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A comparative study of different carbon fuels in an electrolyte-supported hybrid direct carbon fuel cell

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  • Xu, Xiaoyong
  • Zhou, Wei
  • Liang, Fengli
  • Zhu, Zhonghua

Abstract

An electrolyte-supported hybrid direct carbon fuel cell (DCFC) was used to evaluate the performance of different carbon fuels in this study. The direct carbon fuel cell consists of a samarium doped ceria (SDC) electrolyte, a Ni/SDC anode and a Ba0.5Sr0.5Co0.8Fe0.2O3−δ cathode. Three types of carbon (graphite, coal and activated carbon) and three particle sizes of activated carbon (70, 250 and 500μm) were investigated at 650–750°C. The electrochemical reactivity of these three types of carbon fuels was in the order of activated carbon>German creek coal>graphite. Sulphur in German creek coal has poisoning effect on Ni catalyst resulting in lower power density of the fuel cells. The activated carbon (250μm) fuelled hybrid DCFC achieved a peak power density of 158.3mWcm−2 at 750°C along with the maximum current density of 561.5mAcm−2. However, the stability of the hybrid DCFC is poor and need to be improved at the present.

Suggested Citation

  • Xu, Xiaoyong & Zhou, Wei & Liang, Fengli & Zhu, Zhonghua, 2013. "A comparative study of different carbon fuels in an electrolyte-supported hybrid direct carbon fuel cell," Applied Energy, Elsevier, vol. 108(C), pages 402-409.
    • Handle: RePEc:eee:appene:v:108:y:2013:i:c:p:402-409
    DOI: 10.1016/j.apenergy.2013.03.053
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    References listed on IDEAS

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    1. Zongping Shao & Sossina M. Haile, 2004. "A high-performance cathode for the next generation of solid-oxide fuel cells," Nature, Nature, vol. 431(7005), pages 170-173, September.
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    2. Cai, Weizi & Zhou, Qian & Xie, Yongmin & Liu, Jiang & Long, Guohui & Cheng, Shuang & Liu, Meilin, 2016. "A direct carbon solid oxide fuel cell operated on a plant derived biofuel with natural catalyst," Applied Energy, Elsevier, vol. 179(C), pages 1232-1241.
    3. Duan, Nan-Qi & Cao, Yong & Hua, Bin & Chi, Bo & Pu, Jian & Luo, Jingli & Jian, Li, 2016. "Tubular direct carbon solid oxide fuel cells with molten antimony anode and refueling feasibility," Energy, Elsevier, vol. 95(C), pages 274-278.
    4. Hao, Wenbin & Mi, Yongli, 2016. "Evaluation of waste paper as a source of carbon fuel for hybrid direct carbon fuel cells," Energy, Elsevier, vol. 107(C), pages 122-130.
    5. Juan Carlos Henao (Editor) & María del Pilar García Pachón (Editor), 2016. "Minería y desarrollo. Tomo 2: Medio ambiente y desarrollo sostenible," Books, Universidad Externado de Colombia, Facultad de Derecho, number 878, October.
    6. Hao, Wenbin & He, Xiaojin & Mi, Yongli, 2014. "Achieving high performance in intermediate temperature direct carbon fuel cells with renewable carbon as a fuel source," Applied Energy, Elsevier, vol. 135(C), pages 174-181.
    7. Qu, Jifa & Wang, Wei & Chen, Yubo & Deng, Xiang & Shao, Zongping, 2016. "Stable direct-methane solid oxide fuel cells with calcium-oxide-modified nickel-based anodes operating at reduced temperatures," Applied Energy, Elsevier, vol. 164(C), pages 563-571.
    8. Jiao, Yong & Tian, Wenjuan & Chen, Huili & Shi, Huangang & Yang, Binbin & Li, Chao & Shao, Zongping & Zhu, Zhenping & Li, Si-Dian, 2015. "In situ catalyzed Boudouard reaction of coal char for solid oxide-based carbon fuel cells with improved performance," Applied Energy, Elsevier, vol. 141(C), pages 200-208.
    9. Guo, Liang & Calo, J.M. & Kearney, Clare & Grimshaw, Pengpeng, 2014. "The anodic reaction zone and performance of different carbonaceous fuels in a batch molten hydroxide direct carbon fuel cell," Applied Energy, Elsevier, vol. 129(C), pages 32-38.

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