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Oxygen-enriched hierarchical porous carbons derived from lignite for high-performance supercapacitors

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  • Liu, Hongwei
  • Wang, Yongzhen
  • Lv, Liang
  • Liu, Xiao
  • Wang, Ziqi
  • Liu, Jun

Abstract

Functional coal-based carbon materials with reasonable pore structure and surface properties have attracted extensive attention for use in high-performance supercapacitors. Herein, a ball milling-assisted bimetallic salt catalytic pyrolysis strategy was developed to prepare oxygen-doped hierarchical porous carbon (OHPC) derived from lignite. The optimized OHPC-1 shows a large specific surface area (1638 m2/g), rational pore structure distribution (mesopores account for 71.3%), and suitable oxygen doping, which ensure sufficient charge storage, rapid electrolyte ions diffusion, as well as the contributed pseudocapacitance. The obtained OHPC-1 exhibits a high specific capacitance of 283 F/g at 0.5 A/g in 6.0 M KOH electrolyte (operating voltage 1.2 V). The assembled OHPC-1//OHPC-1 symmetrical capacitor delivers a high energy density of 16.5 Wh/kg at the power density of 300 W/kg with long cycling stability. In sum, the proposed facile route for high-value utilization of lignite looks promising for the preparation of cost-effective porous carbons for high-performance supercapacitors.

Suggested Citation

  • Liu, Hongwei & Wang, Yongzhen & Lv, Liang & Liu, Xiao & Wang, Ziqi & Liu, Jun, 2023. "Oxygen-enriched hierarchical porous carbons derived from lignite for high-performance supercapacitors," Energy, Elsevier, vol. 269(C).
    • Handle: RePEc:eee:energy:v:269:y:2023:i:c:s0360544223001019
    DOI: 10.1016/j.energy.2023.126707
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    1. Yang, Jie & Dong, Senlin & Xie, Longgui & Cen, Qihong & Zheng, Dalong & Ma, Liping & Dai, Quxiu, 2023. "Analysis of hydrogen-rich syngas generation in chemical looping gasification of lignite: Application of carbide slag as the oxygen carrier, hydrogen carrier, and in-situ carbon capture agent," Energy, Elsevier, vol. 283(C).
    2. Ganesan Sriram & Mahaveer Kurkuri & Tae Hwan Oh, 2023. "Recent Trends in Highly Porous Structured Carbon Electrodes for Supercapacitor Applications: A Review," Energies, MDPI, vol. 16(12), pages 1-36, June.

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