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Moisture-triggered fast crystallization enables efficient and stable perovskite solar cells

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  • Kaikai Liu

    (Huaqiao University)

  • Yujie Luo

    (Huaqiao University)

  • Yongbin Jin

    (Huaqiao University)

  • Tianxiao Liu

    (Henan Normal University)

  • Yuming Liang

    (Huaqiao University)

  • Liu Yang

    (Huaqiao University)

  • Peiquan Song

    (Huaqiao University)

  • Zhiyong Liu

    (Henan Normal University)

  • Chengbo Tian

    (Huaqiao University)

  • Liqiang Xie

    (Huaqiao University)

  • Zhanhua Wei

    (Huaqiao University)

Abstract

Understanding the function of moisture on perovskite is challenging since the random environmental moisture strongly disturbs the perovskite structure. Here, we develop various N2-protected characterization techniques to comprehensively study the effect of moisture on the efficient cesium, methylammonium, and formamidinium triple-cation perovskite (Cs0.05FA0.75MA0.20)Pb(I0.96Br0.04)3. In contrast to the secondary measurements, the established air-exposure-free techniques allow us directly monitor the influence of moisture during perovskite crystallization. We find a controllable moisture treatment for the intermediate perovskite can promote the mass transportation of organic salts, and help them enter the buried bottom of the films. This process accelerates the quasi-solid-solid reaction between organic salts and PbI2, enables a spatially homogeneous intermediate phase, and translates to high-quality perovskites with much-suppressed defects. Consequently, we obtain a champion device efficiency of approaching 24% with negligible hysteresis. The devices exhibit an average T80-lifetime of 852 h (maximum 1210 h) working at the maximum power point.

Suggested Citation

  • Kaikai Liu & Yujie Luo & Yongbin Jin & Tianxiao Liu & Yuming Liang & Liu Yang & Peiquan Song & Zhiyong Liu & Chengbo Tian & Liqiang Xie & Zhanhua Wei, 2022. "Moisture-triggered fast crystallization enables efficient and stable perovskite solar cells," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
    • Handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-32482-y
    DOI: 10.1038/s41467-022-32482-y
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    References listed on IDEAS

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    1. Yujie Luo & Kaikai Liu & Liu Yang & Wenjing Feng & Lingfang Zheng & Lina Shen & Yongbin Jin & Zheng Fang & Peiquan Song & Wanjia Tian & Peng Xu & Yuqing Li & Chengbo Tian & Liqiang Xie & Zhanhua Wei, 2023. "Dissolved-Cl2 triggered redox reaction enables high-performance perovskite solar cells," Nature Communications, Nature, vol. 14(1), pages 1-10, December.

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