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Oxidation-resistant all-perovskite tandem solar cells in substrate configuration

Author

Listed:
  • Yurui Wang

    (Nanjing University)

  • Renxing Lin

    (Nanjing University)

  • Xiaoyu Wang

    (Jilin University)

  • Chenshuaiyu Liu

    (Nanjing University)

  • Yameen Ahmed

    (University of Victoria)

  • Zilong Huang

    (Nanjing University)

  • Zhibin Zhang

    (Peking University)

  • Hongjiang Li

    (Nanjing University)

  • Mei Zhang

    (Nanjing University)

  • Yuan Gao

    (Nanjing University)

  • Haowen Luo

    (Nanjing University)

  • Pu Wu

    (Nanjing University)

  • Han Gao

    (Nanjing University)

  • Xuntian Zheng

    (Nanjing University)

  • Manya Li

    (Nanjing University)

  • Zhou Liu

    (Nanjing University)

  • Wenchi Kong

    (Nanjing University)

  • Ludong Li

    (Nanjing University)

  • Kaihui Liu

    (Peking University)

  • Makhsud I. Saidaminov

    (University of Victoria)

  • Lijun Zhang

    (Jilin University)

  • Hairen Tan

    (Nanjing University)

Abstract

The commonly-used superstrate configuration (depositing front subcell first and then depositing back subcell) in all-perovskite tandem solar cells is disadvantageous for long-term stability due to oxidizable narrow-bandgap perovskite assembled last and easily exposable to air. Here we reverse the processing order and demonstrate all-perovskite tandems in a substrate configuration (depositing back subcell first and then depositing front subcell) to bury oxidizable narrow-bandgap perovskite deep in the device stack. By using guanidinium tetrafluoroborate additive in wide-bandgap perovskite subcell, we achieve an efficiency of 25.3% for the substrate-configured all-perovskite tandem cells. The unencapsulated devices exhibit no performance degradation after storage in dry air for 1000 hours. The substrate configuration also widens the choice of flexible substrates: we achieve 24.1% and 20.3% efficient flexible all-perovskite tandem solar cells on copper-coated polyethylene naphthalene and copper metal foil, respectively. Substrate configuration offers a promising route to unleash the commercial potential of all-perovskite tandem solar cells.

Suggested Citation

  • Yurui Wang & Renxing Lin & Xiaoyu Wang & Chenshuaiyu Liu & Yameen Ahmed & Zilong Huang & Zhibin Zhang & Hongjiang Li & Mei Zhang & Yuan Gao & Haowen Luo & Pu Wu & Han Gao & Xuntian Zheng & Manya Li & , 2023. "Oxidation-resistant all-perovskite tandem solar cells in substrate configuration," Nature Communications, Nature, vol. 14(1), pages 1-11, December.
    • Handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-37492-y
    DOI: 10.1038/s41467-023-37492-y
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    References listed on IDEAS

    as
    1. Alexander D. Jodlowski & Cristina Roldán-Carmona & Giulia Grancini & Manuel Salado & Maryline Ralaiarisoa & Shahzada Ahmad & Norbert Koch & Luis Camacho & Gustavo de Miguel & Mohammad Khaja Nazeeruddi, 2017. "Large guanidinium cation mixed with methylammonium in lead iodide perovskites for 19% efficient solar cells," Nature Energy, Nature, vol. 2(12), pages 972-979, December.
    2. Zhibin Yang & Zhenhua Yu & Haotong Wei & Xun Xiao & Zhenyi Ni & Bo Chen & Yehao Deng & Severin N. Habisreutinger & Xihan Chen & Kang Wang & Jingjing Zhao & Peter N. Rudd & Joseph J. Berry & Matthew C., 2019. "Enhancing electron diffusion length in narrow-bandgap perovskites for efficient monolithic perovskite tandem solar cells," Nature Communications, Nature, vol. 10(1), pages 1-9, December.
    3. Weijun Ke & Mercouri G. Kanatzidis, 2019. "Prospects for low-toxicity lead-free perovskite solar cells," Nature Communications, Nature, vol. 10(1), pages 1-4, December.
    4. Renxing Lin & Ke Xiao & Zhengyuan Qin & Qiaolei Han & Chunfeng Zhang & Mingyang Wei & Makhsud I. Saidaminov & Yuan Gao & Jun Xu & Min Xiao & Aidong Li & Jia Zhu & Edward H. Sargent & Hairen Tan, 2019. "Monolithic all-perovskite tandem solar cells with 24.8% efficiency exploiting comproportionation to suppress Sn(ii) oxidation in precursor ink," Nature Energy, Nature, vol. 4(10), pages 864-873, October.
    5. Tomas Leijtens & Kevin A. Bush & Rohit Prasanna & Michael D. McGehee, 2018. "Opportunities and challenges for tandem solar cells using metal halide perovskite semiconductors," Nature Energy, Nature, vol. 3(10), pages 828-838, October.
    6. Ludong Li & Yurui Wang & Xiaoyu Wang & Renxing Lin & Xin Luo & Zhou Liu & Kun Zhou & Shaobing Xiong & Qinye Bao & Gang Chen & Yuxi Tian & Yu Deng & Ke Xiao & Jinlong Wu & Makhsud I. Saidaminov & Hongz, 2022. "Flexible all-perovskite tandem solar cells approaching 25% efficiency with molecule-bridged hole-selective contact," Nature Energy, Nature, vol. 7(8), pages 708-717, August.
    7. Dewei Zhao & Cong Chen & Changlei Wang & Maxwell M. Junda & Zhaoning Song & Corey R. Grice & Yue Yu & Chongwen Li & Biwas Subedi & Nikolas J. Podraza & Xingzhong Zhao & Guojia Fang & Ren-Gen Xiong & K, 2018. "Efficient two-terminal all-perovskite tandem solar cells enabled by high-quality low-bandgap absorber layers," Nature Energy, Nature, vol. 3(12), pages 1093-1100, December.
    8. Renxing Lin & Jian Xu & Mingyang Wei & Yurui Wang & Zhengyuan Qin & Zhou Liu & Jinlong Wu & Ke Xiao & Bin Chen & So Min Park & Gang Chen & Harindi R. Atapattu & Kenneth R. Graham & Jun Xu & Jia Zhu & , 2022. "All-perovskite tandem solar cells with improved grain surface passivation," Nature, Nature, vol. 603(7899), pages 73-78, March.
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