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Biomass based activated carbons for fuel cells

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  • Volperts, Aleksandrs
  • Plavniece, Ance
  • Dobele, Galina
  • Zhurinsh, Aivars
  • Kruusenberg, Ivar
  • Kaare, Kätlin
  • Locs, Janis
  • Tamasauskaite-Tamasiunaite, Loreta
  • Norkus, Eugenijus

Abstract

This study is devoted to wood and pulping residues based nitrogen doped nanoporous activated carbons for application as catalysts in fuel cells. Carbonaceous materials were obtained by thermochemical activation with NaOH, doping was performed using dicyandiamide. Changes of porous structure in the process of doping were studied and it was found that this treatment decreases porosity of activated carbons. Content of introduced nitrogen depended on the content of elemental oxygen in the structure of precursor. Electrocatalytic activity of activated and nitrogen doped wood char and black liquor was tested and was found to be comparable with commercial 20% Pt/C catalyst. The results of this study demonstrate that nitrogen doped activated carbons on the base of biomass are promising materials for application in fuel elements for oxygen reduction.

Suggested Citation

  • Volperts, Aleksandrs & Plavniece, Ance & Dobele, Galina & Zhurinsh, Aivars & Kruusenberg, Ivar & Kaare, Kätlin & Locs, Janis & Tamasauskaite-Tamasiunaite, Loreta & Norkus, Eugenijus, 2019. "Biomass based activated carbons for fuel cells," Renewable Energy, Elsevier, vol. 141(C), pages 40-45.
    • Handle: RePEc:eee:renene:v:141:y:2019:i:c:p:40-45
    DOI: 10.1016/j.renene.2019.04.002
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    References listed on IDEAS

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    1. Mark K. Debe, 2012. "Electrocatalyst approaches and challenges for automotive fuel cells," Nature, Nature, vol. 486(7401), pages 43-51, June.
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    1. Ance Plavniece & Galina Dobele & Aleksandrs Volperts & Aivars Zhurinsh, 2022. "Hydrothermal Carbonization vs. Pyrolysis: Effect on the Porosity of the Activated Carbon Materials," Sustainability, MDPI, vol. 14(23), pages 1-13, November.
    2. Ance Plavniece & Aleksandrs Volperts & Galina Dobele & Aivars Zhurinsh & Kätlin Kaare & Ivar Kruusenberg & Kaspars Kaprans & Ainars Knoks & Janis Kleperis, 2021. "Wood and Black Liquor-Based N-Doped Activated Carbon for Energy Application," Sustainability, MDPI, vol. 13(16), pages 1-17, August.
    3. Irfan, Muhammad & Liu, Xianhua & Li, Shengling & Khan, Izhar Ullah & Li, Yang & Wang, Jiao & Wang, Xin & Du, Xiwen & Wang, Guangyi & Zhang, Pingping, 2020. "High-performance glucose fuel cell with bimetallic Ni–Co composite anchored on reduced graphene oxide as anode catalyst," Renewable Energy, Elsevier, vol. 155(C), pages 1118-1126.
    4. Donghoon Shin & Akhil Francis & Purushothaman Vellayani Aravind & Theo Woudstra & Wiebren de Jong & Dirk Roekaerts, 2022. "Numerical Evaluation of Biochar Production Performance of Downdraft Gasifier by Thermodynamic Model," Energies, MDPI, vol. 15(20), pages 1-18, October.

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