
    20. Zuhal Akyürek, 2019. "Sustainable Valorization of Animal Manure and Recycled Polyester: Co-pyrolysis Synergy," Sustainability, MDPI, vol. 11(8), pages 1-14, April.

    Corrections

    All material on this site has been provided by the respective publishers and authors. You can help correct errors and omissions. When requesting a correction, please mention this item's handle: RePEc:eee:appene:v:279:y:2020:i:c:s0306261920312915. See general information about how to correct material in RePEc.

    If you have authored this item and are not yet registered with RePEc, we encourage you to do it here. This allows to link your profile to this item. It also allows you to accept potential citations to this item that we are uncertain about.

    If CitEc recognized a bibliographic reference but did not link an item in RePEc to it, you can help with this form .

    If you know of missing items citing this one, you can help us creating those links by adding the relevant references in the same way as above, for each refering item. If you are a registered author of this item, you may also want to check the "citations" tab in your RePEc Author Service profile, as there may be some citations waiting for confirmation.

    For technical questions regarding this item, or to correct its authors, title, abstract, bibliographic or download information, contact: Catherine Liu (email available below). General contact details of provider: http://www.elsevier.com/wps/find/journaldescription.cws_home/405891/description#description .

    Please note that corrections may take a couple of weeks to filter through the various RePEc services.

    IDEAS is a RePEc service. RePEc uses bibliographic data supplied by the respective publishers.