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Process integration and optimization for economical production of commodity chemicals from lignocellulosic biomass

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  • Choe, Bomin
  • Lee, Shinje
  • Won, Wangyun

Abstract

We propose an integrated strategy for the production of vital platform chemicals, levoglucosenone (LGO) and 5-hydroxymethylfurfural (HMF), used to produce a high-value chemical, 1,6-hexandiol, from lignocellulosic biomass. In such processes of producing essential chemicals from biomass, cellulose loading in the solvent has a significant impact on production yield and, consequently, the economics of the process. In this study, we compare four different loadings of 1, 3, 5, and 10 wt% to suggest the optimal cellulose loading in tetrahydrofuran. The integrated process is economically optimal at a cellulose loading of 5 wt%. The minimum selling price (MSP) of the LGO and HMF mixture is estimated to be $2387/ton, which is competitive compared with the previously reported MSP of $2920/ton (He et al. Green Chemistry,19, 3642–3653, 2017), at the optimal loading of 5 wt%.

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  • Choe, Bomin & Lee, Shinje & Won, Wangyun, 2020. "Process integration and optimization for economical production of commodity chemicals from lignocellulosic biomass," Renewable Energy, Elsevier, vol. 162(C), pages 242-248.
    • Handle: RePEc:eee:renene:v:162:y:2020:i:c:p:242-248
    DOI: 10.1016/j.renene.2020.07.111
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    References listed on IDEAS

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    1. Jung, Wonho & Park, Junhyung & Won, Wangyun & Lee, Kwang Soon, 2018. "Simulated moving bed adsorption process based on a polyethylenimine-silica sorbent for CO2 capture with sensible heat recovery," Energy, Elsevier, vol. 150(C), pages 950-964.
    2. Won, Wangyun & Maravelias, Christos T., 2017. "Thermal fractionation and catalytic upgrading of lignocellulosic biomass to biofuels: Process synthesis and analysis," Renewable Energy, Elsevier, vol. 114(PB), pages 357-366.
    3. Wang, Haiyong & Zhu, Changhui & Li, Dan & Liu, Qiying & Tan, Jin & Wang, Chenguang & Cai, Chiliu & Ma, Longlong, 2019. "Recent advances in catalytic conversion of biomass to 5-hydroxymethylfurfural and 2, 5-dimethylfuran," Renewable and Sustainable Energy Reviews, Elsevier, vol. 103(C), pages 227-247.
    4. Huang, Kefeng & Won, Wangyun & Barnett, Kevin J. & Brentzel, Zachary J. & Alonso, David M. & Huber, George W. & Dumesic, James A. & Maravelias, Christos T., 2018. "Improving economics of lignocellulosic biofuels: An integrated strategy for coproducing 1,5-pentanediol and ethanol," Applied Energy, Elsevier, vol. 213(C), pages 585-594.
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    Cited by:

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    2. Wiranarongkorn, K. & Im-orb, K. & Patcharavorachot, Y. & Maréchal, F. & Arpornwichanop, A., 2023. "Comparative techno-economic and energy analyses of integrated biorefinery processes of furfural and 5-hydroxymethylfurfural from biomass residue," Renewable and Sustainable Energy Reviews, Elsevier, vol. 175(C).
    3. Kim, H. & Baek, S. & Won, W., 2022. "Integrative technical, economic, and environmental sustainability analysis for the development process of biomass-derived 2,5-furandicarboxylic acid," Renewable and Sustainable Energy Reviews, Elsevier, vol. 157(C).
    4. Bangalore Ashok, Rahul Prasad & Oinas, Pekka & Forssell, Susanna, 2022. "Techno-economic evaluation of a biorefinery to produce γ-valerolactone (GVL), 2-methyltetrahydrofuran (2-MTHF) and 5-hydroxymethylfurfural (5-HMF) from spruce," Renewable Energy, Elsevier, vol. 190(C), pages 396-407.

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