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Hydrogen production by advanced proton exchange membrane (PEM) water electrolysers—Reduced energy consumption by improved electrocatalysis

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  • Marshall, A.
  • Børresen, B.
  • Hagen, G.
  • Tsypkin, M.
  • Tunold, R.

Abstract

Proton exchange membrane (PEM) water electrolysis systems offers several advantages over traditional technologies including greater energy efficiency, higher production rates, and more compact design. Normally in these systems, the anode has the largest overpotential at typical operating current densities. By development of the electrocatalytic material used for the oxygen evolving electrode, great improvements in efficiency can be made. We find that using cyclic voltammetry and steady state polarisation analysis, enables us to separate the effects of true specific electrocatalytic activity and active surface area. Understanding these two factors is critical in developing better electrocatalytic materials in order to further improve the performance of PEM water electrolysis cells. The high current performance of a PEM water electrolysis cell using these oxides as the anode electrocatalyst has also been examined by steady state polarisation measurements and electrochemical impedance spectroscopy. Overall the best cell voltage obtained is 1.567V at 1Acm−2 and 80°C was achieved when using Nafion 115 as the electrolyte membrane.

Suggested Citation

  • Marshall, A. & Børresen, B. & Hagen, G. & Tsypkin, M. & Tunold, R., 2007. "Hydrogen production by advanced proton exchange membrane (PEM) water electrolysers—Reduced energy consumption by improved electrocatalysis," Energy, Elsevier, vol. 32(4), pages 431-436.
    • Handle: RePEc:eee:energy:v:32:y:2007:i:4:p:431-436
    DOI: 10.1016/j.energy.2006.07.014
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    3. Deshmukh, Sachin S. & Boehm, Robert F., 2008. "Review of modeling details related to renewably powered hydrogen systems," Renewable and Sustainable Energy Reviews, Elsevier, vol. 12(9), pages 2301-2330, December.
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    8. Wang, Shuofeng & Ji, Changwei & Zhang, Jian & Zhang, Bo, 2011. "Comparison of the performance of a spark-ignited gasoline engine blended with hydrogen and hydrogen–oxygen mixtures," Energy, Elsevier, vol. 36(10), pages 5832-5837.
    9. Ravichandran, S. & Venkatkarthick, R. & Sankari, A. & Vasudevan, S. & Jonas Davidson, D. & Sozhan, G., 2014. "Platinum deposition on the nafion membrane by impregnation reduction using nonionic surfactant for water electrolysis – An alternate approach," Energy, Elsevier, vol. 68(C), pages 148-151.
    10. Pantò, Fabiola & Siracusano, Stefania & Briguglio, Nicola & Aricò, Antonino Salvatore, 2020. "Durability of a recombination catalyst-based membrane-electrode assembly for electrolysis operation at high current density," Applied Energy, Elsevier, vol. 279(C).
    11. Santos, D.M.F. & Šljukić, B. & Sequeira, C.A.C. & Macciò, D. & Saccone, A. & Figueiredo, J.L., 2013. "Electrocatalytic approach for the efficiency increase of electrolytic hydrogen production: Proof-of-concept using platinum--dysprosium alloys," Energy, Elsevier, vol. 50(C), pages 486-492.
    12. Abdollahipour, Armin & Sayyaadi, Hoseyn, 2022. "Optimal design of a hybrid power generation system based on integrating PEM fuel cell and PEM electrolyzer as a moderator for micro-renewable energy systems," Energy, Elsevier, vol. 260(C).
    13. Sequeira, C.A.C. & Santos, D.M.F. & Brito, P.S.D., 2011. "Electrocatalytic activity of simple and modified Fe–P electrodeposits for hydrogen evolution from alkaline media," Energy, Elsevier, vol. 36(2), pages 847-853.
    14. Abdollahipour, Armin & Sayyaadi, Hoseyn, 2022. "A novel electrochemical refrigeration system based on the combined proton exchange membrane fuel cell-electrolyzer," Applied Energy, Elsevier, vol. 316(C).
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    16. M, Aravindan & V, Madhan Kumar & Hariharan, V.S. & Narahari, Tharun & P, Arun Kumar & K, Madhesh & G, Praveen Kumar & Prabakaran, Rajendran, 2023. "Fuelling the future: A review of non-renewable hydrogen production and storage techniques," Renewable and Sustainable Energy Reviews, Elsevier, vol. 188(C).
    17. Samuel Simon Araya & Vincenzo Liso & Xiaoti Cui & Na Li & Jimin Zhu & Simon Lennart Sahlin & Søren Højgaard Jensen & Mads Pagh Nielsen & Søren Knudsen Kær, 2020. "A Review of The Methanol Economy: The Fuel Cell Route," Energies, MDPI, vol. 13(3), pages 1-32, January.
    18. Vo, Truc T.Q. & Rajendran, Karthik & Murphy, Jerry D., 2018. "Can power to methane systems be sustainable and can they improve the carbon intensity of renewable methane when used to upgrade biogas produced from grass and slurry?," Applied Energy, Elsevier, vol. 228(C), pages 1046-1056.
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    20. El-Askary, W.A. & Sakr, I.M. & Ibrahim, K.A. & Balabel, A., 2015. "Hydrodynamics characteristics of hydrogen evolution process through electrolysis: Numerical and experimental studies," Energy, Elsevier, vol. 90(P1), pages 722-737.
    21. Qian, Guangfu & Mo, Yanshan & Yu, Chen & Zhang, Hao & Yu, Tianqi & Luo, Lin & Yin, Shibin, 2020. "Free-standing bimetallic CoNiTe2 nanosheets as efficient catalysts with high stability at large current density for oxygen evolution reaction," Renewable Energy, Elsevier, vol. 162(C), pages 2190-2196.

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