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An experimental based optimization of a novel water lean amine solvent for post combustion CO2 capture process

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  • Hwang, Junhyeok
  • Kim, Jeongnam
  • Lee, Hee Won
  • Na, Jonggeol
  • Ahn, Byoung Sung
  • Lee, Sang Deuk
  • Kim, Hoon Sik
  • Lee, Hyunjoo
  • Lee, Ung

Abstract

The development of new amine solvents without the major drawbacks of conventional amines is crucial to industrial applications of CO2 capture. This paper presents a water-lean CO2 capture solvent having a low regeneration energy and low degradation. The water-lean solvent, K2Sol, is a sterically hindered diamine; because of the hindered amine site, K2Sol easily forms bicarbonate, resulting in a high absorption capacity. The minimum solvent regeneration energy is obtained using Gaussian process Bayesian optimization (GPBO) and bench-scale pilot plant experiments. GPBO finds the optimal solution using the input and output relationship of experiments; thus, expensive first-principle model construction can be avoided. According to the pilot plant experiment, the optimal regeneration energies of monoethanolamine (MEA) and K2Sol are 4.3 and 2.8 GJ/t CO2, respectively, indicating that K2Sol requires only 65% of the regeneration energy of MEA. Fewer than 30 experiments are required to find the optimal pilot plant operation for both the MEA and K2Sol experiments. We also describe the superior properties of K2Sol in terms of the CO2 loading, cyclic capacity, regeneration temperature, and degradation.

Suggested Citation

  • Hwang, Junhyeok & Kim, Jeongnam & Lee, Hee Won & Na, Jonggeol & Ahn, Byoung Sung & Lee, Sang Deuk & Kim, Hoon Sik & Lee, Hyunjoo & Lee, Ung, 2019. "An experimental based optimization of a novel water lean amine solvent for post combustion CO2 capture process," Applied Energy, Elsevier, vol. 248(C), pages 174-184.
    • Handle: RePEc:eee:appene:v:248:y:2019:i:c:p:174-184
    DOI: 10.1016/j.apenergy.2019.04.135
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    References listed on IDEAS

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    2. Zhao, Jun & Fu, Jianxin & Deng, Shuai & Wang, Junyao & Xu, Yaofeng, 2020. "Decoupled thermal-driven absorption-based CO2 capture into heat engine plus carbon pump: A new understanding with the case study," Energy, Elsevier, vol. 210(C).
    3. Fu, Kun & Zheng, Mingzhen & Wang, Haijie & Fu, Dong, 2022. "Effect of water content on the characteristics of CO2 capture processes in absorbents of 2-ethylhexan-1-amine + diglyme," Energy, Elsevier, vol. 244(PA).
    4. Miriam Navarrete Procopio & Gustavo Urquiza & Laura Castro, 2023. "Analysis of Absorber Packed Height for Power Plants with Post-Combustion CO 2 Capture," Sustainability, MDPI, vol. 15(12), pages 1-17, June.
    5. Fu, Kun & Zheng, Mingzhen & Fu, Dong, 2023. "Low partial pressure CO2 capture in packed tower by EHA+Diglyme water-lean absorbent," Energy, Elsevier, vol. 266(C).
    6. Kim, Jeongnam & Na, Jonggeol & Kim, Kyeongsu & Bak, Ji Hyun & Lee, Hyunjoo & Lee, Ung, 2021. "Learning the properties of a water-lean amine solvent from carbon capture pilot experiments," Applied Energy, Elsevier, vol. 283(C).
    7. Muhammad Imran & Usman Ali & Ali Hasnain, 2021. "Impact of blends of aqueous amines on absorber intercooling for post combustion CO2 capture system," Energy & Environment, , vol. 32(5), pages 921-944, August.
    8. Won, Yooseob & Kim, Jae-Young & Park, Young Cheol & Yi, Chang-Keun & Nam, Hyungseok & Woo, Je-Min & Jin, Gyoung-Tae & Park, Jaehyeon & Lee, Seung-Yong & Jo, Sung-Ho, 2020. "Post-combustion CO2 capture process in a circulated fluidized bed reactor using 200 kg potassium-based sorbent: The optimization of regeneration condition," Energy, Elsevier, vol. 208(C).

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