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Modeling of PEM fuel cell with thin MEA under low humidity operating condition

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  • Li, Yubai
  • Zhou, Zhifu
  • Liu, Xianglei
  • Wu, Wei-Tao

Abstract

Compared to conventional proton exchange membrane (PEM) fuel cell with thick membrane electrode assembly, today’s automotive PEM fuel cell adopts thin MEA with thin catalyst coated membrane (CCM). The objective of this modeling study is to shed light on PEM fuel cell with thin MEA under low humidity operation condition. The effects of cathode catalyst oxygen reduction reaction activity and local O2 transport resistance on automotive PEM fuel cell high current operation are elucidated. The local O2 transport resistance is found to have large impacts on limiting current density. The effects of cathode humidifier elimination, operating pressure, and stoichiometry ratio on PEM fuel cell performance are also discussed. The thin membrane in thin MEA has much lower ohmic resistance compared with thick membrane, and it is easy to be hydrated under low humidity condition. But H2 crossover is stronger for thin membrane and needs to be watched out when thinning the membrane. In addition, a 50 cm2 PEM fuel cell with counter-cross flow field is simulated for demonstration of medium scale PEM fuel cell modeling. Under 0.65 V and 50%/0% humidity operating conditions, the 50 cm2 PEM fuel cell is predicted to supply average current density of 2.51 A/cm2.

Suggested Citation

  • Li, Yubai & Zhou, Zhifu & Liu, Xianglei & Wu, Wei-Tao, 2019. "Modeling of PEM fuel cell with thin MEA under low humidity operating condition," Applied Energy, Elsevier, vol. 242(C), pages 1513-1527.
    • Handle: RePEc:eee:appene:v:242:y:2019:i:c:p:1513-1527
    DOI: 10.1016/j.apenergy.2019.03.189
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    5. Milos Milanovic & Verica Radisavljevic-Gajic, 2019. "Multi-Timescale-Based Partial Optimal Control of a Proton-Exchange Membrane Fuel Cell," Energies, MDPI, vol. 13(1), pages 1-24, December.
    6. Vu, Hoang Nghia & Truong Le Tri, Dat & Nguyen, Huu Linh & Kim, Younghyeon & Yu, Sangseok, 2023. "Multifunctional bypass valve for water management and surge protection in a proton-exchange membrane fuel cell supply-air system," Energy, Elsevier, vol. 278(C).
    7. Pandu Ranga Tirumalasetti & Fang-Bor Weng & Mangaliso Menzi Dlamini & Chia-Hung Chen, 2024. "Numerical Simulation of Double Layered Wire Mesh Integration on the Cathode for a Proton Exchange Membrane Fuel Cell (PEMFC)," Energies, MDPI, vol. 17(2), pages 1-15, January.
    8. Zhang, Qinguo & Tong, Zheming & Tong, Shuiguang & Cheng, Zhewu, 2021. "Self-humidifying effect of air self-circulation system for proton exchange membrane fuel cell engines," Renewable Energy, Elsevier, vol. 164(C), pages 1143-1155.
    9. Wei, Pengnan & Chang, Guofeng & Fan, Ruijia & Xu, Yiming & Chen, Siqi, 2023. "Investigation of output performance and temperature distribution uniformity of PEMFC based on Pt loading gradient design," Applied Energy, Elsevier, vol. 352(C).
    10. Hou, Junbo & Yang, Min & Ke, Changchun & Zhang, Junliang, 2020. "Control logics and strategies for air supply in PEM fuel cell engines," Applied Energy, Elsevier, vol. 269(C).
    11. Abdollahipour, Armin & Sayyaadi, Hoseyn, 2022. "A novel electrochemical refrigeration system based on the combined proton exchange membrane fuel cell-electrolyzer," Applied Energy, Elsevier, vol. 316(C).
    12. Ruzzante, Pascal & Li, Xianguo, 2023. "3D hybrid stochastic reconstruction of catalyst layers in proton exchange membrane fuel cells from 2D images," Energy, Elsevier, vol. 281(C).
    13. Yao, Jing & Wu, Zhen & Wang, Huan & Yang, Fusheng & Xuan, Jin & Xing, Lei & Ren, Jianwei & Zhang, Zaoxiao, 2022. "Design and multi-objective optimization of low-temperature proton exchange membrane fuel cells with efficient water recovery and high electrochemical performance," Applied Energy, Elsevier, vol. 324(C).
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