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Simulated moving bed adsorption process based on a polyethylenimine-silica sorbent for CO2 capture with sensible heat recovery

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  • Jung, Wonho
  • Park, Junhyung
  • Won, Wangyun
  • Lee, Kwang Soon

Abstract

A simulated moving bed (SMB) adsorption process with heat integration was numerically investigated and is proposed as a viable option for CO2 capture. An amine-functionalized silica sorbent, 0.37 EB-PEI, was used for the SMB process. The process was configured by directly converting a moving bed process; it consists of four separate stages with internal plate heat exchangers for adsorption, cooling, heating, and desorption. The proposed process was extended to the multi-bed scale for continuous capture of CO2 and full integration of the heat produced during the process. A dynamic simulator was constructed to analyze the process behavior, focusing on the energy demand under various operating conditions. As a result, the proposed SMB process was estimated to require 255 kWh/t-CO2 of energy up to CO2 liquefaction; this work reveals the potential of the SMB process for commercial carbon capture through further improvement of the sorbent material.

Suggested Citation

  • Jung, Wonho & Park, Junhyung & Won, Wangyun & Lee, Kwang Soon, 2018. "Simulated moving bed adsorption process based on a polyethylenimine-silica sorbent for CO2 capture with sensible heat recovery," Energy, Elsevier, vol. 150(C), pages 950-964.
    • Handle: RePEc:eee:energy:v:150:y:2018:i:c:p:950-964
    DOI: 10.1016/j.energy.2018.03.022
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    References listed on IDEAS

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    1. Mondal, Monoj Kumar & Balsora, Hemant Kumar & Varshney, Prachi, 2012. "Progress and trends in CO2 capture/separation technologies: A review," Energy, Elsevier, vol. 46(1), pages 431-441.
    2. Lara, Y. & Martínez, A. & Lisbona, P. & Romeo, L.M., 2016. "Heat integration of alternative Ca-looping configurations for CO2 capture," Energy, Elsevier, vol. 116(P1), pages 956-962.
    3. Woosung Choi & Kyungmin Min & Chaehoon Kim & Young Soo Ko & Jae Wan Jeon & Hwimin Seo & Yong-Ki Park & Minkee Choi, 2016. "Epoxide-functionalization of polyethyleneimine for synthesis of stable carbon dioxide adsorbent in temperature swing adsorption," Nature Communications, Nature, vol. 7(1), pages 1-8, November.
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    Citations

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    Cited by:

    1. Li, Shuangjun & Yuan, Xiangzhou & Deng, Shuai & Zhao, Li & Lee, Ki Bong, 2021. "A review on biomass-derived CO2 adsorption capture: Adsorbent, adsorber, adsorption, and advice," Renewable and Sustainable Energy Reviews, Elsevier, vol. 152(C).
    2. Vogtenhuber, H. & Hofmann, R. & Helminger, F. & Schöny, G., 2018. "Process simulation of an efficient temperature swing adsorption concept for biogas upgrading," Energy, Elsevier, vol. 162(C), pages 200-209.
    3. Jung, Wonho & Lee, Kwang Soon, 2019. "Novel short-cut estimation method for the optimum total energy demand of solid sorbents in an adsorption-based CO2 capture process," Energy, Elsevier, vol. 180(C), pages 640-648.
    4. Jung, Wonho & Lee, Jinwon, 2022. "Thermodynamic and kinetic modeling of a novel polyamine-based solvent for energy-efficient CO2 capture with energy analysis," Energy, Elsevier, vol. 239(PE).
    5. Choe, Bomin & Lee, Shinje & Won, Wangyun, 2020. "Process integration and optimization for economical production of commodity chemicals from lignocellulosic biomass," Renewable Energy, Elsevier, vol. 162(C), pages 242-248.
    6. Jung, Wonho & Lee, Jinwon, 2022. "Economic evaluation for four different solid sorbent processes with heat integration for energy-efficient CO2 capture based on PEI-silica sorbent," Energy, Elsevier, vol. 238(PC).
    7. Park, Junhyung & Won, Wangyun & Jung, Wonho & Lee, Kwang Soon, 2019. "One-dimensional modeling of a turbulent fluidized bed for a sorbent-based CO2 capture process with solid–solid sensible heat exchange," Energy, Elsevier, vol. 168(C), pages 1168-1180.
    8. Jung, Wonho & Lee, Jinwon, 2022. "Pseudo counter-current turbulent fluidized bed process with sensible heat recovery for energy-efficient CO2 capture using an amine-functionalized solid sorbent," Energy, Elsevier, vol. 240(C).
    9. Nie, Lijuan & Jin, Junsu & Chen, Jian & Mi, Jianguo, 2018. "Preparation and performance of amine-based polyacrylamide composite beads for CO2 capture," Energy, Elsevier, vol. 161(C), pages 60-69.

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