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Synthesis of dry sorbents for carbon dioxide capture using coal fly ash and its performance

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  • Lee, Jaehee
  • Han, Sang-Jun
  • Wee, Jung-Ho

Abstract

The present paper investigates the application of raw coal fly ash (FA) to dry-based CO2 fixation. Dry sorbents are manufactured by mixing FA, NaOH, CaO and a small amount of water and their absorption behavior, performance, regeneration and leaching efficiency are analyzed. The CO2 absorption efficiency (AE) of FA-added sorbent (WNCF) is higher than that of FA-free sorbents (WNC) and its absorption behavior is improved. In addition, CO2 desorption from carbonated WNCF (CWNCF) occurs at 100°C lower than that from carbonated WNC (CWNC) and its desorption efficiency is 16.5% point higher than that of CWNC, due to the FA addition to the sorbent. However, the AE of regenerated CWNCF is substantially lower than that of fresh WNCF, which indicates that CWNCF cannot easily be regenerated by simple desorption increasing temperature. This is ascribed to the effect of the added FA and water in contributing to the production of Ca- and Na-based carbonated materials that cannot readily be regenerated during the carbonation. Some of the inherent K and Ca components present in the raw FA participate in the carbonation of WNCF, and Cr is co-precipitated during WNCF carbonation to become a stabilized material.

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  • Lee, Jaehee & Han, Sang-Jun & Wee, Jung-Ho, 2014. "Synthesis of dry sorbents for carbon dioxide capture using coal fly ash and its performance," Applied Energy, Elsevier, vol. 131(C), pages 40-47.
    • Handle: RePEc:eee:appene:v:131:y:2014:i:c:p:40-47
    DOI: 10.1016/j.apenergy.2014.06.009
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    3. Ji, Long & Yu, Hai & Li, Kangkang & Yu, Bing & Grigore, Mihaela & Yang, Qi & Wang, Xiaolong & Chen, Zuliang & Zeng, Ming & Zhao, Shuaifei, 2018. "Integrated absorption-mineralisation for low-energy CO2 capture and sequestration," Applied Energy, Elsevier, vol. 225(C), pages 356-366.
    4. Li, Yingjie & Su, Mengying & Xie, Xin & Wu, Shuimu & Liu, Changtian, 2015. "CO2 capture performance of synthetic sorbent prepared from carbide slag and aluminum nitrate hydrate by combustion synthesis," Applied Energy, Elsevier, vol. 145(C), pages 60-68.
    5. Hosseini, Tahereh & Haque, Nawshad & Selomulya, Cordelia & Zhang, Lian, 2016. "Mineral carbonation of Victorian brown coal fly ash using regenerative ammonium chloride – Process simulation and techno-economic analysis," Applied Energy, Elsevier, vol. 175(C), pages 54-68.
    6. Guo, Yafei & Zhao, Chuanwen & Chen, Xiaoping & Li, Changhai, 2015. "CO2 capture and sorbent regeneration performances of some wood ash materials," Applied Energy, Elsevier, vol. 137(C), pages 26-36.

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