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Liquid Water Characteristics in the Compressed Gradient Porosity Gas Diffusion Layer of Proton Exchange Membrane Fuel Cells Using the Lattice Boltzmann Method

Author

Listed:
  • Song Yan

    (School of Automotive Studies, Tongji University, Shanghai 201804, China)

  • Mingyang Yang

    (School of Automotive Studies, Tongji University, Shanghai 201804, China)

  • Chuanyu Sun

    (School of Electrical Engineering & Automation, Harbin Institute of Technology, Harbin 150001, China)

  • Sichuan Xu

    (School of Automotive Studies, Tongji University, Shanghai 201804, China)

Abstract

The mitigation of water flooding in the gas diffusion layer (GDL) at relatively high current densities is indispensable for enhancing the performance of proton exchange membrane fuel cells (PEMFCs). In this paper, a 2D multicomponent LBM model is developed to investigate the effects of porosity distribution and compression on the liquid water dynamic behaviors and distribution. The results suggest that adopting the gradient GDL structure with increasing porosity along the thickness direction significantly reduces the breakthrough time and steady–state total water saturation inside the GDL. Moreover, the positive gradient structure reaches the highest breakthrough time and water saturation at 10% compression ratio (CR) when the GDL is compressed, and the corresponding values decrease with further increase of the CR. Considering the breakthrough time, total water saturation and water distribution at the entrance of the GDL at the same time, the gradient structure with continuously increasing porosity can perform better water management capacity at 30% CR. This paper is useful for understanding the two–phase process in a gradient GDL structure and provides guidance for future design and manufacturing.

Suggested Citation

  • Song Yan & Mingyang Yang & Chuanyu Sun & Sichuan Xu, 2023. "Liquid Water Characteristics in the Compressed Gradient Porosity Gas Diffusion Layer of Proton Exchange Membrane Fuel Cells Using the Lattice Boltzmann Method," Energies, MDPI, vol. 16(16), pages 1-18, August.
    • Handle: RePEc:gam:jeners:v:16:y:2023:i:16:p:6010-:d:1218709
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    References listed on IDEAS

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    1. Pourrahmani, Hossein & Van herle, Jan, 2022. "Water management of the proton exchange membrane fuel cells: Optimizing the effect of microstructural properties on the gas diffusion layer liquid removal," Energy, Elsevier, vol. 256(C).
    2. Abdul Ghani Olabi & Tabbi Wilberforce & Abdulrahman Alanazi & Parag Vichare & Enas Taha Sayed & Hussein M. Maghrabie & Khaled Elsaid & Mohammad Ali Abdelkareem, 2022. "Novel Trends in Proton Exchange Membrane Fuel Cells," Energies, MDPI, vol. 15(14), pages 1-35, July.
    3. Guo, Lingyi & Chen, Li & Zhang, Ruiyuan & Peng, Ming & Tao, Wen-Quan, 2022. "Pore-scale simulation of two-phase flow and oxygen reactive transport in gas diffusion layer of proton exchange membrane fuel cells: Effects of nonuniform wettability and porosity," Energy, Elsevier, vol. 253(C).
    4. Annunziata D’Orazio & Arash Karimipour & Ramin Ranjbarzadeh, 2023. "Lattice Boltzmann Modelling of Fluid Flow through Porous Media: A Comparison between Pore-Structure and Representative Elementary Volume Methods," Energies, MDPI, vol. 16(14), pages 1-20, July.
    5. Park, Jaeman & Oh, Hwanyeong & Lee, Yoo Il & Min, Kyoungdoug & Lee, Eunsook & Jyoung, Jy-Young, 2016. "Effect of the pore size variation in the substrate of the gas diffusion layer on water management and fuel cell performance," Applied Energy, Elsevier, vol. 171(C), pages 200-212.
    6. Ijaodola, O.S. & El- Hassan, Zaki & Ogungbemi, E. & Khatib, F.N. & Wilberforce, Tabbi & Thompson, James & Olabi, A.G., 2019. "Energy efficiency improvements by investigating the water flooding management on proton exchange membrane fuel cell (PEMFC)," Energy, Elsevier, vol. 179(C), pages 246-267.
    7. Oh, Hwanyeong & Park, Jaeman & Min, Kyoungdoug & Lee, Eunsook & Jyoung, Jy-Young, 2015. "Effects of pore size gradient in the substrate of a gas diffusion layer on the performance of a proton exchange membrane fuel cell," Applied Energy, Elsevier, vol. 149(C), pages 186-193.
    8. Kui Jiao & Jin Xuan & Qing Du & Zhiming Bao & Biao Xie & Bowen Wang & Yan Zhao & Linhao Fan & Huizhi Wang & Zhongjun Hou & Sen Huo & Nigel P. Brandon & Yan Yin & Michael D. Guiver, 2021. "Designing the next generation of proton-exchange membrane fuel cells," Nature, Nature, vol. 595(7867), pages 361-369, July.
    9. Kong, Im Mo & Jung, Aeri & Kim, Young Sang & Kim, Min Soo, 2017. "Numerical investigation on double gas diffusion backing layer functionalized on water removal in a proton exchange membrane fuel cell," Energy, Elsevier, vol. 120(C), pages 478-487.
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