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Experimental study of the influence of dynamic load cycle and operating parameters on the durability of PEMFC

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  • Chu, Tiankuo
  • Xie, Meng
  • Yu, Yue
  • Wang, Baoyun
  • Yang, Daijun
  • Li, Bing
  • Ming, Pingwen
  • Zhang, Cunman

Abstract

Driving conditions and control strategies have closely been associated with proton exchange membrane fuel cell (PEMFC) durability for vehicle applications. This study tests two identical 3-cell PEMFC stacks for both 1000 h under two dynamic load cycles with different load ranges and inconsistent operating parameters. We calculated and analyzed the attenuation of fuel cell performance under different dynamic load cycles. After 1000 h, the mean cell voltage degradation percentage under (Dynamic load cycles) DLC-01and DLC-02 at 1000 mA cm−2 were 5.90% and 5.67%, respectively. Compared to DLC-01, the voltage degradation percentages of DLC-02 under low current densities were significantly lower, particularly in the first 400 h period. The EIS (Electrochemical Impedance Spectroscopy) revealed the evolution of the ohmic, charge transfer, and mass transport resistances. A more severe catalyst layer degradation was depicted by the significant increase of charge transfer resistance in the first 400 h under the DLC-01. An empirical formula was proposed to calculate the corresponding polarization losses quntitatively; this was key in distinguishing the source of different voltage loss. Collectively, this article uncovers the influence of the operating condition and control strategy on fuel cell durability.

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  • Chu, Tiankuo & Xie, Meng & Yu, Yue & Wang, Baoyun & Yang, Daijun & Li, Bing & Ming, Pingwen & Zhang, Cunman, 2022. "Experimental study of the influence of dynamic load cycle and operating parameters on the durability of PEMFC," Energy, Elsevier, vol. 239(PD).
    • Handle: RePEc:eee:energy:v:239:y:2022:i:pd:s0360544221026050
    DOI: 10.1016/j.energy.2021.122356
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    References listed on IDEAS

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    1. Mark K. Debe, 2012. "Electrocatalyst approaches and challenges for automotive fuel cells," Nature, Nature, vol. 486(7401), pages 43-51, June.
    2. Pei, Pucheng & Chen, Huicui, 2014. "Main factors affecting the lifetime of Proton Exchange Membrane fuel cells in vehicle applications: A review," Applied Energy, Elsevier, vol. 125(C), pages 60-75.
    3. Chen, Qin & Zhang, Guobin & Zhang, Xuzhong & Sun, Cheng & Jiao, Kui & Wang, Yun, 2021. "Thermal management of polymer electrolyte membrane fuel cells: A review of cooling methods, material properties, and durability," Applied Energy, Elsevier, vol. 286(C).
    4. Wang, Junye, 2017. "System integration, durability and reliability of fuel cells: Challenges and solutions," Applied Energy, Elsevier, vol. 189(C), pages 460-479.
    5. Stacy, John & Regmi, Yagya N. & Leonard, Brian & Fan, Maohong, 2017. "The recent progress and future of oxygen reduction reaction catalysis: A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 69(C), pages 401-414.
    6. Chu, Tiankuo & Zhang, Ruofan & Wang, Yanbo & Ou, Mingyang & Xie, Meng & Shao, Hangyu & Yang, Daijun & Li, Bing & Ming, Pingwen & Zhang, Cunman, 2021. "Performance degradation and process engineering of the 10 kW proton exchange membrane fuel cell stack," Energy, Elsevier, vol. 219(C).
    7. Zhang, Guobin & Yuan, Hao & Wang, Yun & Jiao, Kui, 2019. "Three-dimensional simulation of a new cooling strategy for proton exchange membrane fuel cell stack using a non-isothermal multiphase model," Applied Energy, Elsevier, vol. 255(C).
    8. Shan, Jing & Gazdzicki, Pawel & Lin, Rui & Schulze, Mathias & Friedrich, K. Andreas, 2017. "Local resolved investigation of hydrogen crossover in polymer electrolyte fuel cell," Energy, Elsevier, vol. 128(C), pages 357-365.
    9. Chen, Huicui & Song, Zhen & Zhao, Xin & Zhang, Tong & Pei, Pucheng & Liang, Chen, 2018. "A review of durability test protocols of the proton exchange membrane fuel cells for vehicle," Applied Energy, Elsevier, vol. 224(C), pages 289-299.
    10. Garcia-Sanchez, D. & Morawietz, T. & da Rocha, P. Gama & Hiesgen, R. & Gazdzicki, P. & Friedrich, K.A., 2020. "Local impact of load cycling on degradation in polymer electrolyte fuel cells," Applied Energy, Elsevier, vol. 259(C).
    11. Olabi, A.G. & Wilberforce, Tabbi & Abdelkareem, Mohammad Ali, 2021. "Fuel cell application in the automotive industry and future perspective," Energy, Elsevier, vol. 214(C).
    Full references (including those not matched with items on IDEAS)

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    3. Rabeh Abbassi & Salem Saidi & Abdelkader Abbassi & Houssem Jerbi & Mourad Kchaou & Bilal Naji Alhasnawi, 2023. "Accurate Key Parameters Estimation of PEMFCs’ Models Based on Dandelion Optimization Algorithm," Mathematics, MDPI, vol. 11(6), pages 1-21, March.
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    5. Sun, Yun & Lin, Yixiong & Wang, Qinglian & Yang, Chen & Yin, Wang & Wan, Zhongmin & Qiu, Ting, 2024. "Novel design and numerical investigation of a windward bend flow field for proton exchange membrane fuel cell," Energy, Elsevier, vol. 290(C).
    6. Li, Haolong & Chen, Qihong & Zhang, Liyan & Liu, Li & Xiao, Peng, 2023. "Degradation prediction of proton exchange membrane fuel cell based on the multi-inputs Bi-directional long short-term memory," Applied Energy, Elsevier, vol. 344(C).
    7. Huang, Weifeng & Niu, Tong & Zhang, Caizhi & Fu, Zuhang & Zhang, Yuqi & Zhou, Weijiang & Pan, Zehua & Zhang, Kaiqing, 2023. "Experimental study of the performance degradation of proton exchange membrane fuel cell based on a multi-module stack under selected load profiles by clustering algorithm," Energy, Elsevier, vol. 270(C).
    8. Lin, Rui & Dong, Mengcheng & Lan, Shunbo & Lou, Mingyu, 2023. "Numerical simulation of liquid water transport in perforated cracks of microporous layer," Energy, Elsevier, vol. 262(PB).
    9. Guan, Dong & Pan, Biyu & Chen, Zhen & Li, Jing & Shen, Hui & Pang, Huan, 2023. "Quantitative modeling and bio-inspired optimization the clamping load on the bipolar plate in PEMFC," Energy, Elsevier, vol. 263(PD).
    10. Chen, Dongfang & Pei, Pucheng & Meng, Yining & Ren, Peng & Li, Yuehua & Wang, Mingkai & Wang, Xizhong, 2022. "Novel extraction method of working condition spectrum for the lifetime prediction and energy management strategy evaluation of automotive fuel cells," Energy, Elsevier, vol. 255(C).
    11. Fan, Lixin & Tu, Zhengkai & Chan, Siew Hwa, 2022. "Technological and Engineering design of a megawatt proton exchange membrane fuel cell system," Energy, Elsevier, vol. 257(C).
    12. Zhou, Yu & Chen, Ben & Chen, Wenshang & Deng, Qihao & Shen, Jun & Tu, Zhengkai, 2022. "A novel opposite sinusoidal wave flow channel for performance enhancement of proton exchange membrane fuel cell," Energy, Elsevier, vol. 261(PB).
    13. Saka, Kenan & Orhan, Mehmet Fatih, 2022. "Analysis of stack operating conditions for a polymer electrolyte membrane fuel cell," Energy, Elsevier, vol. 258(C).
    14. Rahmani, Ebrahim & Moradi, Tofigh & Ghandehariun, Samane & Naterer, Greg F. & Ranjbar, Amirhossein, 2023. "Enhanced mass transfer and water discharge in a proton exchange membrane fuel cell with a raccoon channel flow field," Energy, Elsevier, vol. 264(C).
    15. Meng, Kai & Chen, Ben & Zhou, Haoran & Shen, Jun & Shen, Zuguo & Tu, Zhengkai, 2022. "Investigation on degradation mechanism of hydrogen–oxygen proton exchange membrane fuel cell under current cyclic loading," Energy, Elsevier, vol. 242(C).
    16. Huang, Ruike & Peng, Yiqiang & Yang, Jibin & Xu, Xiaohui & Deng, Pengyi, 2022. "Correlation analysis and prediction of PEM fuel cell voltage during start-stop operation based on real-world driving data," Energy, Elsevier, vol. 260(C).
    17. Siwen Gu & Jiaan Wang & Xinmin You & Yu Zhuang, 2023. "Investigating the Parameter-Driven Cathode Gas Diffusion of PEMFCs with a Piecewise Linearization Model," Energies, MDPI, vol. 16(9), pages 1-12, April.

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