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Oxygen-enriched gasification of lignocellulosic biomass: Syngas analysis, physicochemical characteristics of the carbon-rich material and its utilization as an anode in lithium ion battery

Author

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  • Chen, Tianju
  • Zhang, Juan
  • Wang, Zhiqi
  • Zhao, Ruidong
  • He, Jianjiang
  • Wu, Jinhu
  • Qin, Jianguang

Abstract

Syngas from conventional biomass gasification has low calorific value, low H2/CO ratio, and high tar content. Oxygen and steam gasification are effective ways to improve the quality of syngas. Gas-carbon co-generation is possible due to the lower temperature at the bottom of the downdraft fixed-bed gasifier. Oxygen-enriched gasification of biomass is investigated in this work. The H2 content in the syngas increased from 34 v% to 45 v% when steam was added. The physicochemical characteristics of the activation carbon (AC) are determined by the Brunauer-Emmett-Teller (BET), Raman, Fourier transform infrared spectrometry (FTIR), X-ray diffractometer (XRD), X-ray photoelectron spectroscopy (XPS), scanning electron microscopy (SEM) and transmission electron microscope (TEM). In addition, the AC from the activation of carbon-rich production used as anode in lithium ion batteries (LIBs) is attempted. The BET of the ACo and ACo-s is 1715.32 m2 g−1 and 1409.02 m2 g−1, respectively. The biomass-derived carbon material had less graphitic crystalline structure, less functional groups and graphene-like porous structure after activation. At the current density of 100 mA g−1, a reversible lithium storage capacity of 327 mAh g−1 for a carbon-based electrode is obtained. This research provides a new roadmap for high-value-added products from the thermo-chemical conversion of biomass.

Suggested Citation

  • Chen, Tianju & Zhang, Juan & Wang, Zhiqi & Zhao, Ruidong & He, Jianjiang & Wu, Jinhu & Qin, Jianguang, 2020. "Oxygen-enriched gasification of lignocellulosic biomass: Syngas analysis, physicochemical characteristics of the carbon-rich material and its utilization as an anode in lithium ion battery," Energy, Elsevier, vol. 212(C).
    • Handle: RePEc:eee:energy:v:212:y:2020:i:c:s0360544220318788
    DOI: 10.1016/j.energy.2020.118771
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    Cited by:

    1. Yang, Shiliang & Liang, Jin & Wang, Shuai & Wang, Hua, 2021. "High-fidelity investigation of thermochemical conversion of biomass material in a full-loop circulating fluidized bed gasifier," Energy, Elsevier, vol. 224(C).
    2. Liu, Hongwei & Wang, Yongzhen & Lv, Liang & Liu, Xiao & Wang, Ziqi & Liu, Jun, 2023. "Oxygen-enriched hierarchical porous carbons derived from lignite for high-performance supercapacitors," Energy, Elsevier, vol. 269(C).
    3. He, Yifeng & Liu, Ronghou & Yellezuome, Dominic & Peng, Wanxi & Tabatabaei, Meisam, 2022. "Upgrading of biomass-derived bio-oil via catalytic hydrogenation with Rh and Pd catalysts," Renewable Energy, Elsevier, vol. 184(C), pages 487-497.
    4. Małgorzata Sieradzka & Agata Mlonka-Mędrala & Izabela Kalemba-Rec & Markus Reinmöller & Felix Küster & Wojciech Kalawa & Aneta Magdziarz, 2022. "Evaluation of Physical and Chemical Properties of Residue from Gasification of Biomass Wastes," Energies, MDPI, vol. 15(10), pages 1-19, May.

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