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Prediction of non-uniform reactions in PEMFC based on the multi-physics quantity fusion graph auto-encoder network

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  • Zhang, Pulin
  • Qiu, Diankai
  • Peng, Linfa

Abstract

To meet the demands of high power output, proton exchange membrane fuel cells (PEMFCs) with large area have become a significant focus of research. However, non-uniform reactions in fuel cells are unavoidable in practice, leading to performance degradation and reduced stack lifespan. Understanding the distribution of physical quantity changes within the fuel cell and predicting its future internal states are crucial for control and maintenance of fuel cells. This paper proposes a Multi-Physics quantity fusion Graph Auto-Encoder network (MP-GAE), which is a transient prediction model for the performance and multi-physical field distribution in fuel cell by focusing on three aspects: reaction time, spatial location, and the coupling relationships of multiple physical fields. Based on graph attention mechanisms and temporal networks, a Partitioned Temporal Graph Attention Network (PT-GAT) is established to extract spatiotemporal regularities. Based on the Auto-Encoder structure and the interrelationships among the five physical quantities, these prediction models are integrated into MP-GAE to enhance the model's prediction performance. Experimental results show that MP-GAE can accurately predict changes in physical fields and performs well under complex conditions such as variations in load current density, gas pressure, inlet relative humidity, stoichiometric ratio and temperature. The proposed model effectively predicts the non-uniform variation processes of five physical quantities within the reaction area of fuel cells, providing information and assistance for the control and management of large-area fuel cells.

Suggested Citation

  • Zhang, Pulin & Qiu, Diankai & Peng, Linfa, 2025. "Prediction of non-uniform reactions in PEMFC based on the multi-physics quantity fusion graph auto-encoder network," Applied Energy, Elsevier, vol. 383(C).
  • Handle: RePEc:eee:appene:v:383:y:2025:i:c:s0306261925000959
    DOI: 10.1016/j.apenergy.2025.125365
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    References listed on IDEAS

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    1. Pu, Zonghua & Zhang, Gaixia & Hassanpour, Amir & Zheng, Dewen & Wang, Shanyu & Liao, Shijun & Chen, Zhangxin & Sun, Shuhui, 2021. "Regenerative fuel cells: Recent progress, challenges, perspectives and their applications for space energy system," Applied Energy, Elsevier, vol. 283(C).
    2. Li, Jianwei & Yan, Chonghao & Yang, Qingqing & Hao, Dong & Zou, Weitao & Gao, Lei & Zhao, Xuan, 2023. "Quantitative diagnosis of PEMFC membrane humidity with a vector-distance based characteristic mapping approach," Applied Energy, Elsevier, vol. 335(C).
    3. Kim, Bosung & Cha, Dowon & Kim, Yongchan, 2015. "The effects of air stoichiometry and air excess ratio on the transient response of a PEMFC under load change conditions," Applied Energy, Elsevier, vol. 138(C), pages 143-149.
    4. He, Yuxuan & Su, Huai & Zio, Enrico & Peng, Shiliang & Fan, Lin & Yang, Zhaoming & Yang, Zhe & Zhang, Jinjun, 2023. "A systematic method of remaining useful life estimation based on physics-informed graph neural networks with multisensor data," Reliability Engineering and System Safety, Elsevier, vol. 237(C).
    5. Zhou, Su & Fan, Lei & Zhang, Gang & Gao, Jianhua & Lu, Yanda & Zhao, Peng & Wen, Chaokai & Shi, Lin & Hu, Zhe, 2022. "A review on proton exchange membrane multi-stack fuel cell systems: architecture, performance, and power management," Applied Energy, Elsevier, vol. 310(C).
    6. Chen, Huicui & Zhang, Ruirui & Xia, Zhifeng & Weng, Qianyao & Zhang, Tong & Pei, Pucheng, 2023. "Experimental investigation on PEM fuel cell flooding mitigation under heavy loading condition," Applied Energy, Elsevier, vol. 349(C).
    7. Zhu, Li & Chen, Junghui, 2018. "Prognostics of PEM fuel cells based on Gaussian process state space models," Energy, Elsevier, vol. 149(C), pages 63-73.
    8. Ye, Lingfeng & Qiu, Diankai & Peng, Linfa & Lai, Xinmin, 2024. "Conduction mechanism analysis and modeling of different gas diffusion layers for PEMFC to improve their bulk conductivities via microstructure design," Applied Energy, Elsevier, vol. 362(C).
    9. Zhang, Shuanyang & Liu, Shun & Xu, Hongtao & Liu, Gaojie & Wang, Ke, 2022. "Performance of proton exchange membrane fuel cells with honeycomb-like flow channel design," Energy, Elsevier, vol. 239(PB).
    10. Hua, Zhiguang & Zheng, Zhixue & Péra, Marie-Cécile & Gao, Fei, 2020. "Remaining useful life prediction of PEMFC systems based on the multi-input echo state network," Applied Energy, Elsevier, vol. 265(C).
    11. Zhang, Xin & Zhang, Chunlei & Zhang, Zhijin & Gao, Sen & Li, He, 2024. "Coordinated management of oxygen excess ratio and cathode pressure for PEMFC based on synthesis variable-gain robust predictive control," Applied Energy, Elsevier, vol. 367(C).
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