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Research of Proton Exchange Membrane Fuel Cell Modeling on Concentration Polarization under Variable-Temperature Operating Conditions

Author

Listed:
  • Teng Teng

    (School of Mechanical, Electronic and Control Engineering, Beijing Jiaotong University, Beijing 100044, China)

  • Xin Zhang

    (School of Mechanical, Electronic and Control Engineering, Beijing Jiaotong University, Beijing 100044, China)

  • Qicheng Xue

    (School of Mechanical, Electronic and Control Engineering, Beijing Jiaotong University, Beijing 100044, China)

  • Baodi Zhang

    (School of Mechanical, Electronic and Control Engineering, Beijing Jiaotong University, Beijing 100044, China)

Abstract

In this study, a concentration overvoltage model that focuses on describing variable-temperature operating condition properties for PEMFCs is established. Sensitivity analysis and a quantification study of oxygen transport resistance are carried out based on the oxygen transport resistance model and measurement data. By analyzing the influence of temperature on cathode oxygen transport resistance, the key structural parameters of the cathode oxygen transport resistance models are estimated, and the parameter modification method of fuel cell limiting current density under variable temperatures is proposed. Based on the polarization curve test experiments under variable-temperature conditions, it is demonstrated that the newly developed concentration overvoltage model reduces the relative error of simulation for a low Pt loading fuel cell in the high current region by 2.97% and 10.06% at 60 °C and 80 °C, respectively. The newly established concentration overvoltage model of a PEMFC solves the problem that the parameter of limiting current density is set without considering the influence of fuel cell temperature fluctuation, which leads to the poor simulation accuracy of the concentration overvoltage model in the high current region.

Suggested Citation

  • Teng Teng & Xin Zhang & Qicheng Xue & Baodi Zhang, 2024. "Research of Proton Exchange Membrane Fuel Cell Modeling on Concentration Polarization under Variable-Temperature Operating Conditions," Energies, MDPI, vol. 17(3), pages 1-17, February.
    • Handle: RePEc:gam:jeners:v:17:y:2024:i:3:p:730-:d:1332725
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    References listed on IDEAS

    as
    1. Hou, Yuze & Deng, Hao & Pan, Fengwen & Chen, Wenmiao & Du, Qing & Jiao, Kui, 2019. "Pore-scale investigation of catalyst layer ingredient and structure effect in proton exchange membrane fuel cell," Applied Energy, Elsevier, vol. 253(C), pages 1-1.
    2. Song Yan & Mingyang Yang & Chuanyu Sun & Sichuan Xu, 2023. "Liquid Water Characteristics in the Compressed Gradient Porosity Gas Diffusion Layer of Proton Exchange Membrane Fuel Cells Using the Lattice Boltzmann Method," Energies, MDPI, vol. 16(16), pages 1-18, August.
    3. He, Pu & Mu, Yu-Tong & Park, Jae Wan & Tao, Wen-Quan, 2020. "Modeling of the effects of cathode catalyst layer design parameters on performance of polymer electrolyte membrane fuel cell," Applied Energy, Elsevier, vol. 277(C).
    4. Liu, Jia Xing & Guo, Hang & Ye, Fang & Ma, Chong Fang, 2017. "Two-dimensional analytical model of a proton exchange membrane fuel cell," Energy, Elsevier, vol. 119(C), pages 299-308.
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