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A novel nickel catalyst supported on activated coal fly ash for syngas production via biogas dry reforming

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  • Gao, Yuchen
  • Jiang, Jianguo
  • Meng, Yuan
  • Aihemaiti, Aikelaimu
  • Ju, Tongyao
  • Chen, Xuejing
  • Yan, Feng

Abstract

In this study, we prepared novel Ni catalysts via wet impregnation of a support formed of industrial solid waste. Raw, alkali-treated, and alkali/acid co-treated coal fly ash were used for the first time as support for biogas dry reforming catalysts. The proposed two-step activation approach was highly effective in improving the surface area and changing the elemental composition of supports, thus enhancing the activity of the Ni catalysts. All catalysts prepared in this study effectively catalyzed the biogas dry reforming reaction; the catalyst using alkali/acid co-treated coal fly ash as support exhibited the best catalytic activity, with CH4 and CO2 conversion rates exceeding 95%, and good stability during 12 h of biogas dry reforming at 850 °C. This catalyst is highly competitive in terms of both activity and stability compared with most current Ni catalysts formed using commercial SiO2 supports. This study provides a new method for high-value application of coal fly ash, facilitating the manufacture of promising catalysts for biogas dry reforming.

Suggested Citation

  • Gao, Yuchen & Jiang, Jianguo & Meng, Yuan & Aihemaiti, Aikelaimu & Ju, Tongyao & Chen, Xuejing & Yan, Feng, 2020. "A novel nickel catalyst supported on activated coal fly ash for syngas production via biogas dry reforming," Renewable Energy, Elsevier, vol. 149(C), pages 786-793.
    • Handle: RePEc:eee:renene:v:149:y:2020:i:c:p:786-793
    DOI: 10.1016/j.renene.2019.12.096
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    References listed on IDEAS

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    1. Budzianowski, Wojciech M., 2016. "A review of potential innovations for production, conditioning and utilization of biogas with multiple-criteria assessment," Renewable and Sustainable Energy Reviews, Elsevier, vol. 54(C), pages 1148-1171.
    2. Aramouni, Nicolas Abdel Karim & Touma, Jad G. & Tarboush, Belal Abu & Zeaiter, Joseph & Ahmad, Mohammad N., 2018. "Catalyst design for dry reforming of methane: Analysis review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 82(P3), pages 2570-2585.
    3. Hakawati, Rawan & Smyth, Beatrice M. & McCullough, Geoffrey & De Rosa, Fabio & Rooney, David, 2017. "What is the most energy efficient route for biogas utilization: Heat, electricity or transport?," Applied Energy, Elsevier, vol. 206(C), pages 1076-1087.
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    2. Iulianelli, Adolfo & Brunetti, Adele & Pino, Lidia & Italiano, Cristina & Ferrante, Giovanni Drago & Gensini, Mario & Vita, Antonio, 2023. "An integrated two stages inorganic membrane-based system to generate and recover decarbonized H2: An experimental study and performance indexes analysis," Renewable Energy, Elsevier, vol. 210(C), pages 472-485.
    3. Parente, Marcelo & Soria, M.A. & Madeira, Luis M., 2020. "Hydrogen and/or syngas production through combined dry and steam reforming of biogas in a membrane reactor: A thermodynamic study," Renewable Energy, Elsevier, vol. 157(C), pages 1254-1264.
    4. Darmansyah, Darmansyah & You, Sheng-Jie & Wang, Ya-Fen, 2023. "Advancements of coal fly ash and its prospective implications for sustainable materials in Southeast Asian countries: A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 188(C).
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