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Thermodynamics and regeneration studies of CO2 adsorption on activated carbon

Author

Listed:
  • Qigang Cen
  • Mengxiang Fang
  • Tao Wang
  • Izabela Majchrzak‐Kucęba
  • Dariusz Wawrzyńczak
  • Zhongyang Luo

Abstract

The kinetic and thermodynamic studies of CO2 adsorption on activated carbon were carried out in a fixed bed. Six different CO2 concentrations (from 5% up to 18 vol.%) and four temperatures (303 K, 313 K, 323 K, and 333 K) were applied to investigate dynamic adsorption behaviors. It showed that the increase in temperature led to faster adsorption kinetics, but also reduced the adsorption capacity. An isotherms modeling was made by the Langmuir isotherm model. The experimental isotherms data were well fitted. Then, based on the adsorption isotherms, the isosteric heats of CO2 adsorption were determined by Clausius‐Clapeyron equation. The calculated isosteric heat declined slightly with the adsorbed amount on activated carbon, and had an average value of 16.09 kJ/mol, which is much lower than the actual heat of adsorption measured by calorimeter. Moreover, regeneration experiments by vacuum evacuation (

Suggested Citation

  • Qigang Cen & Mengxiang Fang & Tao Wang & Izabela Majchrzak‐Kucęba & Dariusz Wawrzyńczak & Zhongyang Luo, 2016. "Thermodynamics and regeneration studies of CO2 adsorption on activated carbon," Greenhouse Gases: Science and Technology, Blackwell Publishing, vol. 6(6), pages 787-796, December.
    • Handle: RePEc:wly:greenh:v:6:y:2016:i:6:p:787-796
    DOI: 10.1002/ghg.1621
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    References listed on IDEAS

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    1. Leung, Dennis Y.C. & Caramanna, Giorgio & Maroto-Valer, M. Mercedes, 2014. "An overview of current status of carbon dioxide capture and storage technologies," Renewable and Sustainable Energy Reviews, Elsevier, vol. 39(C), pages 426-443.
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    1. Akinola, Toluleke E. & Bonilla Prado, Phebe L. & Wang, Meihong, 2022. "Experimental studies, molecular simulation and process modelling\simulation of adsorption-based post-combustion carbon capture for power plants: A state-of-the-art review," Applied Energy, Elsevier, vol. 317(C).
    2. Hu, Xiayi (Eric) & Liu, Libin & Luo, Xiao & Xiao, Gongkui & Shiko, Elenica & Zhang, Rui & Fan, Xianfeng & Zhou, Yefeng & Liu, Yang & Zeng, Zhaogang & Li, Chao'en, 2020. "A review of N-functionalized solid adsorbents for post-combustion CO2 capture," Applied Energy, Elsevier, vol. 260(C).
    3. Hongyu Zhao & Xiaona Luo & Haijiao Zhang & Nannan Sun & Wei Wei & Yuhan Sun, 2018. "Carbon†based adsorbents for post†combustion capture: a review," Greenhouse Gases: Science and Technology, Blackwell Publishing, vol. 8(1), pages 11-36, February.

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