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Waste to Carbon: Influence of Structural Modification on VOC Emission Kinetics from Stored Carbonized Refuse-Derived Fuel

Author

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  • Andrzej Białowiec

    (Faculty of Life Sciences and Technology, Wrocław University of Environmental and Life Sciences, 50-375 Wrocław, Poland)

  • Monika Micuda

    (Faculty of Life Sciences and Technology, Wrocław University of Environmental and Life Sciences, 50-375 Wrocław, Poland)

  • Antoni Szumny

    (Faculty of Biotechnology and Food Science, Wrocław University of Environmental and Life Sciences, 50-375 Wrocław, Poland)

  • Jacek Łyczko

    (Faculty of Biotechnology and Food Science, Wrocław University of Environmental and Life Sciences, 50-375 Wrocław, Poland)

  • Jacek A. Koziel

    (Department of Agricultural and Biosystems Engineering, Iowa State University, Ames, IA 50011, USA)

Abstract

The torrefaction of municipal solid waste is one of the solutions related to the Waste to Carbon concept, where high-quality fuel—carbonized refuse-derived fuel (CRDF)—is produced. An identified potential problem is the emission of volatile organic compounds (VOCs) during CRDF storage. Kinetic emission parameters have not yet been determined. It was also shown that CRDF can be pelletized for energy densification and reduced volume during storage and transportation. Thus, our working hypothesis was that structural modification (via pelletization) might mitigate VOC emissions and influence emission kinetics during CRDF storage. Two scenarios of CRDF structural modification on VOC emission kinetics were tested, (i) pelletization and (ii) pelletization with 10% binder addition and compared to ground (loose) CRDF (control). VOC emissions from simulated sealed CRDF storage were measured with headspace solid-phase microextraction and gas chromatography–mass spectrometry. It was found that total VOC emissions from stored CRDF follow the first-order kinetic model for both ground and pelletized material, while individual VOC emissions may deviate from this model. Pelletization significantly decreased (63%~86%) the maximum total VOC emission potential from stored CDRF. Research on improved sustainable CRDF storage is warranted. This could involve VOC emission mechanisms and environmental-risk management.

Suggested Citation

  • Andrzej Białowiec & Monika Micuda & Antoni Szumny & Jacek Łyczko & Jacek A. Koziel, 2019. "Waste to Carbon: Influence of Structural Modification on VOC Emission Kinetics from Stored Carbonized Refuse-Derived Fuel," Sustainability, MDPI, vol. 11(3), pages 1-13, February.
    • Handle: RePEc:gam:jsusta:v:11:y:2019:i:3:p:935-:d:205194
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    References listed on IDEAS

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    1. Jorge Miguel Carneiro Ribeiro & Radu Godina & João Carlos de Oliveira Matias & Leonel Jorge Ribeiro Nunes, 2018. "Future Perspectives of Biomass Torrefaction: Review of the Current State-Of-The-Art and Research Development," Sustainability, MDPI, vol. 10(7), pages 1-17, July.
    2. Andrzej Białowiec & Monika Micuda & Jacek A. Koziel, 2018. "Waste to Carbon: Densification of Torrefied Refuse-Derived Fuel," Energies, MDPI, vol. 11(11), pages 1-20, November.
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    Cited by:

    1. Jacek Łyczko & Jacek A. Koziel & Chumki Banik & Andrzej Białowiec, 2021. "The Proof-of-Concept: The Transformation of Naphthalene and Its Derivatives into Decalin and Its Derivatives during Thermochemical Processing of Sewage Sludge," Energies, MDPI, vol. 14(20), pages 1-11, October.
    2. Adrian Knapczyk & Sławomir Francik & Marcin Jewiarz & Agnieszka Zawiślak & Renata Francik, 2020. "Thermal Treatment of Biomass: A Bibliometric Analysis—The Torrefaction Case," Energies, MDPI, vol. 14(1), pages 1-31, December.
    3. Kacper Świechowski & Marek Liszewski & Przemysław Bąbelewski & Jacek A. Koziel & Andrzej Białowiec, 2019. "Fuel Properties of Torrefied Biomass from Pruning of Oxytree," Data, MDPI, vol. 4(2), pages 1-10, April.
    4. Paweł Stępień & Kacper Świechowski & Martyna Hnat & Szymon Kugler & Sylwia Stegenta-Dąbrowska & Jacek A. Koziel & Piotr Manczarski & Andrzej Białowiec, 2019. "Waste to Carbon: Biocoal from Elephant Dung as New Cooking Fuel," Energies, MDPI, vol. 12(22), pages 1-32, November.
    5. Kacper Świechowski & Martyna Hnat & Paweł Stępień & Sylwia Stegenta-Dąbrowska & Szymon Kugler & Jacek A. Koziel & Andrzej Białowiec, 2020. "Waste to Energy: Solid Fuel Production from Biogas Plant Digestate and Sewage Sludge by Torrefaction-Process Kinetics, Fuel Properties, and Energy Balance," Energies, MDPI, vol. 13(12), pages 1-37, June.
    6. Paweł Stępień & Małgorzata Serowik & Jacek A. Koziel & Andrzej Białowiec, 2019. "Waste to Carbon: Estimating the Energy Demand for Production of Carbonized Refuse-Derived Fuel," Sustainability, MDPI, vol. 11(20), pages 1-17, October.

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