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Experimental validation for enhancement of PEMFC cold start performance: Based on the optimization of micro porous layer

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  • Lin, Rui
  • Zhong, Di
  • Lan, Shunbo
  • Guo, Rong
  • Ma, Yunyang
  • Cai, Xin

Abstract

The cold start is one of the key research fields in PEMFC studies. The improvement of PEMFC’s (proton exchange membrane fuel cell) unassisted cold start performance has played a positive role in promoting the industrialization and commercialization of FCV (fuel cell vehicle). In this work, as the key point of MEA (membrane electrode assembly) structure optimization, MPL (micro porous layer) aims to make the generated water can be retained in the CLs (catalyst layer) and membrane in the form of membrane water at the initial period of cold start. And the cold start performance of the optimized MEA single cell and stack are observed and analyzed by the segmented cell technology. After comparing with the cold start performance of the commercial MEA single cell and stack under the same conditions, the improvement of the cold start performance is verified. The single cell of MEA1 could achieve a quick unassisted cold start at a start-up temperature of −15 °C, and the cold start time under 0.2 V in CV (constant voltage) mode is 153 s, while the commercial MEA single cell can only achieve a successful cold start under the minimum start-up temperature of −10 °C. The optimized MEA stack can realize a quick unassisted cold start at a startup temperature of −20 °C, and the cold start time under 0.1 V in CV mode is 63 s, while the commercial MEA stack can only achieve a successful cold start under the minimum startup temperature of −15 °C.

Suggested Citation

  • Lin, Rui & Zhong, Di & Lan, Shunbo & Guo, Rong & Ma, Yunyang & Cai, Xin, 2021. "Experimental validation for enhancement of PEMFC cold start performance: Based on the optimization of micro porous layer," Applied Energy, Elsevier, vol. 300(C).
    • Handle: RePEc:eee:appene:v:300:y:2021:i:c:s0306261921007182
    DOI: 10.1016/j.apenergy.2021.117306
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    References listed on IDEAS

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    1. Tang, Hong-Yue & Santamaria, Anthony D. & Bachman, John & Park, Jae Wan, 2013. "Vacuum-assisted drying of polymer electrolyte membrane fuel cell," Applied Energy, Elsevier, vol. 107(C), pages 264-270.
    2. Xu, Xinhai & Xu, Ben & Dong, Jun & Liu, Xiaotong, 2017. "Near-term analysis of a roll-out strategy to introduce fuel cell vehicles and hydrogen stations in Shenzhen China," Applied Energy, Elsevier, vol. 196(C), pages 229-237.
    3. Mark K. Debe, 2012. "Electrocatalyst approaches and challenges for automotive fuel cells," Nature, Nature, vol. 486(7401), pages 43-51, June.
    4. Zhong, Di & Lin, Rui & Jiang, Zhenghua & Zhu, Yike & Liu, Dengchen & Cai, Xin & Chen, Liang, 2020. "Low temperature durability and consistency analysis of proton exchange membrane fuel cell stack based on comprehensive characterizations," Applied Energy, Elsevier, vol. 264(C).
    5. Zhang, Qian & Lin, Rui & Técher, Ludovic & Cui, Xin, 2016. "Experimental study of variable operating parameters effects on overall PEMFC performance and spatial performance distribution," Energy, Elsevier, vol. 115(P1), pages 550-560.
    6. Lin, Rui & Zhu, Yike & Ni, Meng & Jiang, Zhenghua & Lou, Diming & Han, Lihang & Zhong, Di, 2019. "Consistency analysis of polymer electrolyte membrane fuel cell stack during cold start," Applied Energy, Elsevier, vol. 241(C), pages 420-432.
    7. Rabbani, Abid & Rokni, Masoud, 2013. "Effect of nitrogen crossover on purging strategy in PEM fuel cell systems," Applied Energy, Elsevier, vol. 111(C), pages 1061-1070.
    8. Huo, Sen & Jiao, Kui & Park, Jae Wan, 2019. "On the water transport behavior and phase transition mechanisms in cold start operation of PEM fuel cell," Applied Energy, Elsevier, vol. 233, pages 776-788.
    9. Amamou, A. & Kandidayeni, M. & Boulon, L. & Kelouwani, S., 2018. "Real time adaptive efficient cold start strategy for proton exchange membrane fuel cells," Applied Energy, Elsevier, vol. 216(C), pages 21-30.
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    Cited by:

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    2. Li, Bing & Wan, Kechuang & Xie, Meng & Chu, Tiankuo & Wang, Xiaolei & Li, Xiang & Yang, Daijun & Ming, Pingwen & Zhang, Cunman, 2022. "Durability degradation mechanism and consistency analysis for proton exchange membrane fuel cell stack," Applied Energy, Elsevier, vol. 314(C).
    3. Yang, Liu & Cao, Chenxi & Gan, Quanquan & Pei, Hao & Zhang, Qi & Li, Ping, 2022. "Revealing failure modes and effect of catalyst layer properties for PEM fuel cell cold start using an agglomerate model," Applied Energy, Elsevier, vol. 312(C).
    4. Kang, Zhenye & Wang, Hao & Liu, Yanrong & Mo, Jingke & Wang, Min & Li, Jing & Tian, Xinlong, 2022. "Exploring and understanding the internal voltage losses through catalyst layers in proton exchange membrane water electrolysis devices," Applied Energy, Elsevier, vol. 317(C).

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