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Study on premixed combustion characteristics of co-firing ammonia/methane fuels

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  • Xiao, Hua
  • Valera-Medina, Agustin
  • Bowen, Philip J

Abstract

Ammonia is believed to eventually play an important role in substituting conventional fossil fuels for future energy systems. In this study, to gain a deep insight into the combustion properties of co-firing ammonia/methane fuel blends for the power and steel industry, a detailed chemical-kinetics mechanism model was developed for comprehensively modelling ammonia/methane fuels combustion. Characteristics of ignition delay time, unstretched laminar flame speed and NO, CO2 and CO emissions in the exhaust gas were obtained over a wide range of equivalence ratios and ammonia fractions. High NO emissions will be a main problem as CO and CO2 emissions tend to drop when adding ammonia into methane. To gain a further understanding of the effect of ammonia substituting methane for combustion use, analyses of laminar premixed flame structures were performed. The impact of ammonia substitution was illustrated by analysing relevant specific radicals. Furthermore, to study the combustion characteristics of ammonia/methane under more practical conditions, effects of engine relevant conditions (elevated pressure and initial temperature) were also studied. Results indicate that pressure has a more prominent effect than initial temperature and there is a good potential that unwanted emissions can be reduced significantly under industrial conditions.

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  • Xiao, Hua & Valera-Medina, Agustin & Bowen, Philip J, 2017. "Study on premixed combustion characteristics of co-firing ammonia/methane fuels," Energy, Elsevier, vol. 140(P1), pages 125-135.
    • Handle: RePEc:eee:energy:v:140:y:2017:i:p1:p:125-135
    DOI: 10.1016/j.energy.2017.08.077
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    References listed on IDEAS

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    1. Valera-Medina, Agustin & Marsh, Richard & Runyon, Jon & Pugh, Daniel & Beasley, Paul & Hughes, Timothy & Bowen, Phil, 2017. "Ammonia–methane combustion in tangential swirl burners for gas turbine power generation," Applied Energy, Elsevier, vol. 185(P2), pages 1362-1371.
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    6. Hookyung Lee & Min-Jung Lee, 2021. "Recent Advances in Ammonia Combustion Technology in Thermal Power Generation System for Carbon Emission Reduction," Energies, MDPI, vol. 14(18), pages 1-29, September.
    7. Liu, Shibo & Zou, Chun & Song, Yu & Cheng, Sizhe & Lin, Qianjin, 2019. "Experimental and numerical study of laminar flame speeds of CH4/NH3 mixtures under oxy-fuel combustion," Energy, Elsevier, vol. 175(C), pages 250-258.
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    10. Nithin Mukundakumar & Rob Bastiaans, 2022. "DNS Study of Spherically Expanding Premixed Turbulent Ammonia-Hydrogen Flame Kernels, Effect of Equivalence Ratio and Hydrogen Content," Energies, MDPI, vol. 15(13), pages 1-16, June.
    11. Muhammad Aziz & Agung Tri Wijayanta & Asep Bayu Dani Nandiyanto, 2020. "Ammonia as Effective Hydrogen Storage: A Review on Production, Storage and Utilization," Energies, MDPI, vol. 13(12), pages 1-25, June.
    12. Li, Jun & Huang, Hongyu & Deng, Lisheng & He, Zhaohong & Osaka, Yugo & Kobayashi, Noriyuki, 2019. "Effect of hydrogen addition on combustion and heat release characteristics of ammonia flame," Energy, Elsevier, vol. 175(C), pages 604-617.
    13. Wang, Siqi & Chong, Cheng Tung & Xie, Tian & Józsa, Viktor & Ng, Jo-Han, 2023. "Ammonia/methane dual-fuel injection and Co-firing strategy in a swirl flame combustor for pollutant emissions control," Energy, Elsevier, vol. 281(C).
    14. Wei, Wenwen & Li, Gesheng & Zhang, Zunhua & Long, Yanxiang & Zhang, Hanyuyang & Huang, Yong & Zhou, Mengni & Wei, Yi, 2023. "Effects of ammonia addition on the performance and emissions for a spark-ignition marine natural gas engine," Energy, Elsevier, vol. 272(C).
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    17. Skabelund, Brent B. & Stechel, Ellen B. & Milcarek, Ryan J., 2023. "Thermodynamic analysis of a gas turbine utilizing ternary CH4/H2/NH3 fuel blends," Energy, Elsevier, vol. 282(C).

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