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An Experimental Study on Thermal Performance of Graphite-Based Phase-Change Materials for High-Power Batteries

Author

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  • Danial Karimi

    (Research Group MOBI—Mobility, Logistics and Automotive Technology Research Centre, Vrije Universiteit Brussel, Pleinlaan 2, 1050 Brussels, Belgium
    Flanders Make, 3001 Heverlee, Belgium)

  • Hamidreza Behi

    (Research Group MOBI—Mobility, Logistics and Automotive Technology Research Centre, Vrije Universiteit Brussel, Pleinlaan 2, 1050 Brussels, Belgium
    Flanders Make, 3001 Heverlee, Belgium)

  • Joeri Van Mierlo

    (Research Group MOBI—Mobility, Logistics and Automotive Technology Research Centre, Vrije Universiteit Brussel, Pleinlaan 2, 1050 Brussels, Belgium
    Flanders Make, 3001 Heverlee, Belgium)

  • Maitane Berecibar

    (Research Group MOBI—Mobility, Logistics and Automotive Technology Research Centre, Vrije Universiteit Brussel, Pleinlaan 2, 1050 Brussels, Belgium)

Abstract

High-power lithium-ion capacitors (LiC) are hybrid energy storage systems (EES) with the combined benefits of lithium-ion batteries (LiB) and supercapacitors, such as high specific energy, high specific power, and a long lifetime. Such advanced technology can be used in high-power applications when high charging and discharging are demanded. Nevertheless, their performance and lifetime highly depend on temperature. In this context, this paper presents an optimal passive thermal management system (TMS) employing phase-change materials (PCM) combined with graphite to maintain the LiC maximum temperature. To evaluate the thermal response of the PCM and the PCM/G, experimental tests have been performed. The results exhibit that when the cell is under natural convection, the maximum temperature exceeds 55 °C, which is very harmful for the cell’s lifetime. Using the pure paraffin PCM, the maximum temperature of the LiC was reduced from 55.3 °C to 40.2 °C, which shows a 27.3% temperature reduction compared to natural convection. Using the PCM/G composite, the maximum temperature was reduced from 55.3 °C (natural convection) to 38.5 °C, a 30.4% temperature reduction compared to natural convection. The main reason for this temperature reduction is the PCM’s high latent heat fusion, as well as the graphite thermal conductivity. Moreover, different PCM/G thicknesses were investigated for which the maximum temperature of the LiC reached 38.02 °C, 38.57 °C, 41.18 °C, 43.61 °C, and 46.98 °C for the thicknesses of 15 mm, 10 mm, 7 mm, 5 mm, and 2 mm, respectively. In this context, a thickness of 10 mm is the optimum thickness to reduce the cost, weight, volume, and temperature.

Suggested Citation

  • Danial Karimi & Hamidreza Behi & Joeri Van Mierlo & Maitane Berecibar, 2022. "An Experimental Study on Thermal Performance of Graphite-Based Phase-Change Materials for High-Power Batteries," Energies, MDPI, vol. 15(7), pages 1-13, March.
    • Handle: RePEc:gam:jeners:v:15:y:2022:i:7:p:2515-:d:782501
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    References listed on IDEAS

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    1. Hamidreza Behi & Mohammadreza Behi & Ali Ghanbarpour & Danial Karimi & Aryan Azad & Morteza Ghanbarpour & Masud Behnia, 2021. "Enhancement of the Thermal Energy Storage Using Heat-Pipe-Assisted Phase Change Material," Energies, MDPI, vol. 14(19), pages 1-19, September.
    2. Safdari, Mojtaba & Ahmadi, Rouhollah & Sadeghzadeh, Sadegh, 2020. "Numerical investigation on PCM encapsulation shape used in the passive-active battery thermal management," Energy, Elsevier, vol. 193(C).
    3. Khaleghi, Sahar & Hosen, Md Sazzad & Karimi, Danial & Behi, Hamidreza & Beheshti, S. Hamidreza & Van Mierlo, Joeri & Berecibar, Maitane, 2022. "Developing an online data-driven approach for prognostics and health management of lithium-ion batteries," Applied Energy, Elsevier, vol. 308(C).
    4. Behi, Hamidreza & Karimi, Danial & Jaguemont, Joris & Gandoman, Foad Heidari & Kalogiannis, Theodoros & Berecibar, Maitane & Van Mierlo, Joeri, 2021. "Novel thermal management methods to improve the performance of the Li-ion batteries in high discharge current applications," Energy, Elsevier, vol. 224(C).
    5. Hamidreza Behi & Theodoros Kalogiannis & Mahesh Suresh Patil & Joeri Van Mierlo & Maitane Berecibar, 2021. "A New Concept of Air Cooling and Heat Pipe for Electric Vehicles in Fast Discharging," Energies, MDPI, vol. 14(20), pages 1-15, October.
    6. Danial Karimi & Sahar Khaleghi & Hamidreza Behi & Hamidreza Beheshti & Md Sazzad Hosen & Mohsen Akbarzadeh & Joeri Van Mierlo & Maitane Berecibar, 2021. "Lithium-Ion Capacitor Lifetime Extension through an Optimal Thermal Management System for Smart Grid Applications," Energies, MDPI, vol. 14(10), pages 1-14, May.
    7. Danial Karimi & Hamidreza Behi & Mohsen Akbarzadeh & Joeri Van Mierlo & Maitane Berecibar, 2021. "Holistic 1D Electro-Thermal Model Coupled to 3D Thermal Model for Hybrid Passive Cooling System Analysis in Electric Vehicles," Energies, MDPI, vol. 14(18), pages 1-20, September.
    8. Samimi, Fereshteh & Babapoor, Aziz & Azizi, Mohammadmehdi & Karimi, Gholamreza, 2016. "Thermal management analysis of a Li-ion battery cell using phase change material loaded with carbon fibers," Energy, Elsevier, vol. 96(C), pages 355-371.
    9. Hamidreza Behi & Danial Karimi & Rekabra Youssef & Mahesh Suresh Patil & Joeri Van Mierlo & Maitane Berecibar, 2021. "Comprehensive Passive Thermal Management Systems for Electric Vehicles," Energies, MDPI, vol. 14(13), pages 1-15, June.
    10. Seham Shahid & Martin Agelin-Chaab, 2017. "Analysis of Cooling Effectiveness and Temperature Uniformity in a Battery Pack for Cylindrical Batteries," Energies, MDPI, vol. 10(8), pages 1-17, August.
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    1. Karimi, Danial & Behi, Hamidreza & Berecibar, Maitane & Van Mierlo, Joeri, 2023. "A comprehensive coupled 0D-ECM to 3D-CFD thermal model for heat pipe assisted-air cooling thermal management system under fast charge and discharge," Applied Energy, Elsevier, vol. 339(C).

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