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Improved hydrogen storage dynamics of amorphous and nanocrystalline Ce-Mg-Ni-based CeMg12-type alloys synthesized by ball milling

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  • Zhang, Yanghuan
  • Zhang, Wei
  • Bu, Wengang
  • Cai, Ying
  • Qi, Yan
  • Guo, Shihai

Abstract

In this paper, we applied ball milling technique to prepare amorphous and nanocrystalline CeMg11Ni + x wt.% Ni (x = 100, 200) alloys which gaseous and electrochemical hydrogen storage dynamics and structure characteristics were systematically studied. It is shown that increasing Ni proportion promotes the amorphization of alloys, meanwhile, it improves their gaseous and electrochemical hydrogenation dynamics significantly. Besides, adjusting milling duration markedly changes the hydrogen storage performances. With the prolonging of milling time, the hydrogen storage capacity has a maximal value, which are 5.949 wt.% and 6.157 wt.% respectively for x = 100 and 200 alloys, while the dehydriding rate always increases. The hydriding rate and high rate discharge ability have the maximal values with the variation of milling time as well. The improved gaseous hydrogen storage dynamics is convinced to be connected with the reduction of dehydrogenation activation energy resulted by increasing Ni proportion and prolonging milling duration.

Suggested Citation

  • Zhang, Yanghuan & Zhang, Wei & Bu, Wengang & Cai, Ying & Qi, Yan & Guo, Shihai, 2019. "Improved hydrogen storage dynamics of amorphous and nanocrystalline Ce-Mg-Ni-based CeMg12-type alloys synthesized by ball milling," Renewable Energy, Elsevier, vol. 132(C), pages 167-175.
    • Handle: RePEc:eee:renene:v:132:y:2019:i:c:p:167-175
    DOI: 10.1016/j.renene.2018.07.134
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    References listed on IDEAS

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    1. Won, Wangyun & Kwon, Hweeung & Han, Jee-Hoon & Kim, Jiyong, 2017. "Design and operation of renewable energy sources based hydrogen supply system: Technology integration and optimization," Renewable Energy, Elsevier, vol. 103(C), pages 226-238.
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    6. Matsunaga, T. & Buchter, F. & Miwa, K. & Towata, S. & Orimo, S. & Züttel, A., 2008. "Magnesium borohydride: A new hydrogen storage material," Renewable Energy, Elsevier, vol. 33(2), pages 193-196.
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    Cited by:

    1. Salehabadi, Ali & Morad, Norhashimah & Ahmad, Mardiana Idayu, 2020. "A study on electrochemical hydrogen storage performance of β-copper phthalocyanine rectangular nanocuboids," Renewable Energy, Elsevier, vol. 146(C), pages 497-503.
    2. Yong, Hui & Guo, Shihai & Yuan, Zeming & Qi, Yan & Zhao, Dongliang & Zhang, Yanghuan, 2020. "Catalytic effect of in situ formed Mg2Ni and REHx (RE: Ce and Y) on thermodynamics and kinetics of Mg-RE-Ni hydrogen storage alloy," Renewable Energy, Elsevier, vol. 157(C), pages 828-839.
    3. Yong, Hui & Wei, Xin & Hu, Jifan & Yuan, Zeming & Wu, Ming & Zhao, Dongliang & Zhang, Yanghuan, 2020. "Influence of Fe@C composite catalyst on the hydrogen storage properties of Mg–Ce–Y based alloy," Renewable Energy, Elsevier, vol. 162(C), pages 2153-2165.
    4. Zheng, Jianpeng & Chen, Liubiao & Liu, Xuming & Zhu, Honglai & Zhou, Yuan & Wang, Junjie, 2020. "Thermodynamic optimization of composite insulation system with cold shield for liquid hydrogen zero-boil-off storage," Renewable Energy, Elsevier, vol. 147(P1), pages 824-832.

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