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Recent progress in the thermal and catalytic conversion of lignin

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  • Ha, Jeong-Myeong
  • Hwang, Kyung-Ran
  • Kim, Young-Min
  • Jae, Jungho
  • Kim, Kwang Ho
  • Lee, Hyung Won
  • Kim, Jae-Young
  • Park, Young-Kwon

Abstract

The issues over increases in energy demand and environmental pollution attributed to excessive use of fossil fuel have been the driving forces of the exploration for eco-friendly resource. Lignocellulosic biomass consisting of carbohydrates and lignin can be a renewable feedstock for replacing fossil fuels in the future because it is a plentiful and carbon neutral material. Especially, lignin, cross-linked phenolic polymers, is a topic of interest owing to its abundant production from pulp/paper industries as well as lignocellulose based biorefinery. The large potential of platform chemicals and biofuels from lignin has opened up an extensive range of opportunities to develop thermal and catalytic conversion technology. Over a few decades, several lignin conversion processes including catalytic pyrolysis, catalytic depolymerization, and catalytic oxidation have been developed to improve target products yields and to suppress side reactions. More recently, lignin-first approaches which maintain carbohydrates intact by selective extraction of lignin as valuable phenolics from whole biomass has been suggested. This review introduces recent ten years progress on thermal and catalytic conversion technology in terms of process type, catalyst development, and target products. This review is expected to offer an influential information for future research into the thermal and catalytic conversion of lignin as well as lignocellulosic feedstock.

Suggested Citation

  • Ha, Jeong-Myeong & Hwang, Kyung-Ran & Kim, Young-Min & Jae, Jungho & Kim, Kwang Ho & Lee, Hyung Won & Kim, Jae-Young & Park, Young-Kwon, 2019. "Recent progress in the thermal and catalytic conversion of lignin," Renewable and Sustainable Energy Reviews, Elsevier, vol. 111(C), pages 422-441.
    • Handle: RePEc:eee:rensus:v:111:y:2019:i:c:p:422-441
    DOI: 10.1016/j.rser.2019.05.034
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    4. Nwosu, Ugochukwu & Wang, Aiguo & Palma, Bruna & Zhao, Heng & Khan, Mohd Adnan & Kibria, Md & Hu, Jinguang, 2021. "Selective biomass photoreforming for valuable chemicals and fuels: A critical review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 148(C).
    5. Radhakrishnan, Rokesh & Patra, Pradipta & Das, Manali & Ghosh, Amit, 2021. "Recent advancements in the ionic liquid mediated lignin valorization for the production of renewable materials and value-added chemicals," Renewable and Sustainable Energy Reviews, Elsevier, vol. 149(C).
    6. Fan, Yongsheng & Lu, Dongsheng & Han, Yue & Yang, Jiaheng & Qian, Cheng & Li, Binyu, 2023. "Production of light aromatics from biomass components co-pyrolyzed with polyethylene via non-thermal plasma synergistic upgrading," Energy, Elsevier, vol. 265(C).
    7. Huang, Youwang & Wang, Haiyong & Zhang, Xinghua & Zhang, Qi & Wang, Chenguang & Ma, Longlong, 2022. "Accurate prediction of chemical exergy of technical lignins for exergy-based assessment on sustainable utilization processes," Energy, Elsevier, vol. 243(C).
    8. Wang, Bin & Wang, Shuang-Fei & Lam, Su Shiung & Sonne, Christian & Yuan, Tong-Qi & Song, Guo-Yong & Sun, Run-Cang, 2020. "A review on production of lignin-based flocculants: Sustainable feedstock and low carbon footprint applications," Renewable and Sustainable Energy Reviews, Elsevier, vol. 134(C).

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