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Mechanisms and kinetics of CO2 hydrogenation to value-added products: A detailed review on current status and future trends

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  • Saeidi, Samrand
  • Najari, Sara
  • Fazlollahi, Farhad
  • Nikoo, Maryam Khoshtinat
  • Sefidkon, Fatemeh
  • Klemeš, Jiří Jaromír
  • Baxter, Larry L.

Abstract

Global warming, fossil fuel depletion and energy security are driving scientists to investigate the mechanism of hydrocarbons production from CO2 hydrogenation. The need for more comprehensive understanding on mechanism of CO2 hydrogenation to hydrocarbons remains controversial because of the complex reaction mechanism and a large number of involved species. The micro mechanism of CO2 hydrogenation to hydrocarbons has been considered as a possible remedy to fulfill the requirements. This review comprehensively discusses two processes: reverse water gas shift (RWGS) and CO2 hydrogenation to hydrocarbons. The review includes reaction mechanisms and catalyst effects on yields and rates. In addition, the review outlines each of the Fischer-Tropsch (FT) micro mechanisms. The review infers some mechanisms from existing work and proposes a new mechanism that improves several predictions. These mechanisms form the design basis for optimal reactor design.

Suggested Citation

  • Saeidi, Samrand & Najari, Sara & Fazlollahi, Farhad & Nikoo, Maryam Khoshtinat & Sefidkon, Fatemeh & Klemeš, Jiří Jaromír & Baxter, Larry L., 2017. "Mechanisms and kinetics of CO2 hydrogenation to value-added products: A detailed review on current status and future trends," Renewable and Sustainable Energy Reviews, Elsevier, vol. 80(C), pages 1292-1311.
  • Handle: RePEc:eee:rensus:v:80:y:2017:i:c:p:1292-1311
    DOI: 10.1016/j.rser.2017.05.204
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    References listed on IDEAS

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    1. Ail, Snehesh Shivananda & Dasappa, S., 2016. "Biomass to liquid transportation fuel via Fischer Tropsch synthesis – Technology review and current scenario," Renewable and Sustainable Energy Reviews, Elsevier, vol. 58(C), pages 267-286.
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    3. Budzianowski, Wojciech M., 2012. "Value-added carbon management technologies for low CO2 intensive carbon-based energy vectors," Energy, Elsevier, vol. 41(1), pages 280-297.
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    5. Budzianowski, Wojciech M. & Postawa, Karol, 2017. "Renewable energy from biogas with reduced carbon dioxide footprint: Implications of applying different plant configurations and operating pressures," Renewable and Sustainable Energy Reviews, Elsevier, vol. 68(P2), pages 852-868.
    6. Leung, Dennis Y.C. & Caramanna, Giorgio & Maroto-Valer, M. Mercedes, 2014. "An overview of current status of carbon dioxide capture and storage technologies," Renewable and Sustainable Energy Reviews, Elsevier, vol. 39(C), pages 426-443.
    7. Gabriele Centi & Siglinda Perathoner, 2011. "CO 2 ‐based energy vectors for the storage of solar energy," Greenhouse Gases: Science and Technology, Blackwell Publishing, vol. 1(1), pages 21-35, March.
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    1. repec:eee:energy:v:147:y:2018:i:c:p:187-196 is not listed on IDEAS

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